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Related papers: Oxygen vacancies in vanadium dioxide: A DFT$+V$ st…

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First-principles calculations to study the electronic and magnetic properties of bulk, oxygen-deficient SrTiO$_3$ (STO) under different doping conditions and densities have been conducted. The appearance of magnetism in oxygen-deficient STO…

Materials Science · Physics 2016-03-30 Alejandro Lopez-Bezanilla , P. Ganesh , Peter B. Littlewood

Electrons in correlated insulators are prevented from conducting by Coulomb repulsion between them. When an insulator-to-metal transition is induced in a correlated insulator by doping or heating, the resulting conducting state can be…

In this work an overall electronic structure including the position and formation energies of various intrinsic defects are computed for anatase using Density Functional Theory aided by Hubbard correction (DFT+U). The intrinsic point…

In order to study the origin of metallization of VO$_2$ induced by electron injection, we deposit K atoms onto the surface of VO$_2$ films grown on TiO$_2$ (001) substrates, and we investigate the change in the electronic and crystal…

Strongly Correlated Electrons · Physics 2019-03-27 Daisuke Shiga , Makoto Minohara , Miho Kitamura , Ryu Yukawa , Koji Horiba , Hiroshi Kumigashira

In the present work, we investigate oxygen vacancies (V$_\mathrm{O}$) in Co$_3$O$_4$, both in the bulk phase and under liquid-phase ethylene glycol oxidation, by combining theoretical and experimental techniques. Density functional theory…

We have studied electrical switching with S-shaped I-V characteristics in two-terminal MOM devices based on vanadium dioxide thin films. The switching effect is associated with the metal-insulator phase transition. Relaxation oscillations…

Applied Physics · Physics 2020-01-08 Alexander Pergament , Andrei Velichko , Maksim Belyaev , Vadim Putrolaynen

Vanadium dioxide (VO2) is a popular candidate for electronic and optical switching applications due to its well-known semiconductor-metal transition. Its study is notoriously challenging due to the interplay of long and short range elastic…

We present a state-of-the-art density functional theory (DFT) study which models crucial features of the partially disordered orbital order stacking in the prototypical layered transition metal dichalcogenide 1T-TaS2 . Our results not only…

Strongly Correlated Electrons · Physics 2018-12-05 Tobias Ritschel , Helmuth Berger , Jochen Geck

Electrically driven metal-insulator transition in vanadium dioxide (VO2) is of interest in emerging memory devices, neural computation, and high speed electronics. We report on the fabrication of out-of-plane VO2 metal-insulator-metal (MIM)…

Mesoscale and Nanoscale Physics · Physics 2013-07-16 You Zhou , Xiaonan Chen , Changhyun Ko , Zheng Yang , Chandra Mouli , Shriram Ramanathan

The description of the molecular solid phase of O$_2$, especially its ground-state antiferromagnetic insulating phase, is known to be quite unsatisfactory within the conventional local and semilocal density functional approximations used in…

Materials Science · Physics 2017-12-18 Shusuke Kasamatsu , Takeo Kato , Osamu Sugino

We investigated the magnetic and electric properties of nanometer-sized vanadium dioxide (VO$_2$) particles. VO$_2$ nanoparticles were formed by milling VO$_2$ powder. We measured the magnetic field dependence of the magnetization of the…

Materials Science · Physics 2024-04-05 Tsuyoshi Hatano , Akihiro Fukawa , Hiroki Yamamoto , Keiichirou Akiba , Kouichi Takase

Enhanced conductivity at ferroelectric domain walls in BiFeO$_3$ has been widely observed, yet the microscopic origins of this effect, including electronic contributions from domain-wall defects, are incompletely understood at the atomistic…

Materials Science · Physics 2025-07-17 Guo-Dong Zhao , Ismaila Dabo , Long-Qing Chen

To explore the potential of molecular gas treatment of freshly cut lithium foils in non-electrolyte based passivation of high energy-density Li anodes, density functional theory (DFT) has been used to study the decomposition of molecular…

Materials Science · Physics 2015-06-01 Stephan L. Koch , Benjamin J. Morgan , Stefano Passerini , Gilberto Teobaldi

Oxygen vacancies in two-dimensional metal-oxide structures garner much attention due to unique conductive, magnetic and even superconductive functionalities they induce. Ferroelectric domain walls have been a prominent recent example…

Materials Science · Physics 2021-04-22 Hemaprabha Elangovan , Maya Barzilay , Jiawei Huang , Shi Liu , Shai Cohen , Yachin Ivry

Defects such as oxygen vacancy are widely considered to be critical for the performance of HfO2-based devices, and yet atomistic mechanisms underlying various exotic effects such as wake-up and fluid imprint remain elusive. Here, guided by…

Materials Science · Physics 2023-03-03 Liyang Ma , Shi Liu

We present {\it ab initio} LDA+DMFT results for the many-particle density of states of $VO_{2}$ on the metallic side of the strongly first-order ($T$-driven) insulator-metal transition. In strong contrast to LDA predictions, there is {\it…

Strongly Correlated Electrons · Physics 2015-06-24 M. S. Laad , L. Craco , E. Müller-Hartmann

VO2 samples are grown with different oxygen concentrations leading to different monoclinic, M1 and triclinic, T insulating phases which undergo a first order metal to insulator transition (MIT) followed by a structural phase transition…

Materials Science · Physics 2017-05-12 Raktima Basu , Manas Sardar , Santanu Bera , P. Magudapathy , Sandip Dhara

Synchrotron X-ray total scattering studies of structural changes in rutile VO2 at the metal-insulator transition temperature of 340 K reveal that monoclinic and tetragonal phases of VO2 coexist in equilibrium, as expected for a first-order…

Materials Science · Physics 2010-08-10 Serena A. Corr , Daniel P. Shoemaker , Brent C. Melot , Ram Seshadri

We investigate the electronic properties of semi-metallic (12,0) carbon nanotubes in the presence of a variety of mono-, di- and hexa-vacancy defects, by using first principle DFT combined with non-equilibrium Green's function technique. We…

Mesoscale and Nanoscale Physics · Physics 2009-10-08 Hui Zeng , Huifang Hu , Jean-Pierre Leburton

We perform full-potential screened-hybrid density-functional theory (DFT) calculations to compare the thermodynamic stability of neutral and charged states of the surface oxygen vacancy at the rutile TiO$_2$(110) surface. Solid-state…

Materials Science · Physics 2015-08-19 Daniel Berger , Harald Oberhofer , Karsten Reuter