English

Quantum disordered ground state in the spin-orbit coupled Jeff = 1/2 distorted honeycomb magnet BiYbGeO5

Strongly Correlated Electrons 2023-05-18 v1 Materials Science

Abstract

We delineate quantum magnetism in the strongly spin-orbit coupled, distorted honeycomb-lattice antiferromagnet BiYbGeO5_{5}. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an effective Jeff=1/2J_{\rm eff}=1/2 Kramers doublet of Yb3+^{3+}. The ground state is nonmagnetic with a tiny spin gap. Temperature-dependent magnetic susceptibility, magnetization isotherm, and heat capacity could be modeled well assuming isolated spin dimers with anisotropic exchange interactions JZ2.6J_{\rm Z} \simeq 2.6~K and JXY1.3J_{\rm XY} \simeq 1.3~K. Heat capacity measurements backed by muon spin relaxation suggest the absence of magnetic long-range order down to at least 80\,mK both in zero field and in applied fields. This sets BiYbGeO5_5 apart from Yb2_2Si2_2O7_7 with its unusual regime of magnon Bose-Einstein condensation and suggests negligible interdimer couplings, despite only a weak structural deformation of the honeycomb lattice.

Keywords

Cite

@article{arxiv.2305.10221,
  title  = {Quantum disordered ground state in the spin-orbit coupled Jeff = 1/2 distorted honeycomb magnet BiYbGeO5},
  author = {S. Mohanty and S. S. Islam and N. Winterhalter-Stocker and A. Jesche and G. Simutis and Ch. Wang and Z. Guguchia and J. Sichelschmidt and M. Baenitz and A. A. Tsirlin and P. Gegenwart and R. Nath},
  journal= {arXiv preprint arXiv:2305.10221},
  year   = {2023}
}

Comments

6 pages, 5 figures