Related papers: Engineering High-Order Harmonic Generation through…
High-order harmonic generation (HHG) is investigated for H$_2^+$ and its isotopomers under seven- and ten-cycle trapezoidal laser pulses at 800 nm wavelength and $I$=4$\times 10^{14}$ W$/$cm$^2$ intensity. We solved numerically…
We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…
High Harmonic Generation (HHG) creates coherent high frequency radiation via the process of strong field ionization followed by recombination. Recently, a complementary approach based on Frustrated Tunnel Ionization (FTI) was demonstrated…
In this work we study the impact of chromatic focusing of few-cycle laser pulses on high-order harmonic generation (HHG) through analysis of the emitted extreme ultraviolet (XUV) radiation. Chromatic focusing is usually avoided in the…
High-harmonic generation (HHG) is a nonlinear process in which a strong driving field interacts with a material, resulting in the frequency up-conversion of the driver into its high-order harmonics. This process is highly sensitive to the…
Vigorous efforts to harness the topological properties of light have enabled a multitude of novel applications. Translating the applications of structured light to higher spatial and temporal resolutions mandates their controlled…
The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the…
Recent breakthroughs in high repetition-rate extreme ultraviolet (XUV) light sources and photoelectron analyzers have led to dramatic advances in the performance of time-resolved photoemission experiments. In this perspective article, we…
Fourth-generation storage-ring light sources have achieved transverse emittances approaching the diffraction limit at x-ray wavelengths, while their longitudinal coherence remains limited. Existing laser-modulation schemes can induce strong…
An important goal in molecular physics and chemistry today is to obtain structure-dependent information about molecular function to obtain a deeper understanding into chemical reactions. However, until now, asymmetric tops, which comprise…
Recently, the size-dependence of high-order harmonic generation (HHG) in quantum dots has been investigated experimentally. In particular, for longer driving wavelengths and QDs smaller than 3\,nm, HHG was strongly suppressed, however,…
One key parameter in the high-order harmonic generation (HHG) phenomenon is the exact frequency of the generated harmonic field. Its deviation from perfect harmonics of the laser frequency can be explained considering (i) the single-atom…
Attosecond pulses, produced through high-order harmonic generation in gases, have been successfully used for observing ultrafast, sub-femtosecond electron dynamics in atoms, molecules and solid state systems. Today's typical attosecond…
We employ the two-band density-matrix equations and time-dependent density functional theory to calculate high-order harmonic generation (HOHG) in graphene under a femtosecond laser irradiation. Our investigation uncovers a striking…
We report on experimental investigation of nonperturbative high harmonic generation (HHG) in monolayer MoS2 in the ultraviolet spectral region driven by mid-infrared light. We study how the HHG is influenced by pre-excitation of the…
Preparation of nonclassical light with special quantum properties is essential for quantum technologies. High-harmonic generation (HHG) is a process which not only enables the creation of attosecond pulses but also has the potential to…
We theoretically investigate high-order harmonic generation (HHG) and its ellipticity in gapped graphene, driven by a femtosecond short-pulse laser at various orientation angles, employing the two-band density-matrix equations within the…
We report on the comparative experimental investigation on third and fifth harmonic generation (THG and FHG) in atomic and molecular gases driven by mid-infrared ultrafast laser pulses at a wavelength of ~1500 nm. We observe that the…
The duration of isolated attosecond pulses created via high-order harmonic generation is determined by the number of optical cycles in the driving laser. Achieving shorter attosecond soft X-ray pulses requires minimizing the number of…
High-quality ultrafast light sources are critical for developing advanced time- and angle-resolved photoemission spectroscopy (TrARPES). While the application of high harmonic generation (HHG) light sources in TrARPES has increased…