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Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…

The sensitivity of molecular fingerprinting is dramatically improved when placing the absorbing sample in a high-finesse optical cavity, thanks to the large increase of the effective path-length. As demonstrated recently, when the…

Dual-frequency comb spectroscopy has emerged as a disruptive technique for measuring wide-spanning spectra with high resolution, yielding a particularly powerful technique for sensitive multi-component gas analysis. We present a…

Optical frequency combs have the potential to improve the precision of the radial velocity measurement of celestial bodies, leading to breakthroughs in such fields as exoplanet exploration. For these purposes, the comb must have a broad…

Instrumentation and Methods for Astrophysics · Physics 2023-06-06 Keisuke Nakamura , Ken Kashiwagi , Sho Okubo , Hajime Inaba

Multi-dimensional coherent spectroscopy (MDCS)1,2 is a powerful method for optical spectroscopy that has become an important tool for studying ultrafast dynamics in a wide range of systems. It is an optical analog of multidimensional…

Optics · Physics 2018-10-24 Bachana Lomsadze , Brad. C. Smith , Steven T. Cundiff

Dual comb spectroscopy allows for high-resolution spectra to be measured over broad bandwidths, but an essential requirement for coherent integration is the availability of a phase reference. Usually, this means that the combs' phase and…

Optics · Physics 2016-06-01 David Burghoff , Yang Yang , Qing Hu

The search for earth-like exoplanets with the Doppler radial velocity technique is an extremely challenging and multifaceted precision spectroscopy problem. Currently, one of the limiting instrumental factors in reaching the required…

Rapid characterization of optical and vibrational spectra with high resolution can identify species in cluttered environments and is important for assays and early alerts. In this regard, dual-comb spectroscopy has emerged as a powerful…

Optics · Physics 2016-12-21 Myoung-Gyun Suh , Qi-Fan Yang , Ki Youl Yang , Xu Yi , Kerry Vahala

We propose a new approach to near-infrared molecular spectroscopy, harnessing advanced concepts of optical telecommunications and supercontinuum photonics. We generate, without mode-locked lasers, two frequency combs of slightly different…

Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…

High finesse frequency combs (HFC) with large ratio of the frequency spacing to the width of the spectral components have demonstrated remarkable results in many applications such as precision spectroscopy and metrology. We found that low…

Optical frequency combs are key to optical precision measurements. While most frequency combs operate in the near-infrared regime, many applications require combs at mid-infrared, visible or even ultra-violet wavelengths. Frequency combs…

Broadband dual-comb spectroscopy (DCS) based on portable mode-locked fiber frequency combs is a powerful tool for in situ, calibration free, multi-species spectroscopy. While the acquisition of a single spectrum with mode-locked DCS…

Optics · Physics 2021-02-03 Nazanin Hoghooghi , Ryan K. Cole , Gregory B. Rieker

Optical frequency combs based on mode-locked lasers have proven to be invaluable tools for a wide range of applications in precision spectroscopy and metrology. A novel principle of optical frequency comb generation in whispering-gallery…

Optics · Physics 2015-06-12 Pascal Del'Haye , Scott B. Papp , Scott A. Diddams

Cavity-enhanced frequency comb spectroscopy for molecule detection in the mid-infrared powerfully combines high resolution, high sensitivity, and broad spectral coverage. However, this technique, and essentially all spectroscopic methods,…

A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…

Optics · Physics 2009-11-13 Ian Coddington , William C. Swann , Nathan R. Newbury

Optical frequency comb, as a spectrum made of discrete and equally spaced spectral lines, is a light source with essential applications in modern technology. Cavity optomechanical systems were found to be a feasible candidate for realizing…

Optics · Physics 2024-08-13 Xin Gu , Jinlian Zhang , Shulin Ding , Xiaoshun Jiang , Bing He , Qing Lin