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$1T$-TiSe$_2$ is believed to posses a soft electronic mode, i.e., plasmon or exciton, that might be responsible for the exciton condensation and charge-density-wave (CDW) transition. Here, we explore collective electronic excitations in…

Materials Science · Physics 2024-05-24 Zahra Torbatian , Dino Novko

Transition metal dichalcogenides (TMDs), whether in bulk or in monolayer form, exhibit a rich variety of charge-density-wave (CDW) phases and stronger periodic lattice distortions. While the actual role of nesting has been under debate, it…

Strongly Correlated Electrons · Physics 2018-12-12 Diego Pasquier , Oleg V. Yazyev

Recent experiments suggest that excitonic degrees of freedom play an important role in precipitating the charge density wave (CDW) transition in $1T$-$\mathrm{TiSe}_2$. Through systematic calculations of the electronic and phonon spectrum…

Mesoscale and Nanoscale Physics · Physics 2018-12-03 Chuan Chen , Bahadur Singh , Hsin Lin , Vitor M. Pereira

The Bose-Einstein condensation of excitons continues to garner immense attention as a prototypical example for observing emergent properties from many-body quantum effects. In particular, Titanium Diselenide (TiSe$_2$) is a promising…

Materials Science · Physics 2019-12-06 Chao Lian , Zulfikhar A. Ali , Bryan M. Wong

TiSe$_2$ has long been considered one of the best candidate materials to host the elusive excitonic insulator (EI) phase. However, a finite coupling to the lattice can generically be expected, while a lack of "smoking-gun" signatures for…

A new state of matter, an excitonic insulator (EI) state, was predicted to emerge from Bose-Einstein condensation of electron-hole pairs. Some candidate materials were suggested but it has been elusive to confirm its existence. Recent works…

Strongly Correlated Electrons · Physics 2021-05-12 Jin Mo Bok , Jungseek Hwang , Han-Yong Choi

The excitonic insulator (EI) is a Bose-Einstein condensation (BEC) of excitons bound by electron-hole interaction in a solid, which could support high-temperature BEC transition. The material realization of EI has been elusive, which is…

The complex phase diagram of 1T-TiSe2 consists of a charge density wave (CDW) below 200 K, and CDW fluctuations of still unknown origin at higher temperatures. Here, we use time-resolved extreme ultraviolet momentum microscopy and density…

TiSe$_2$ is thought to be an insulator with a bandgap of ~0.1eV. It has attracted a much interest because, among of a rich array of unique properties, many have thought TiSe$_2$ is a rare realisation of an excitonic insulator. Below 200 K,…

Materials Science · Physics 2025-06-10 Ross E. Larsen , Dimitar Pashov , Matthew D. Watson , Swagata Acharya , Mark van Schilfgaarde

A variety of experiments have been carried out to establish the origin of the chiral charge-density wave transition in 1T-TiSe$_2$, which in turn has led to contradictory conclusions on the origin of this transition. Some studies suggest…

Materials Science · Physics 2020-10-05 Darshana Wickramaratne , Richard Schaller , Gary Wiederrecht , Goran Karapetrov , I. I. Mazin

An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…

Strongly Correlated Electrons · Physics 2022-09-02 Selene Mor , Marc Herzog , Claude Monney , Julia Stähler

Renew interest in the charge density wave phase of TiSe$_2$ stems from the realization of its unique driving mechanism, the so called excitonic insulator phase. Existing claims are motivated by model calculations of the band structure. In…

Strongly Correlated Electrons · Physics 2024-08-13 Turgut Yilmaz , Anil Rajapitamahuni , Elio Vescovo

We present a new high-resolution angle-resolved photoemission study of 1\textit{T}-TiSe$_{2}$ in both, its room-temperature, normal phase and its low-temperature, charge-density wave phase. At low temperature the photoemission spectra are…

Strongly Correlated Electrons · Physics 2009-11-13 H. Cercellier , C. Monney , F. Clerc , C. Battaglia , L. Despont , M. G. Garnier , H. Beck , L. Patthey , H. Berger , P. Aebi

Charge density wave (CDW) is a collective quantum phenomenon with a charge modulation in solids1-2. Condensation of electron and hole pairs with finite momentum will lead to such an ordered state3-7. However, lattice symmetry breaking…

Recently there has been a renewed interest in the charge density wave transition of TiSe2, fuelled by the possibility that this transition may be driven by the formation of an excitonic insulator or even an excitonic condensate. We show…

Strongly Correlated Electrons · Physics 2010-04-29 Jasper van Wezel , Paul Nahai-Williamson , Siddarth S. Saxena

Excitonic insulators (EI) arise from the formation of bound electron-hole pairs (excitons) in semiconductors and provide a solid-state platform for quantum many-boson physics. Strong exciton-exciton repulsion is expected to stabilize…

Excitonic insulator (EI) was proposed in 60's as a distinct insulating state originating from pure electronic interaction, but its material realization has been elusive with extremely few material candidates and with only limited evidence…

Materials Science · Physics 2019-03-06 Jinwon Lee , Chang-Jong Kang , Man Jin Eom , Jun Sung Kim , Byung Il Min , Han Woong Yeom

An excitonic insulator$^{1,2}$ (EI) is a correlated many-body state of electron-hole pairs, potentially leading to high-temperature condensate and superfluidity$^{3-7}$. Despite ever-growing experiments suggesting possible EI states in…

Materials Science · Physics 2025-03-17 Fang Zhang , Jiawei Ruan , Gurjyot Sethi , Chen Hu , Steven G. Louie

We examine the competition between the charge-density wave (CDW) instability and the excitonic condensate (EC) in spatially separated layers of electrons and holes. The CDW and the EC order parameters (OPs), described by two different…

Strongly Correlated Electrons · Physics 2016-08-03 Ege Özgün , Tuğrul Hakioğlu

An excitonic insulator (EI) phase is a consequence of collective many-body effects where an optical band gap is formed by the condensation of electron-hole pairs or excitons. We report pressure-dependent optical pump optical probe…

Materials Science · Physics 2024-11-28 Vikas Arora , Victor S Muthu , Arijit Sinha , Luminita Harnagea , U V Waghmare , A K Sood
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