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Hindered adsorbed layers completely filling the nanopores must cause significant deviations from the classical BET isotherms for multimolecular adsorption of vapor in porous solids. Since the point of transition from free to hindered…

Chemical Physics · Physics 2019-01-01 Zdenek P. Bazant , Hoang Thai Nguyen

Molybdenum disulfide (MoS2) has drawn great interest for tunable photonics and optoelectronics advancement. Its solution processing, though scalable, results in randomly networked ensembles of discrete nanosheets with compromised properties…

Liquids under confinement differ in behavior from their bulk counterparts and can acquire properties that are specific to the confined phase and linked to the nature and structure of the host matrix. While confined liquid water is not a new…

Materials Science · Physics 2020-07-22 François-Xavier Coudert

Pattern formation induced by wrinkling is a very common phenomenon exhibited in soft-matter substrates. In all these systems wrinkles develop in presence of compressively stressed thin films lying on compliant substrates. Here we…

Mesoscale and Nanoscale Physics · Physics 2019-03-26 Maria Caterina Giordano , Francesco Buatier de Mongeot

Photoluminescence excitation measurements in semi-conducting carbon nanotubes show a systematic non-resonant contribution between the well known excitonic resonances. Using a global analysis method, we were able to delineate the…

Solution-processed two-dimensional (2D) materials hold promise for their scalable applications. However, the random, fragmented nature of the solution-processed nanoflakes and the poor percolative conduction through their discrete networks…

Reactions at solid-water interfaces play a foundational role in water treatment systems, catalysis, chemical separations, and in predicting chemical fate and transport in the environment. Over the last century, experimental measurements and…

Chemical Physics · Physics 2022-12-14 Anastasia G. Ilgen , Kevin Leung , Louise J. Criscenti , Jeffery A. Greathouse

The microwave absorption and noise caused by quantum two-level systems (TLS) dramatically suppress the coherence in Josephson junction qubits that are promising candidates for a quantum information applications. Microwave absorption by TLSs…

Mesoscale and Nanoscale Physics · Physics 2018-07-04 Alexander L. Burin , Andrii O. Maksymov

The advancement of nanoscale electronics has been limited by energy dissipation challenges for over a decade. Such limitations could be particularly severe for two-dimensional (2D) semiconductors integrated with flexible substrates or…

The success of isolating small flakes of atomically thin layers through mechanical exfoliation has triggered enormous research interest in graphene and other two-dimensional materials. For device applications, however, controlled large-area…

Materials Science · Physics 2014-07-17 Yingnan Liu , Rudresh Ghosh , Di Wu , Ariel Ismach , Rodney Ruoff , Keji Lai

We have studied the adsorption of gas molecules (CO, NO, NO2, O2, N2, CO2, and NH3) on graphene nanoribbons (GNRs) using first principles methods. The adsorption geometries, adsorption energies, charge transfer, and electronic band…

Materials Science · Physics 2008-09-20 Bing Huang , Zuanyi Li , Zhirong Liu , Gang Zhou , Shaogang Hao , Jian Wu , Bing-Lin Gu , Wenhui Duan

The interplay of topology and superconductivity has become a subject of intense research in condensed matter physics for the pursuit of topologically non-trivial forms of superconducting pairing. An intrinsically normal-conducting material…

Due to the drastically different intralayer versus interlayer bonding strengths, the mechanical, thermal, and electrical properties of two-dimensional (2D) materials are highly anisotropic between the in-plane and out-of-plane directions.…

We show here that the morphological pathway of spontaneous dewetting of ultrathin Ag films on SiO2 under nanosecond laser melting is found to be film thickness dependent. For films with thickness h between 2 <= h <= 9.5 nm, the morphology…

Materials Science · Physics 2015-05-18 H. Krishna , R. Sachan , J. Strader , C. Favazza , M. Khenner , Ramki Kalyanaraman

Atomic monolayers represent a novel class of materials to study localized and free excitons in two dimensions and to engineer optoelectronic devices based on their significant optical response. Here, we investigate the role of the substrate…

Mesoscale and Nanoscale Physics · Physics 2017-07-21 Oliver Iff , Yu-Ming He , Nils Lundt , Sebastian Stoll , Vasilij Baumann , Sven Höfling , Christian Schneider

Optical response of artificial composite nanoscale molecules comprising a closely spaced noble metal nanoparticle and a semiconductor quantum dot have been studied theoretically. We consider a system composed of an Au particle and CdSe or…

Quantum Physics · Physics 2010-12-30 A. V. Malyshev , V. A. Malyshev

We present a systematic study of top-down processed GaN/AlN heterostructures for intersubband optoelectronic applications. Samples containing quantum well superlattices that display either near- or mid-infrared intersubband absorption were…

The nanoscale optical properties of high-quality MoS$_2$ nanoribbons are investigated using THz nanoscopy based on a scattering-type scanning probe. The nanoribbons comprise a multi-layer core, surrounded by monolayer edges. A featureless…

In this article, we report the first observation of nanosecond laser induced transient dual absorption bands, one in the bandgap (TA1) and another in the sub-bandgap (TA2) regions of a-Ge5As30Se65 thin films. Strikingly, these bands are…

Materials Science · Physics 2015-09-25 Pritam Khan , Tarun Saxena , K. V. Adarsh

Relating the electromagnetic scattering and absorption properties of an individual particle to the reflection and transmission coefficients of a two-dimensional material composed of these particles is a crucial concept that has driven both…

Optics · Physics 2019-10-02 Romain Dezert , Philippe Richetti , Alexandre Baron