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Cu2(pymca)3(ClO4) (pymca: pyrimidine-2-carboxylate) consists of a slightly distorted honeycomb lattice of Cu2+ spins, which shows no long-range magnetic order down to 0.6 K. A magnetization study revealed 1/3 and 2/3 plateau phases [A.…

Strongly Correlated Electrons · Physics 2025-08-11 Masaaki Matsuda , Alexander I. Kolesnikov , Zentaro Honda , Tokuro Shimokawa , Sho Inoue , Yasuo Narumi , Masayuki Hagiwara

Spin-1/2 chains with alternating antiferromagnetic (AF) and ferromagnetic (FM) couplings exhibit quantum entanglement like the integer-spin Haldane chains and might be similarly utilized for quantum computations. Such alternating AF-FM…

Strongly Correlated Electrons · Physics 2020-12-09 Shang Gao , Ling-Fang Lin , Andrew F. May , Binod K. Rai , Qiang Zhang , Elbio Dagotto , Andrew D. Christianson , Matthew B. Stone

In a recent paper by Schmitt et al. (arXiv:1402.1091), signs of two exchange interactions of one-dimensional alternating chains in distorted honeycomb systems of Na3Cu2SbO6 and Na2Cu2TeO6 are argued by theoretical calculations. Although the…

Strongly Correlated Electrons · Physics 2014-02-28 Masatoshi Sato , Yoshiaki Kobayashi

Spin-$1/2$ chains with alternating antiferromagnetic and ferromagnetic couplings have attracted considerable interest due to the topological character of their spin excitations. Here, using density functional theory and density matrix…

Magnetic excitation spectra of quantum spins of Na3Cu2SbO6 with the distorted honeycomb structure have been measured by neutron inelastic scattering. The intensity distribution and the dispersion curves of the excitations indicate that the…

Strongly Correlated Electrons · Physics 2009-11-13 Yoko Miura , Yukio Yasui , Taketo Moyoshi , Masatoshi Sato , Kazuhisa Kakurai

We report the signatures of dynamic spin fluctuations in the layered honeycomb Li$_3$Cu$_2$SbO$_6$ compound, with a 3$d$ S = 1/2 $d^9$ Cu$^{2+}$ configuration, through muon spin rotation and relaxation ($\mu$SR) and neutron scattering…

Cobalt-based quantum magnets forming layered honeycomb arrangements have attracted much attention recently, as they are considered as a potential platform for materials with exotic Kitaev spin exchange. Amongst the discussed candidate…

Strongly Correlated Electrons · Physics 2026-05-28 Abdul Basit , Richard A. Mole , Alex J. Brown , Jiatu Liu , Chris D. Ling , Stephan Rachel

The microscopic spin-spin correlations in the 2D layered spin-1 honeycomb lattice compound Na2Ni2TeO6 have been investigated by neutron diffraction and inelastic neutron scattering. The honeycomb lattice of spin-1 Ni2+ ions, within the…

Strongly Correlated Electrons · Physics 2022-02-17 A. K. Bera , S. M. Yusuf , L. Keller , F. Yokaichiya , J. R. Stewart

The spin-1/2 alternating Heisenberg chain system Na$_3$Cu$_2$SbO$_6$ features two relevant exchange couplings: $J_{1a}$ within the structural Cu$_2$O$_6$ dimers and $J_{1b}$ between the dimers. Motivated by the controversially discussed…

Strongly Correlated Electrons · Physics 2014-11-13 M. Schmitt , O. Janson , S. Golbs , M. Schmidt , W. Schnelle , J. Richter , H. Rosner

A recent study [Tassel {\it et al.}, Phys. Rev. Lett. {\bf 105}, 167205 (2010)] has proposed a remarkable spin model for (CuCl)LaNb2O7, in which dimers are ferromagnetically coupled to each other on the distorted Shastry-Sutherland lattice.…

Strongly Correlated Electrons · Physics 2011-08-17 Shunsuke Furukawa , Tyler Dodds , Yong Baek Kim

We report on band structure calculations and a microscopic model of the low-dimensional magnet beta-Cu2V2O7. Magnetic properties of this compound can be described by a spin-1/2 anisotropic honeycomb lattice model with the averaged coupling…

Strongly Correlated Electrons · Physics 2010-10-12 Alexander A. Tsirlin , Oleg Janson , Helge Rosner

We investigate the ground-state phase diagram of a spin-1/2 honeycomb-lattice antiferromagnetic (AF) Heisenberg model with three exchange interactions, $J_{\rm A}$, $J_{\rm B}$, and $J_{\rm C}$ that is realized in a distorted…

Strongly Correlated Electrons · Physics 2022-06-29 Tokuro Shimokawa , Ken'ichi Takano , Zentaro Honda , Akira Okutani , Masayuki Hagiwara

The electronic and magnetic structure, including the Heisenberg model exchange interaction parameters, was explored for the recently proposed novel cuprate Cu$_2$F$_5$. Using the DFT+U calculation, it is shown that the compound is formed by…

Strongly Correlated Electrons · Physics 2021-08-11 Dmitry M. Korotin , Dmitry Y. Novoselov , Vladimir I. Anisimov , Artem R. Oganov

Unconventional magnetism including altermagnetism and unconventional compensated magnetism, characterized by its duality of real-space antiferromagnetic alignment and momentum-space spin splitting, has garnered widespread attention. While…

Materials Science · Physics 2025-06-10 Xiao-Yao Hou , Ze-Feng Gao , Huan-Cheng Yang , Peng-Jie Guo , Zhong-Yi Lu

The synthesis, structure, and basic magnetic properties of Na2Co2TeO6 and Na3Co2SbO6 are reported. The crystal structures were determined by neutron powder diffraction. Na2Co2TeO6 has a two-layer hexagonal structure (space group P6322)…

Materials Science · Physics 2022-04-26 L. Viciu , Q. Huang , E. Morosan , H. W. Zandbergen , N. I. Greenbaum , T. McQueen , R. J. Cava

We delineate quantum magnetism in the strongly spin-orbit coupled, distorted honeycomb-lattice antiferromagnet BiYbGeO$_{5}$. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an…

Using thermodynamic measurements and density-functional band-structure calculations, we explore magnetic behavior of SrCuTe2O6. Despite being a structural sibling of a three-dimensional frustrated system PbCuTe2O6, this spin-1/2 quantum…

Materials Science · Physics 2015-06-29 N. Ahmed , A. A. Tsirlin , R. Nath

Two-dimensional high-spin bipartite honeycomb networks, where anisotropy, competing exchange interactions, and spin fluctuations interplay, provide an alternative platform to test theoretical models that distinguish between classical and…

Strongly Correlated Electrons · Physics 2026-05-05 M. Barik , Q. Faure , F. Damay , J. P. Embs , S. Petit , P. Khuntia

A classical-quantum chain composed of regularly alternating Ising and Heisenberg spins is rigorously solved by considering two distinct local anisotropy axes of the Ising spins. The ground-state phase diagram and magnetization curves are…

Strongly Correlated Electrons · Physics 2018-06-13 J. Torrico , J. Strecka , M. Hagiwara , O. Rojas , S. M. de Souza , Y. Han , Z. Honda , M. L. Lyra

Sr$_2$CuTeO$_6$ presents an opportunity for exploring low-dimensional magnetism on a square lattice of $S=1/2$ Cu$^{2+}$ ions. We employ ab initio multi-reference configuration interaction calculations to unravel the Cu$^{2+}$ electronic…

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