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A detailed study of the structural and magnetic properties of a spin-$5/2$ triangular lattice antiferromagnet RbFe(HPO$_{3}$)$_{2}$ is presented using x-ray diffraction, magnetization, heat capacity, and $^{31}$P nuclear magnetic resonance…

Materials Science · Physics 2025-11-24 V. Nagpal , Sebin J. Sebastian , Surya P. Patra , S. Shibash , Q. -P. Ding , Y. Furukawa , R. Nath

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

Strongly Correlated Electrons · Physics 2021-03-30 J. Khatua , T. Arh , Shashi B. Mishra , H. Luetkens , A. Zorko , B. Sana , M. S. Ramachandra Rao , B. R. K. Nanda , P. Khuntia

We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca$_3$CoNb$_2$O$_9$, in which the effective spin of Co$^{2+}$ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and…

Strongly Correlated Electrons · Physics 2015-12-25 J. Dai , P. Zhou , P. S. Wang , F. Pang , T J. Munsie , G. M. Luke , J. S. Zhang , Weiqiang Yu

Frustrated magnetism in face-centred cubic (fcc) magnetic sublattices remains underexplored but holds considerable potential for exotic magnetic behaviour. Here we report on the crystal structure, magnetic and thermodynamic properties of…

The intermetallic compound Nd$_2$Co$_{0.85}$Si$_{2.88}$ having a triangular lattice could be synthesized in single-phase only with defect crystal structure. Investigation through different experimental techniques indicate the presence of…

Magnetic frustration and disorder are key ingredients to prevent the onset of magnetic order. In the disordered hexagonal double perovskite BaTi$_{1/2}$Mn$_{1/2}$O$_{3}$, Mn$^{4+}$ cations, with $S=3/2$ spins, can either form highly…

Hybrid transition metal oxides continue to attract attention due to their multiple degrees of freedom ($e.g.$, lattice, charge, spin, and orbital) and versatile properties. Here we investigate the magnetic and electronic properties of the…

Strongly Correlated Electrons · Physics 2022-05-17 Ke Yang , Wenjing Xu , Di Lu , Yuxuan Zhou , Lu Liu , Yaozhenghang Ma , Guangyu Wang , Hua Wu

Magnetic properties and magnetic structure of the Ba$_{2}$Mn(PO$_{4}$)$_{2}$ antiferromagnet featuring frustrated zigzag chains of $S=\frac{5}{2}$ Mn$^{2+}$ ions are reported based on neutron diffraction, density-functional band-structure…

Strongly Correlated Electrons · Physics 2018-04-10 Arvind Yogi , A. K. Bera , Ashwin Mohan , Ruta Kulkarni , S. M. Yusuf , A. Hoser , A. A. Tsirlin , A. Thamizhavel

We investigate the magnetic ground state of CuNdO$_2$, which is a delafossite with a triangular lattice of magnetic Nd$^{3+}$ ions that are well separated by non-magnetic Cu spacer layers. From inelastic neutron scattering measurements of…

Structural and magnetic properties of a two-dimensional spin-$\frac{5}{2}$ frustrated triangular lattice antiferromagnet NH$_{4}$Fe(PO$_{3}$F)$_2$ are explored via x-ray diffraction, magnetic susceptibility, high-field magnetization, heat…

Materials Science · Physics 2025-02-11 S. Mohanty , K. M. Ranjith , C. S. Saramgi , Y. Skourski , B. Büchner , H. -J. Grafe , R. Nath

We model changes of magnetic ordering in Mn-antiperovskite nitrides driven by biaxial lattice strain at zero and at finite temperature. We employ a non-collinear spin-polarised density functional theory to compare the response of the…

Strongly Correlated Electrons · Physics 2017-06-07 J. Zemen , E. Mendive Tapia , Z. Gercsi , R. Banerjee , C. E. Patrick , J. B. Staunton , K. G. Sandeman

