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Related papers: Precision measurement of the $^{176}\mathrm{Lu}^+$…

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We report on an absolute frequency measurement of the ${\rm Lu}^{+}\,(^{3}\rm D_1)$ standard frequency which is defined as the hyperfine-average of $^{1}\rm S_0$ to $^{3}\rm D_1$ optical clock transitions in $^{176}{\rm Lu}^{+}$. The…

Atomic Physics · Physics 2026-01-12 Zhao Zhang , Qi Zhao , Qin Qichen , N. Jayjong , M. D. K. Lee , K. J. Arnold , M. D. Barrett

High precision spectroscopy of the $^1S_0$-to-${^1}D_2$ clock transition of $^{176}$Lu is reported. Measurements are performed with Hertz level precision with the accuracy of the hyperfine-averaged frequency limited by the calibration of an…

Atomic Physics · Physics 2019-03-06 R. Kaewuam , T. R. Tan , K. J. Arnold , M. D. Barrett

Precision measurements of the Lu$^+$ $^3D_1$ and $^3D_2$ quadrupole moments have been carried out giving $\Theta(^3D_1)=0.63862(74)\,e a_0^2$ and $\Theta(^3D_2)=0.8602(14)\,e a_0^2$, respectively. The measurements utilize the differential…

Atomic Physics · Physics 2020-11-04 R. Kaewuam , T. R. Tan , Zhiqiang Zhang , K. J. Arnold , M. S. Safronova , M. D. Barrett

Accurate measurements of different transition frequencies between atomic levels of the electronic and hyperfine structure over time are used to investigate temporal variations of the fine structure constant $\alpha$ and the…

Atomic Physics · Physics 2014-12-01 N. Huntemann , B. Lipphardt , Chr. Tamm , V. Gerginov , S. Weyers , E. Peik

We perform high resolution spectroscopy on $^{176}$Lu$^+$ including the $^1S_0\leftrightarrow{^3}D_1$ and $^1S_0\leftrightarrow{^3}D_2$ clock transitions. Hyperfine structures and optical frequencies relative to the $^1S_0$ ground state of…

Atomic Physics · Physics 2019-01-09 R. Kaewuam , A. Roy , T. R. Tan , K. J. Arnold , M. D. Barrett

We have performed Fourier transform microwave spectroscopy of benzonitrile, without and with applied electric fields. From the field-free hyperfine-resolved microwave transitions we simultaneously derive accurate values for the rotational…

Chemical Physics · Physics 2007-12-21 Kirstin Wohlfart , Melanie Schnell , Jens-Uwe Grabow , Jochen Küpper

We report the first laser spectroscopy of the $^1$S$_0$ to $^3$D$_1$ clock transition in $^{175}$Lu$^+$. Clock operation is demonstrated on three pairs of Zeeman transitions, one pair from each hyperfine manifold of the $^3$D$_1$ term. We…

Atomic Physics · Physics 2017-03-07 Kyle J. Arnold , R. Kaewuam , A. Roy , E. Paez , S. Wang , M. D. Barrett

We report measurements of the Lande g-factors for the 5d6s $^3$D$_2$ hyperfine levels of $^{176}$Lu$^+$ to a fractional inaccuracy of $5\times 10^{-7}$. Combining these measurements with theoretical calculations allows us to estimate…

Atomic Physics · Physics 2025-07-23 Qi Zhao , M. D. K. Lee , Qin Qichen , Zhao Zhang , N. Jayjong , K. J. Arnold , M. D. Barrett

We experimentally investigate an optical frequency standard based on the 467 nm (642 THz) electric-octupole reference transition 2S1/2(F=0) -> F7/2(F=3) in a single trapped 171Yb+ ion. The extraordinary features of this transition result…

Atomic Physics · Physics 2012-03-02 N. Huntemann , M. Okhapkin , B. Lipphardt , S. Weyers , Chr. Tamm , E. Peik

The hyperfine structure of the S1/2-D5/2 quadrupole transition at 729 nm in 43Ca+ has been investigated by laser spectroscopy using a single trapped 43Ca+ ion. We determine the hyperfine structure constants of the metastable level as…

Atomic Physics · Physics 2015-06-26 J. Benhelm , G. Kirchmair , U. Rapol , T. Koerber , C. F. Roos , R. Blatt

Over a two-year duration, we have compared the frequency of the 199Hg+ 5d106s 2S 1/2 (F=0)<-> 5d9 6s2 2D 5/2 (F=2) electric-quadrupole transition at 282 nm with the frequency of the ground-state hyperfine splitting in neutral 133Cs. These…

Demands from several areas of science and technology have lead to a worldwide search for accurate optical clocks with an uncertainty of 1 part in $10^{18}$, which is $10^{3}$ times more accurate than the present day cesium atomic clocks…

Atomic Physics · Physics 2017-08-23 Chiranjib Sur , K. V. P. Latha , Rajat K. Chaudhuri , B. P. Das , D. Mukherjee

We demonstrate precision measurement and control of inhomogeneous broadening in a multi-ion clock consisting of three $^{176}$Lu$^+$ ions. Microwave spectroscopy between hyperfine states in the $^3D_1$ level is used to characterise…

We measure the differential polarizability of the $^{176}$Lu$^+$ $^1S_0$ -to- ${^3}D_1$ clock transition at multiple wavelengths. This experimentally characterizes the differential dynamic polarizability for frequencies up to 372 THz and…

Atomic Physics · Physics 2019-01-23 K. J. Arnold , R. Kaewuam , T. R. Tan , S. G. Porsev , M. S. Safronova , M. D. Barrett

We propose and experimentally demonstrate a scheme which effects hyperfine averaging during a Ramsey interrogation of a clock transition. The method eliminates the need to average over multiple optical transitions, reduces the sensitivity…

Quantum Physics · Physics 2020-03-04 R. Kaewuam , T. R. Tan , K. J. Arnold , S. R. Chanu , Zhiqiang Zhang , M. D. Barrett

The systematic shifts of the transition frequencies in the molecular hydrogen ions are of relevance to ultra-high-resolution radio-frequency, microwave and optical spectroscopy of these systems, performed in ion traps. We develop the…

Atomic Physics · Physics 2015-06-16 Dimitar Bakalov , Stephan Schiller

Searching for an accurate optical clock which can serve as a better time standard than the present day atomic clock is highly demanding from several areas of science and technology. Several attempts have been made to built more accurate…

Atomic Physics · Physics 2007-09-17 Chiranjib Sur , Rajat K Chaudhuri

We demonstrate a technique for frequency measurements of atomic transitions with a precision of 30 kHz. The frequency is measured using a ring-cavity resonator whose length is calibrated against a reference laser locked to the $D_2$ line of…

Atomic Physics · Physics 2009-11-10 Ayan Banerjee , Dipankar Das , Vasant Natarajan

We evaluate the feasibility of using magnetic-dipole (M1) transitions in highly-charged ions as a basis of an optical atomic clockwork of exceptional accuracy. We consider a range of possibilities, including M1 transitions between clock…

Atomic Physics · Physics 2015-06-23 V. I. Yudin , A. V. Taichenachev , A. Derevianko

We consider hyperfine-mediated effects for clock transitions in $^{176}$Lu$^+$. Mixing of fine structure levels due to the hyperfine interaction bring about modifications to Land\'e $g$-factors and the quadrupole moment for a given state.…

Atomic Physics · Physics 2020-09-08 Zhiqiang Zhang , K. J. Arnold , R. Kaewuam , M. S. Safronova , M. D. Barrett
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