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Polymers near the glass transition temperature Tg often exhibit a breakdown of time-temperature-superposition (TTS), with chain relaxation times and viscosity exhibiting a weaker temperature dependence than segmental relaxation times. The…

Soft Condensed Matter · Physics 2024-03-05 Peijing Yue , David S. Simmons

We report on an extensive study of craze formation in glassy polymers. Molecular dynamics simulations of a coarse-grained bead-spring model were employed to investigate the molecular level processes during craze nucleation, widening, and…

Materials Science · Physics 2009-11-10 Joerg Rottler , Mark O. Robbins

Observations of time-resolved thermal emission from tidally locked exoplanets can tell us about their atmospheric temperature structure. Telescopes such as JWST and ARIEL will improve the quality and availability of these measurements. This…

Earth and Planetary Astrophysics · Physics 2022-12-28 Neil T. Lewis , Mark Hammond

A parallel pseudospectral code for the direct numerical simulation (DNS) of isotropic turbulence has been developed. The code has been extensively benchmarked using established results from literature. The code has been used to conduct a…

Fluid Dynamics · Physics 2013-06-17 Samuel R. Yoffe

We investigate the strain-rate-dependent mechanical behavior and deformation mechanisms of a refractory high entropy alloy, Ti29Zr24Nb23Hf24 (at.%), with a single-phase body-centered cubic (BCC) structure. High-temperature compression tests…

Materials Science · Physics 2020-12-03 Tangqing Cao , Wenqi Guo , Wang Lu , Yunfei Xue , Wenjun Lu , Jing Su , Christian H. Liebscher , Chang Liu , Gerhard Dehm

Understanding fluctuation-induced breakages in polymers has important implications for basic and applied sciences. Here I present for the first time an analytical treatment of the thermal breakage problem of a semi-flexible polymer model…

Materials Science · Physics 2015-06-12 Chiu Fan Lee

Refractory body-centered cubic (BCC) metals and alloys are of extraordinary importance in modern technological and structural applications. However, their wider adoption in science and technology is severely restricted by low-temperature…

Many glass-forming fluids exhibit a remarkable thermodynamic scaling in which dynamic properties, such as the viscosity, the relaxation time, and the diffusion constant, can be described under different thermodynamic conditions in terms of…

Soft Condensed Matter · Physics 2015-06-16 Wen-Sheng Xu , Karl F. Freed

We study the thermal breakage of a discrete one-dimensional string, with open and fixed ends, in the heavily damped regime. Basing our analysis on the multidimensional Kramers escape theory, we are able to make analytical predictions on the…

Statistical Mechanics · Physics 2009-09-24 Chiu Fan Lee

The research reveals the existence of a constant characteristic time of preparatory micro-structural processes before the onset of macro-failure at various high loading rates of brittle and quasi-brittle materials. The presence of this…

Materials Science · Physics 2023-01-23 Ivan Smirnov

Compression-induced buckling instability of metal thin films on a compliant base result in surface wrinkles. A stiff thin film, perfectly bonded to an infinitely deep pre-stretched dielectric elastomer (DE) substrate, is considered. Linear…

Computational Physics · Physics 2021-08-24 Abhishek Ghosh

The interaction of polymers with small-scale velocity gradients can trigger a coil-stretch transition in the polymers. We analyze this transition within a direct numerical simulation of shear turbulence with an Oldroyd-B model for the…

Chaotic Dynamics · Physics 2009-11-07 Bruno Eckhardt , Jochen Kronjaeger , Joerg Schumacher

The relationship of base pair openings to DNA flexibility is examined. Published experimental data on the temperature dependence of the persistence length by two different groups are well described in terms of an inhomogeneous Kratky-Porot…

Statistical Mechanics · Physics 2012-02-20 Nikos Theodorakopoulos , Michel Peyrard

While of paramount importance in material science, the dynamics of cracks still lacks a complete physical explanation. The transition from their slow creep behavior to a fast propagation regime is a notable key, as it leads to full material…

Motivated by the very low diffusivity recently found in ab initio simulations of liquid water, we have studied its dependence with temperature, system size, and duration of the simulations. We use ab initio molecular dynamics (AIMD),…

Soft Condensed Matter · Physics 2009-11-10 M. V. Fernandez-Serra , Emilio Artacho

Applying constant tensile stress to a piece of amorphous solid results in a slow extension, followed by an eventual rapid mechanical collapse. This "creep" process is of paramount engineering concern, and as such was the subject of study in…

Soft Condensed Matter · Physics 2022-06-08 Bhanu Prasad Bhowmik , H. G. E. Hentschel , Itamar Procaccia

The dynamics of elastocapillary thinning in high molecular weight polymer solutions are re-examined using high-speed digital video microscopy. At long times, the evolution of the viscoelastic thread deviates from self-similar exponential…

Other Condensed Matter · Physics 2009-11-11 Monica S. N. Oliveira , Gareth H. McKinley

We study the stress response to a step strain of covalently bonded gelatin gels in the temperature range where triple helix reversible crosslink formation is prohibited. We observe slow stress relaxation towards a $T$-dependent finite…

Soft Condensed Matter · Physics 2016-03-23 O. Ronsin , C. Caroli , T Baumberger

We study a highly supercooled two-dimensional fluid mixture via molecular dynamics simulation. We follow bond breakage events among particle pairs, which occur on the scale of the $\alpha$ relaxation time $\tau_{\alpha}$. Large scale…

Soft Condensed Matter · Physics 2015-06-25 Ryoichi Yamamoto , Akira Onuki

Breakage is generally understood in mechanical terms, yet nano-structures can rupture not only under external loads but also via thermal activation. Here we treat in a general framework the statistical mechanics of thermally induced…

Statistical Mechanics · Physics 2015-06-16 Cristiano Nisoli , Douglas Abraham , Turab Lookman , Avadh Saxena