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We report a random singlet ground state in the $S=\frac{1}{2}$ Heisenberg pyrochlore antiferromagnet NaCdCu$_2$F$_7$. Cationic Na$^+$/Cd$^{2+}$ disorder on the pyrochlore $A$ site generates a broad distribution of…

Spin liquids occuring in 2D frustrated spin systems were initially assumed to appear at strongest frustration, but evidence grows that they more likely intervene at transitions between two different types of order. To identify if this is…

Strongly Correlated Electrons · Physics 2013-01-30 Philipp Hauke

Quantum spin liquids (QSLs) are topologically ordered exotic states of matter that host fractionalized excitations. Kitaev proposed a particular route towards a QSL via strongly bond-dependent interactions on the hexagonal lattice. A number…

Strongly Correlated Electrons · Physics 2022-12-06 Xinshu Zhang , Yuanyuan Xu , T. Halloran , Ruidan Zhong , R. J. Cava , C. Broholm , N. Drichko , N. P. Armitage

Quantum spin liquids (QSLs) are long-range entangled phases of frustrated magnets exhibiting fractionalized spin excitations. In two dimensions, there is limited analytical understanding of their excitation spectra beyond parton mean-field…

Strongly Correlated Electrons · Physics 2025-08-01 Josef Willsher , Johannes Knolle

We found a plateau in the magnitude of the isolated magnetic moments as a function of the anisotropy of the transfer integral (t'/t) in the gapless quantum spin liquid (QSL) phase of an S=1/2 triangular lattice molecular solid X[Pd(dmit)2]2…

Strongly Correlated Electrons · Physics 2024-03-20 K. Ueda , S. Fujiyama , R. Kato

Mott insulators with localized magnetic moments will exhibit a quantum spin liquid (QSL) state when the quantum fluctuations are strong enough to suppress the ordering of the spins. Such an entangled state will give rise to collective…

Strongly Correlated Electrons · Physics 2025-04-17 Haiyang Chen , Fo-Hong Wang , Qiang Gao , Xue-Jian Gao , Zhenhua Chen , Yaobo Huang , Kam Tuen Law , Xiao Yan Xu , Peng Chen

The two-dimensional (2D) spin-1/2 kagome Heisenberg antiferromagnet is believed to host quantum spin liquid (QSL) states with no magnetic order, but its ground state remains largely elusive. An important outstanding question concerns the…

Strongly Correlated Electrons · Physics 2024-05-30 S. Suetsugu , T. Asaba , Y. Kasahara , Y. Kohsaka , K. Totsuka , B. Li , Y. Zhao , Y. Li , M. Tokunaga , Y. Matsuda

We analyze the effect of quenched disorder on spin-1/2 quantum magnets in which magnetic frustration promotes the formation of local singlets. Our results include a theory for 2d valence-bond solids subject to weak bond randomness, as well…

Strongly Correlated Electrons · Physics 2018-08-01 Itamar Kimchi , Adam Nahum , T. Senthil

Quenched randomness strongly affects properties of magnetic materials. Two-dimensional (2D) random singlet (RS) states emerge in random $J$-$Q$ model by destroying valence bond solid order with spatial randomness. We examine the 2D RS state…

Strongly Correlated Electrons · Physics 2025-01-10 Chen Peng , Long Zhang

A quantum spin liquid (QSL) is a state of matter in which magnetic spins interact strongly, but quantum fluctuations inhibit long-range magnetic order even at zero temperature. A QSL has been predicted to have a host of exotic properties,…

Pursuing the exotic quantum spin liquid (QSL) state in the Kitaev material $\alpha$-RuCl$_3$ has intrigued great research interest recently. A fascinating question is on the possible existence of field-induced QSL phase in this compound.…

Strongly Correlated Electrons · Physics 2023-09-14 Xu-Guang Zhou , Han Li , Yasuhiro H. Matsuda , Akira Matsuo , Wei Li , Nobuyuki Kurita , Gang Su , Koichi Kindo , Hidekazu Tanaka

We present a quantu spin liquid state in a spin-1/2 honeycomb lattice with randomness in the exchange interaction. That is, we successfully introduce randomness into the organic radial-based complex and realize a random-singlet (RS) state.…

Strongly Correlated Electrons · Physics 2017-09-26 H. Yamaguchi , M. Okada , Y. Kono , S. Kittaka , T. Sakakibara , T. Okabe , Y. Iwasaki , Y. Hosokoshi

PbCuTe$_2$O$_6$ is considered as one of the rare candidate materials for a three-dimensional quantum spin liquid (QSL). This assessment was based on the results of various magnetic experiments, performed mainly on polycrystalline material.…

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

Strongly Correlated Electrons · Physics 2022-03-09 Jiaming Wang , Weishi Yuan , Philip M. Singer , Rebecca W. Smaha , Wei He , Jiajia Wen , Young S. Lee , Takashi Imai

The frustrated magnet has been regarded as a system that could be a promising host material for the quantum spin liquid (QSL). However, it is difficult to determine the spin configuration and the corresponding mechanism in this system,…

Materials Science · Physics 2018-05-14 H. Huang , H. Jang , B. Y. Kang , B. K. Cho , C-C Kao , Y. -J. Liu , J. -S. Lee

Continuous spin excitations are widely recognized as one of the hallmarks of novel spin states in quantum magnets, such as quantum spin liquids (QSLs). Here, we report the observation of such kind of excitations in K2Ni2(SO4)3, which…

Quantum spin liquids (QSLs) are long-range entangled states of quantum magnets which lie beyond the Landau paradigm of classifying phases of matter via broken symmetries. A physical route to arriving at QSLs is via frustration-induced…

Strongly Correlated Electrons · Physics 2017-09-20 Ciarán Hickey , Lukasz Cincio , Zlatko Papić , Arun Paramekanti

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

Strongly Correlated Electrons · Physics 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

Based on experimental data and our theoretical analysis, we provide a strategy for unambiguous establishing of gapless quantum spin liquid state (QSL) in herbertsmithite and other materials. To clarify the nature of QSL, we recommend…

Quantum spin liquid (QSL) represents a new class of condensed matter states characterized by the long-range many-body entanglement of topological orders. The most prominent feature of the elusive QSL state is the existence of fractionalized…