Related papers: Excitons and Optical Response in Excitonic Insulat…
1T-TiSe2 has a semimetallic band structure at room temperature and undergoes phase transition to a triple-q charge density wave (CDW) state with a commensurate superlattice structure (2a * 2a * 2c) below Tc ~ 200 K at ambient pressure. This…
The exact microscopic origin, symmetry, and thermal melting mechanism of the charge density wave (CDW) phase in TiSe$_{2}$ remain a subject of intense debate, particularly regarding the presence of chiral structural order and a multi-step…
The impact of variable Ti self-doping on the 1T-TiSe2 charge density wave (CDW) is studied by scanning tunneling microscopy. Supported by density functional theory we show that agglomeration of intercalated-Ti atoms acts as preferential…
Exciton condensation indicating the spontaneous formation of electron-hole pair can cause the phase transition from a semimetal to an excitonic insulator by gap opening at the Fermi surface. While the idea of this excitonic insulator has…
The strongly correlated charge density wave (CDW) phase of 1T-TiSe$_2$ is being extensively researched to verify the claims of a unique chiral order due to the presence of three equivalent Fermi wavevectors involved in the CDW formation.…
Charge density wave (CDW) materials can undergo an ultrafast phase transition after an ultrashort laser pulse excitation, and the suggested underlying mechanisms have always been associated with two main features: excitonic…
To clarify the origin of a charge-density wave (CDW) phase in 1$T$-TiSe$_2$, we study the ground state property of a half-filled two-band Hubbard model in a triangular lattice including electron-phonon interaction. By using the variational…
Using time- and angle-resolved photoemission spectroscopy with selective near- and mid-infrared photon excitations, we investigate the femtosecond dynamics of the charge density wave (CDW) phase in 1$T$-TiSe$_2$, as well as the dynamics of…
Excitonic insulator is a coherent electronic phase that results from the formation of a macroscopic population of bound particle-hole pairs - excitons. With only a few candidate materials known, the collective excitonic behavior is…
We discuss, from a theoretical point of view, excitonic phases at the pressure induced semiconductor-semimetal transition in $\rm TmSe_{0.45}Te_{0.55}$,focusing, in particular, on the stability against an electron-hole liquid. The…
Research on charge-density-wave (CDW) ordered transition-metal dichalcogenides continues to unravel new states of quantum matter correlated to the intertwined lattice and electronic degrees of freedom. Here, we report an inelastic x-ray…
Excitonic insulators (EIs), arising in semiconductors when the electron-hole binding energy exceeds the band gap, are a solid-state prototype for bosonic phases of matter. Unlike the charged excitations that are frozen and unable to…
Femtosecond time-resolved mid-infrared reflectivity is used to investigate the electron and phonon dynamics occurring at the direct band gap of the excitonic insulator Ta$_2$NiSe$_5$ below the critical temperature of its structural phase…
In order to characterize in detail the charge density wave (CDW) transition of 1$T$-VSe$_2$, its electronic structure and lattice dynamics are comprehensively studied by means of x-ray diffraction, angle resolved photoemission (ARPES),…
Coulomb attraction between electrons and holes in a narrow-gap semiconductor or a semimetal is predicted to lead to an elusive phase of matter dubbed 'excitonic insulator'. However, direct observation of such electronic instability remains…
Superconductivity emerges in $1T$-TiSe$_2$ when its charge density wave (CDW) order is suppressed by Cu intercalation or pressure. Since the CDW state is thought to be an excitonic insulator, an interesting question is whether the…
We report on a transient optical reflectivity study of the charge density wave (CDW) in CuxTiSe2 single crystals. Our measurements reveal that the system undergoes a quantum phase transition at x=0.04 from a strong commensurate CDW (x<0.04)…
We report on the charge dynamics of Ta$_2$Pd$_3$Te$_5$ using temperature-dependent optical spectroscopy with polarized light. We observe a metal-insulator transition characterized by the collapse of Drude response and the emergence of sharp…
The fundamental idea of the excitonic insulator (EI) driven by electron-hole correlations in narrow-gap semiconductors or semimetals was originally proposed in the 1960s, and only theoretical studies had been advanced for a long time.…
We performed ultrasonic measurements on (Ta$_{0.952}$V$_{0.048}$)$_2$NiSe$_5$ to investigate the contribution of acoustic phonons at the zone center to structural and possible excitonic transitions. The transverse elastic constant $C_{55}$…