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The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

A quantum spin liquid (QSL) is an exotic state of matter in which electrons' spins are quantum entangled over long distances, but do not show symmetry-breaking magnetic order in the zero-temperature limit. The observation of QSL states is a…

Strongly Correlated Electrons · Physics 2017-03-08 J. A. M. Paddison , M. Daum , Z. L. Dun , G. Ehlers , Y. Liu , M. B. Stone , H. D. Zhou , M. Mourigal

Currently under active study in condensed matter physics, both theoretically and experimentally, are quantum spin liquid (QSL) states, in which no long-range magnetic ordering appears at low temperatures due to strong quantum fluctuations…

Strongly Correlated Electrons · Physics 2019-07-04 Ruidan Zhong , Shu Guo , Guangyong Xu , Zhijun Xu , Robert J. Cava

We investigate the ground-state and finite-temperature properties of the bond-random $s=1/2$ Heisenberg model on a honeycomb lattice with frustrated nearest- and next-nearest-neighbor antiferromagnetic interactions, $J_1$ and $J_2$, by the…

Strongly Correlated Electrons · Physics 2018-10-24 Kazuki Uematsu , Hikaru Kawamura

The Yb based triangular lattice delafossites $A$Yb$X_2$ ($A$ = alkali metal, $X$ = O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe$_2$ with a perfect…

Strongly Correlated Electrons · Physics 2025-09-23 Barkha Khattar , Anzar Ali , Masahiko Isobe , Yogesh Singh

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

Organic solids host various electronic phases. Especially, a milestone compound of organic solid, $\beta'$-$X$[Pd(dmit)$_2$]$_2$ with $X$=EtMe$_3$Sb shows quantum spin-liquid (QSL) properties suggesting a novel state of matter. However,…

Strongly Correlated Electrons · Physics 2022-04-29 Kota Ido , Kazuyoshi Yoshimi , Takahiro Misawa , Masatoshi Imada

The quantum spin liquid (QSL) is a state manifesting extraordinary many-body entanglement, and the material NaYbSe$_2$ is thought to be one of the most promising candidates for its realization. Through low-temperature heat capacity and…

Strongly Correlated Electrons · Physics 2025-02-11 Luke Pritchard Cairns , Yuanqi Lyu , Chunxiao Liu , Josue Rodriguez , Kenneth Ng , John Singleton , James G. Analytis

We investigate the ground-state and the finite-temperature properties of the bond-random $s=1/2$ Heisenberg model on a square lattice with frustrating nearest- and next-nearest-neighbor antiferromagnetic interactions, $J_1$ and $J_2$, by…

Strongly Correlated Electrons · Physics 2018-10-26 Kazuki Uematsu , Hikaru Kawamura

Quantum spin liquid (QSL) is a novel state of matter with exotic excitations and was theoretically predicted to be realized most possibly in an S=1/2 kagome antiferromagnet. Experimentally searching for the candidate materials is a big…

Strongly Correlated Electrons · Physics 2014-09-15 Yuesheng Li , Bingying Pan , Shiyan Li , Wei Tong , Langsheng Ling , Zhaorong Yang , Junfeng Wang , Zhongjun Chen , Zhonghua Wu , Qingming Zhang

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

Induced by quenched disorder, random-singlet states occur in a variety of low-dimensional spin-1/2 antiferromagnets, some of them candidates for quantum spin liquids. Here we report measurements of the specific heat, magnetization, and…

The quantum spin liquid (QSL) state is an exotic state of matter featuring a high degree of entanglement and lack of long-range magnetic order in the zero-temperature limit. The triangular antiferromagnet YbMgGaO4 is a candidate QSL host,…

The nature of the randomness-induced quantum spin liquid state, the random-singlet state, is investigated in two dimensions (2D) by means of the exact-diagonalization and the Hams-de Raedt methods for several frustrated lattices, e.g., the…

Strongly Correlated Electrons · Physics 2020-01-08 Hikaru Kawamura , Kazuki Uematsu

Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to…

Triangular lattice of rare-earth ions with interacting effective spin-$1/2$ local moments is an ideal platform to explore the physics of quantum spin liquids (QSLs) in the presence of strong spin-orbit coupling, crystal electric fields, and…

Recent studies have revealed that the randomness-induced quantum spin liquid (QSL)-like state is stabilized in certain frustrated quantum magnets in two and three dimensions. In order to clarify the nature of this gapless QSL-like state, we…

Strongly Correlated Electrons · Physics 2021-11-24 Kazuki Uematsu , Toshiya Hikihara , Hikaru Kawamura

One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…

Strongly Correlated Electrons · Physics 2023-01-10 Chengpeng Tu , Dongzhe Dai , Xu Zhang , Chengcheng Zhao , Xiaobo Jin , Bin Gao , Tong Chen , Pengcheng Dai , Shiyan Li

The emergence of a quantum spin liquid (QSL), a state of matter that can result when electron spins are highly correlated but do not become ordered, has been the subject of a considerable body of research in condensed matter physics. Spin…

The three-dimensional $S = {\frac{1}{2}}$ system Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$ consists of two inequivalent Cu$^{2+}$ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility $\chi(T)$, specific heat $C_p(T)$,…