The usual classical behaviour of S = 3/2, B-site ordered double perovskites generally results in simple, commensurate magnetic ground states. In contrast, heat capacity and neutron powder diffraction measurements for the S = 3/2 systems…

Strongly Correlated Electrons · Physics 2015-06-11 A. A. Aczel , D. E. Bugaris , L. Li , J. -Q. Yan , C. de la Cruz , H. -C. zur Loye , S. E. Nagler

Investigation of the oxygen-deficient 112-type ordered oxides of the type LnBaCoMnO5+\delta (Ln = Nd, Eu) evidences certain unusual magnetic behavior at low temperatures, compared to the LnBaCo2O5+\delta cobaltites. One observes that the…

Materials Science · Physics 2015-05-18 Asish K. Kundu , V. Pralong , B. Raveau , V. Caignaert

We report electron spin resonance (ESR) spectroscopy results on the double perovskite Ba$_2$YIrO$_6$. On general grounds, this material is expected to be nonmagnetic due to the strong coupling of the spin and orbital momenta of Ir$^{5+}$…

Strongly Correlated Electrons · Physics 2018-06-12 S. Fuchs , T. Dey , G. Aslan-Cansever , A. Maljuk , S. Wurmehl , B. Büchner , V. Kataev

We report the crystal structure, magnetization and neutron scattering measurements on the double perovskite Ba$_2$YOsO$_6$. The $Fm\overline{3}m$ space group is found both at 290~K and 3.5~K with cell constants $a_0 = 8.3541(4)$~{\AA} and…

We studied structural and magnetic properties of a series of insulating double perovskite compounds, La$_{2-x}$Sr$_{x}$CuRuO$_{6}$ (0 $\le$ x $\le$ 1), representing doping via \textit{A}-site substitution. The end members…

Strongly Correlated Electrons · Physics 2012-09-19 P. Anil Kumar , R. Mathieu , R. Vijayaraghavan , Subham Majumdar , Olof Karis , P. Nordblad , Biplab Sanyal , Olle Eriksson , D. D. Sarma

The $1/4$-filled organic compound, $\delta$-(EDT-TTF-CONMe$_{2}$)$_{2}$AsF$_6$ is a frustrated two-dimensional triangular magnetic system as shown by high-frequency (111.2 and 222.4 GHz) electron spin resonance (ESR) and structural data in…

Strongly Correlated Electrons · Physics 2016-11-22 B. Náfrádi , A. Antal , T. Fehér , L. F. Kiss , C. Mézière , P. Batail , L. Forró , A. Jánossy

The compound Ba3HoRu2O9 magnetically orders at 50 K (TN1) followed by another complex magnetic ordering at 10.2 K (TN2). The 2nd magnetic phase transition was characterized by the co-existence of two competing magnetic ground states…

Strongly Correlated Electrons · Physics 2024-06-18 E. Kushwaha , G. Roy , M. Kumar , A. M. dos Santos , S. Ghosh , D. T. Adroja , V. Caignaert , O. Perez , A. Pautrat , T. Basu

Double perovskites Sr2FeOsO6 and Ca2FeOsO6 show puzzling magnetic properties, the former a low-temperature antiferromagnet while the later a high-temperature insulating ferrimagnet. Here, in order to understand the underlying mechanism, we…

Materials Science · Physics 2015-08-24 Yusheng Hou , Hongjun Xiang , Xingao Gong

We successfully synthesized and characterized the triangular lattice anitferromagnet Ba$_8$MnNb$_6$O$_{24}$, which comprises equilateral spin-5/2 Mn$^{2+}$ triangular layers separated by six non-magnetic Nb$^{5+}$ layers. The detailed…

Materials Science · Physics 2019-06-03 R. Rawl , L. Ge , Z. Lu , Z. Evenson , C. R. Dela Cruz , Q. Huang , M. Lee , E. S. Choi , M. Mourigal , H. D. Zhou , J. Ma
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