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Motivated by theoretical and experimental studies reported by Yamaguchi et al. (Phys. Rev. B 98, 094402 (2018)), we performed a cluster mean-field analysis of an anisotropic Heisenberg model with six competing exchange interactions. We…

Strongly Correlated Electrons · Physics 2025-07-04 L. M. Ramos , F. M. Zimmer , M. Schmidt

This study presents the experimental realization of a spin-1/2 zigzag-square lattice in a verdazyl-based complex, namely ($m$-Py-V-2,6-F$_2$)$[$Cu(hfac)$_2]$. Molecular orbital calculations suggest the presence of five types of frustrated…

We present a new model compound with the S = 1/2 frustrated square lattice composed of the charge-transfer salt (o-MePy-V)PF6. Ab initio calculations indicate the formation of an S = 1/2 square lattice, in which six types of…

Strongly Correlated Electrons · Physics 2018-09-26 H. Yamaguchi , Y. Sasaki , T. Okubo , M. Yoshida , T. Kida , M. Hagiwara , Y. Kono , S. Kittaka , T. Sakakibara , M. Takigawa , Y. Iwasaki , Y. Hosokoshi

We present Quantum Monte-Carlo simulations of an exchange-anisotropic spin-1/2 Heisenberg model on a square lattice with nearest and next-nearest neighbor interactions. The ground state phase diagram shows two classical magnetically ordered…

Strongly Correlated Electrons · Physics 2012-12-20 A. Kalz , A. Honecker , S. Fuchs , T. Pruschke

Geometric frustration among competing spin exchanges can give rise to novel quantum phases by enhancing fluctuations that drive magnetic systems beyond the classical regime. We investigate the frustrated array of strongly correlated spin…

The spin-1/2 Ising-Heisenberg model on martini and martini-diced lattice is exactly solved using a star-triangle transformation, which affords an exact mapping correspondence to an effective spin-1/2 Ising model on a triangular lattice. The…

Statistical Mechanics · Physics 2022-03-23 Hamid Arian Zad , Jozef Strecka

Using exact numerical diagonalization and the conformal field theory approach, we study the effect of magnetic frustrations due to diagonal exchange bonds in a system of two coupled mixed-spin $(1,{1/2})$ Heisenberg chains. It is…

Strongly Correlated Electrons · Physics 2009-11-10 N. B. Ivanov , J. Richter

We study the ground-state phase diagram of a Heisenberg model with spin $S=\frac{1}{2}$ on a diamond-like decorated square lattice. A diamond unit has two types of antiferromagnetic exchange interactions, and the ratio $\lambda$ between the…

Statistical Mechanics · Physics 2016-12-21 Yuhei Hirose , Akihide Oguchi , Yoshiyuki Fukumoto

We investigate the quantum spin-1/2 zigzag chain with frustrated $J_1$-$J_2$ Heisenberg interactions, incorporating additional off-diagonal exchange interactions known as the $\Gamma$ term, both with and without an applied magnetic field.…

Strongly Correlated Electrons · Physics 2024-08-02 Hidehiro Saito , Chisa Hotta

We present a model compound with a spin-1/2 frustrated square lattice, in which three ferromagnetic (F) interactions and one antiferromagnetic (AF) compet. Considering the effective spin-1 formed by the dominant F dimer, this square lattice…

Strongly Correlated Electrons · Physics 2021-08-31 H. Yamaguchi , N. Uemoto , T. Okubo , Y. Kono , S. Kittaka , T. Sakakibara , T. Yajima , S. Shimono , Y. Iwasaki , Y. Hosokoshi

By means of the recently developed algorithm based on the tensor product states, the magnetization process of frustrated spin-1/2 spin-dimer models on a square lattice is investigated. Various field-induced quantum phases are discovered. In…

Strongly Correlated Electrons · Physics 2010-01-26 Pochung Chen , Chen-Yen Lai , Min-Fong Yang

The magnetization process of a frustrated spin-1/2 spin-dimer model on a square lattice is investigated by means of a sign-problem-free quantum Monte Carlo algorithm developed recently. Rich field-induced quantum phases are discovered. We…

Strongly Correlated Electrons · Physics 2017-03-02 Kwai-Kong Ng , Min-Fong Yang

We investigate the phases and phase-transitions in one-dimensional alternating mixed-spin (1/2-1) chain in the presence of both frustration and anisotropy. Frustration is introduced via next-nearest-neighbor interactions, while single-ion…

Strongly Correlated Electrons · Physics 2025-10-31 Soumya Satpathi , Suparna Sarkar , Swapan K. Pati

We successfully synthesized ($p$-Py-V)[Cu(hfac)$_2$], a verdazyl-based complex. Molecular orbital calculations revealed five types of intermolecular interactions between the radical spins and two types of intramolecular interactions between…

We report magnetocaloric and magnetic-torque evidence that in Cs$_{2}$CuBr$_{4}$ -- a geometrically frustrated Heisenberg $S=1/2$ triangular-lattice antiferromagnet -- quantum fluctuations stabilize a series of spin states at simple…

Strongly Correlated Electrons · Physics 2015-05-13 N. A. Fortune , S. T. Hannahs , Y. Yoshida , T. E. Sherline , T. Ono , H. Tanaka , Y. Takano

A large part of the interest in magnets with frustrated antiferromagnetic interactions comes from the many new phases found in applied magnetic field. In this Article, we explore some of the new phases which arise in a model with frustrated…

Strongly Correlated Electrons · Physics 2016-02-29 Luis Seabra , Philippe Sindzingre , Tsutomu Momoi , Nic Shannon

We study the phase diagram of a frustrated spin-1/2 ferromagnetic chain with anisotropic exchange interactions in an external magnetic field, using the density matrix renormalization group method. We show that an easy-axis anisotropy…

Strongly Correlated Electrons · Physics 2009-10-29 F. Heidrich-Meisner , I. P. McCulloch , A. K. Kolezhuk

We consider the spin-1/2 antiferromagnetic Heisenberg model on a bilayer honeycomb lattice including interlayer frustration in the presence of an external magnetic field. In the vicinity of the saturation field, we map the low-energy states…

Strongly Correlated Electrons · Physics 2017-03-22 Taras Krokhmalskii , Vasyl Baliha , Oleg Derzhko , Jörg Schulenburg , Johannes Richter

The spin-$1/2$ Heisenberg chain with a ferromagnetic first-neighbor exchange coupling $J_1$ and an antiferromagnetic second-neighbor $J_2$ has a Haldane dimer ground state with an extremely small spin gap. Thus, the ground state is readily…

Strongly Correlated Electrons · Physics 2020-07-03 Hiroshi Ueda , Shigeki Onoda

We propose a new type of magnetically disordered ground state for a frustrated quantum antiferromagnet. This disordered state is an array of spin singlets spontaneously formed on four spin plaquettes. Both perturbation results and…

Condensed Matter · Physics 2009-10-28 M. E. Zhitomirsky , Kazuo Ueda
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