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Fully symmetric A1g phonons are expected to play a dominant role in electron scattering in strong topological insulators (TIs), thus limiting the ballistic transport of future electronic devices. Here, we report on femtosecond time-resolved…

Mesoscale and Nanoscale Physics · Physics 2018-02-14 Jianbo Hu , Kyushiro Igarashi , Takao Sasagawa , Kazutaka G. Nakamura , Oleg V. Misochko

Coherent control is an optical technique to manipulate quantum states of matter. The coherent control of 40-THz optical phonons in diamond was demonstrated by using a pair of sub-10-fs optical pulses. The optical phonons were detected via…

Multi-gigahertz mechanical vibrations stemming from interactions between light fields and matter, also known as acoustic phonons, have long been a subject of study. In recent years, specially designed functional devices have been developed…

Optics · Physics 2021-04-14 Mamoru Endo , Shota Kimura , Shuntaro Tani , Yohei Kobayashi

The coherent modulation of electronic and vibrational nonlinearities in atoms and molecular gases by intense few-cycle pulses has been used for high-harmonic generation in the soft X-ray and attosecond regime, as well as for Raman frequency…

Materials Science · Physics 2013-09-16 Muneaki Hase , Masayuki Katsuragawa , Anca Monia Constantinescu , Hrvoje Petek

Using sub-picosecond optical pump-probe techniques, coherent zone-folded longitudinal acoustic phonons (ZFLAPs) were generated and controlled in an InGaN multiple quantum well structure. A one-pump, one-probe differential transmission…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Umit Ozgur , Chang-Won Lee , Henry O. Everitt

Here, we investigate phonon mode- and electron band-selective electron-phonon couplings in centrosymmetric 1T$'$-MoTe$_2$ using time- and angle-resolved photoemission spectroscopy combined with frequency-domain analysis. Femtosecond…

Materials Science · Physics 2026-02-24 Carl E. Jensen , Christoph Emeis , Stephan Jauernik , Petra Hein , Fabio Caruso , Michael Bauer

In this study, coherent phonon motion is observed in bandgap excited CuIn$_{x}$Ga$_{(1-x)}$Se$_2$ (CIGS) utilizing extreme ultraviolet (XUV) attosecond transient absorption spectroscopy across the Se M$_{4,5}$ absorption edge. Two…

Information technology demands high-speed optoelectronic devices, but going beyond the one terahertz (THz) barrier is challenging due to the difficulties associated with generating, detecting, and processing high-frequency signals. Here, we…

Mesoscale and Nanoscale Physics · Physics 2021-11-29 Ziqi Li , Bo Peng , Miao-Ling Lin , Yu-Chen Leng , Bin Zhang , Chi Pang , Ping-Heng Tan , Bartomeu Monserrat , Feng Chen

Excitation of four coherent phonon modes of different symmetries has been realized in copper metaborate CuB$_2$O$_4$ via impulsive stimulated Raman scattering (ISRS). Phonons were detected by monitoring changes in the linear optical…

Ultra-high frequency acoustic resonances ($\backsim$2 GHz) trapped within the glass core ($\backsim$1 $\mu$m diameter) of a photonic crystal fiber are selectively excited through electrostriction using laser pulses of duration 100 ps and…

Optics · Physics 2009-04-05 G. S. Wiederhecker , A. Brenn , H. L. Fragnito , P. St. J. Russell

Coherent and squeezed phonon oscillations can be excited in solids impulsively by a single femtosecond pulse whose duration is shorter that a phonon period. By applying the second ultrafast pump pulse these oscillations can be…

Mesoscale and Nanoscale Physics · Physics 2013-04-30 O. V Misochko

Hybrid spin-mechanical systems provide a platform for integrating quantum registers and transducers. Efficient creation and control of such systems require a comprehensive understanding of the individual spin and mechanical components as…

Using femtosecond pump-probe spectroscopy with pulse shaping techniques, one can generate and detect coherent phonons in chirality-specific semiconducting single-walled carbon nanotubes. The signals are resonantly enhanced when the pump…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 G. D. Sanders , C. J. Stanton , J. -H. Kim , K. -J. Yee , Y. -S. Lim , E. H. Haroz , L. G. Booshehri , J. Kono , R. Saito

Phonons are considered to be universal quantum transducers due to their ability to couple to a wide variety of quantum systems. Among these systems, solid-state point defect spins are known for being long-lived optically accessible quantum…

We report an ultrafast optical spectroscopy study on the coherent phonon dynamics in the topological semimetal CeBi and its nonmagnetic isostructural compound LaBi, revealing profound insights into their electronic and magnetic…

Strongly Correlated Electrons · Physics 2025-07-15 Xu-Chen Nie , Chen Zhang , Qi-Yi Wu , Hao Liu , Jie Pang , You-Guo Shi , Zhi-An Xu , Yan-Feng Guo , Ya-Hua Yuan , H. Y. Liu , Yu-Xia Duan , Jian-Qiao Meng

The excitation and detection of coherent phonons has given unique insights into condensed matter, in particular for materials with strong electron-phonon coupling. We report a study of coherent phonons in the layered charge density wave…

We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between…

Superconductivity · Physics 2015-05-25 R. Mankowsky , M. Först , T. Loew , J. Porras , B. Keimer , A. Cavalleri

We present a transient absorption setup combining broadband detection over the visible-UV range with high temporal resolution ($\sim$20fs) which is ideally suited to trigger and detect vibrational coherences in different classes of…

We report femtosecond time-resolved reflectivity measurements of coherent phonons in tellurium performed over a wide range of temperatures (3K to 296K) and pump laser intensities. A totally symmetric A$_{1}$ coherent phonon at 3.6 THz…

Materials Science · Physics 2015-05-20 N. Kamaraju , Sunil Kumar , M. Anija , A. K. Sood

Quantum coherent coupling between a zone-center phonon and two acoustic phonons was observed in two GaAs/AlAs superlattices (8 nm/8 nm and 5.4 nm/5.4 nm) at ambient temperature. Using degenerate coherent phonon spectroscopy, a multi-cycle…

Materials Science · Physics 2019-07-25 Feng He , Nathanial Sheehan , Seth R Bank , Raymond L Orbach , Yaguo Wang
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