Related papers: Chromium-doped uranium dioxide fuels: A review
The neutronic properties of UO2-BeO fuel with various claddings are investigated through the Monte Carlo method and the Linear Reactivity Model. A second order polynomial function is suggested to describe the relationship between the…
The defect chemistry and thermal oxidation of lanthanide (Ln) incorporated-UO2 are critical for understanding and predicting their behavior as enhanced fuels, mixed oxide (MOX) fuels, spent nuclear fuels (SNF), and particles for safeguard…
Undoped and Cr doped \b{eta}-Ga2O3 (100) single crystals are grown by optical floating zone method. The full width at half maximum of rocking curve is found to be 106 arcsec for undoped Ga2O3 crystals whereas the 100 and 200 ppm of Cr doped…
The role of Cr incorporation into the ZnO were probed through investigations into the structural, optical and magnetic properties. Zn1-xCrxO with x = 0, 0.01, 0.03 and 0.05, nanoparticles were prepared by solution combustion method. Powder…
Uranium dioxide has been widely used as a nuclear fuel in commercial light water reactors due to its high uranium density and chemical stability. However, its relatively low thermal conductivity is not optimal from the viewpoints of fuel…
Commercial nuclear power plants extensively rely on fission energy from uranium dioxide (UO2) fuel pellets that provide thermal energy; consequently, generating carbon-free power in current generation reactors. UO2 fuel incurs damage and…
Cr-doped ZnO films were fabricated by a new but feasible method, that is, annealing Cr-Zn layers deposited via DC magnetron sputtering in air. Microstructures of the films were investigated using X-ray diffraction, scanning electron…
In this work, we have developed a model for irradiation-assisted grain growth in nanocrystalline UO$_2$ using the MARMOT code. We include the impact of irradiation on UO$_2$ grain growth by coupling a phase field grain growth model with a…
We have made chromium-doped, silica-based preforms and optical fibres by Modified Chemical Vapour Deposition and have studied the influence of the chemical composition of the doped region on the Cr-oxidation states and the spectroscopic…
A R&D program is developed at the ALTO facility to provide new beams of exotic neutron-rich nuclei, as intense as possible. In the framework of European projects, it has been shown that the use of refractory targets with nanometric…
The technological settings of a modified sol-gel method for preparation of highly fine homogeneous powder Ca2CuO3 doped with uranium 238 (x=0-0.05) is presented. The analysis of structure, purity of phases and the justification for the role…
Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the real-world are often driven by the microstructure, which for many polycrystalline…
The dry conversion process for making UO2 nuclear fuel pellets consists of two steps: hydrolysis of UF6 to UO2F2, followed by reducing pyrohydrolysis to UO2 in a rotary kiln. The physical characteristics (morphology, particle size…
Unraveling the adsorption mechanism and thermodynamics of O$_2$ and H$_2$O on uranium dioxide surfaces is critical for the nuclear fuel storage and uranium corrosion. Based on the first-principles DFT+U-D3 calculations, we carefully test…
Uranium mononitride, UN, is considered a potential accident tolerant fuel due to its high uranium density, high thermal conductivity, and high melting point. Compared with the relatively inert UO2, UN has a high reactivity in water,…
Understanding and predicting the dominant diffusion processes in Cr2O3 is essential to its optimization for anti-corrosion coatings, spintronics, and other applications. Despite significant theoretical effort in modeling defect mediated…
UO2/BeO interfacial thermal resistance (ITR) is calculated by diffuse mismatch model (DMM) and the effects of ITR on UO2-BeO thermal conductivity are investigated. ITR predicted by DMM is on the order of 10-9 m2K/W. Using this ITR, UO2-BeO…
Direct fired supercritical CO2 (sCO2) power cycles allow for the combustion of gaseous fuels under oxyfuel conditions with inherent carbon capture. As the CO2 is captured intrinsically, the efficiency penalty of capture on the overall plant…
In this report we present a systematic study on the preparation of Co:ZnO ceramics via standard solid-state route from different Co precursors (Co3O4, CoO and metallic Co) and atmospheres (O2 and Ar). Particular emphasis was done on the…
The archetypical strongly correlated Mott-phenomena compound V2O3 is known to show a paramagnetic metal-insulator transition driven by doping with chromium atoms and/or (negative) pressure. Via charge self-consistent density-functional…