Related papers: Broadly tunable quantum-enhanced Raman microscopy …
Stochastic resonance (SR) could amplify weak electric-field signals in nonlinear systems by means of the externally injected noises. Here we propose and experimentally demonstrate a modified SR method, termed squeezing-induced SR,…
We present a 40-MHz ultrafast optical parametric amplifier (OPA), tunable from 0.8 to 1 $\mu$m, with a relative intensity noise (RIN) matching the shot-noise floor (-160 dB/Hz) above 2 MHz. The OPA is pumped by a 20-W Kerr-lens mode-locked…
Squeezing of collective atomic spins has been shown to improve the sensitivity of atomic clocks and magnetometers to levels significantly below the standard quantum limit. In most cases the requisite atom-atom entanglement has been…
The on-surface synthesis of graphene nanoribbons (GNRs) allows for the fabrication of atomically precise narrow GNRs. Despite their exceptional properties which can be tuned by ribbon width and edge structure, significant challenges remain…
The hotspots, which are typically found in nanogaps between metal structures, are critical for the enhancement of the electromagnetic field. Surface-enhanced Raman scattering (SERS), a technique known for its exceptional sensitivity and…
Raman spectroscopy's capability to provide meaningful composition predictions is heavily reliant on a pre-processing step to remove insignificant spectral variation. This is crucial in biofluid analysis. Widespread adoption of diagnostics…
Spectral compression of femtosecond pulses by second harmonic generation in the presence of substantial group velocity dispersion provides a convenient source of narrowband Raman pump pulses for femtosecond stimulated Raman spectroscopy…
A spectroscopic imaging-scanning tunneling microscope (SI-STM) allows the atomic scale visualization of surface electronic and magnetic structure of novel quantum materials with high energy resolution. To achieve the optimal performance,…
We present super-resolved coherent anti-Stokes Raman scattering (CARS) microscopy by implementing phase-resolved image scanning microscopy (ISM), achieving up to two-fold resolution increase as compared with a conventional CARS microscope.…
Expressions for the two-dimensional Stimulated x-ray Raman Spectroscopy (2D-SXRS) signal obtained using attosecond x-ray pulses are derived. The 1D- and 2D-SXRS signals are calculated for trans-N-methyl acetamide (NMA) with broad bandwidth…
Raman spectroscopy enables non-destructive, label-free molecular analysis with high specificity, making it a powerful tool for biomedical diagnostics. However, its application to biological tissues is challenged by inherently weak Raman…
Quantum squeezed states enable precision measurements beyond the standard quantum limit, but conventional solid-state media fundamentally limit pump intensities to the ionization threshold. We demonstrate that plasma waves can mediate…
Microwave squeezing represents the ultimate sensitivity frontier for superconducting qubit measurement. However, observation of enhancement has remained elusive, in part because integration with conventional dispersive readout pollutes the…
Recovering both amplitude and phase information from a system is a fundamental goal of optical imaging. At the same time, it is crucial to operate at low photon doses to avoid altering the sample, particularly in biological applications.…
Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…
In continuous-variable quantum information processing, it is crucial to develop high-efficiency and broadband quantum memory of squeezed light, which enables the storage of full-bandwidth information. Here, we present a quantum memory of…
We describe a fully ultra-high vacuum compatible scanning tunneling microscope (STM) optimized for radio-frequency signals. It includes in-situ exchangeable tips adapted to high frequency cabling and a standard sample holder, which offer…
The ability to perform nanometer-scale optical imaging and spectroscopy is key to deciphering the low-energy effects in quantum materials, as well as vibrational fingerprints in planetary and extraterrestrial particles, catalytic…
Resonant soft X-ray scattering (RSXS) is a powerful technique for probing both spatial and electronic structures within solid-state systems. We present a newly developed RSXS capability at beamline 13-3 of the Stanford Synchrotron Radiation…
Raman sensing and Raman microscopy are amongst the most specific optical technologies to identify the chemical compounds of unknown samples, and to enable label-free biomedical imaging with molecular contrast. However, the high cost and…