English

Precursor phase with full phonon softening above the charge-density-wave phase transition in $2H$-TaSe$_2$

Strongly Correlated Electrons 2023-11-13 v1 Superconductivity

Abstract

Research on charge-density-wave (CDW) ordered transition-metal dichalcogenides continues to unravel new states of quantum matter correlated to the intertwined lattice and electronic degrees of freedom. Here, we report an inelastic x-ray scattering investigation of the lattice dynamics of the canonical CDW compound 2H2H-TaSe2_2 complemented by angle-resolved photoemission spectroscopy. Our results rule out the central-peak scenario for the CDW transition in 2H2H-TaSe2_2 and provide evidence for a novel precursor phase above the CDW transition temperature TCDWT_{CDW}. The phase at temperatures between T(=128.7,K)T^{*}\,(= 128.7\,,\rm{K}) and TCDW(=121.3K)T_{CDW}\,(= 121.3\,\rm{K}) is characterized by a fully softened phonon mode and medium-range ordered (ξcorr=100A˚200A˚)\xi_{corr} = 100\,\rm{\mathring{A}}- 200\,\rm{\mathring{A}}) static CDW domains. Only TCDWT_{CDW} is detectable in our photoemission experiments. Thus, 2H2H-TaSe2_2 exhibits structural before electronic static order and emphasizes the important lattice contribution to CDW transitions.

Keywords

Cite

@article{arxiv.2207.11298,
  title  = {Precursor phase with full phonon softening above the charge-density-wave phase transition in $2H$-TaSe$_2$},
  author = {Xingchen Shen and Rolf Heid and Roland Hott and Björn Salzmann and Marli dos Reis Cantarino and Claude Monney and Ayman H. Said and Bridget Murphy and Kai Rossnagel and Stephan Rosenkranz and Frank Weber},
  journal= {arXiv preprint arXiv:2207.11298},
  year   = {2023}
}