English

Development of a Model for Irradiation-Assisted Grain Growth for Nanocrystalline UO2

Materials Science 2025-12-15 v1

Abstract

In this work, we have developed a model for irradiation-assisted grain growth in nanocrystalline UO2_2 using the MARMOT code. We include the impact of irradiation on UO2_2 grain growth by coupling a phase field grain growth model with a heat conduction simulation that features a random heat source representing thermal spikes. Our model parameters have been calibrated against experimental measurements at 300 K. The calibrated model predicts grain growth in an irradiated UO2_2 thin film that compares well with experimental data at 50 K. These results suggest that thermal spikes are the major cause of the irradiation-assisted grain growth observed in the UO2_2 experiments. They also indicate that irradiation-assisted grain growth is only significant with average grain sizes less than 35 nm, and thus can be neglected when considering fuel performance of typical UO2_2 fuel pellets.

Keywords

Cite

@article{arxiv.2512.11289,
  title  = {Development of a Model for Irradiation-Assisted Grain Growth for Nanocrystalline UO2},
  author = {Md Ali Muntaha and Larry Aagesen and Michael Tonks},
  journal= {arXiv preprint arXiv:2512.11289},
  year   = {2025}
}

Comments

29 pages, 11 figures, Submitted to Journal of Nuclear Materials (Currently Under Review)