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Gas-phase complex organic molecules have been detected toward a range of high- and low-mass star-forming regions at abundances which cannot be explained by any known gas-phase chemistry. Recent laboratory experiments show that UV…

Astrophysics of Galaxies · Physics 2015-05-18 Karin I. Oberg , Sandrine Bottinelli , Jes K. Jorgensen , Ewine F. van Dishoeck

Interstellar methanol is considered to be a parent species of larger, more complex organic molecules. A physicochemical simulation of infalling parcels of matter is performed for a low-mass star-forming system to trace the chemical…

Solar and Stellar Astrophysics · Physics 2014-09-09 Maria N. Drozdovskaya , Catherine Walsh , Ruud Visser , Daniel Harsono , Ewine F. van Dishoeck

Our automated reaction discovery program, AutoMeKin, has been utilized to investigate the formation of glycolonitrile (HOCH$_{2}$CN) in the gas phase under the low temperatures of the interstellar medium (ISM). The feasibility of a proposed…

The collisional pumping of CH3OH and OH masers in non-dissociative C-type shock waves is studied. The chemical processes responsible for the evolution of molecule abundances in the shock wave are considered in detail. The large velocity…

Astrophysics of Galaxies · Physics 2021-12-15 A. V. Nesterenok

The detection of complex organic molecules (COMs) toward dense, collapsing prestellar cores has sparked interest in the fields of astrochemistry and astrobiology, yet the mechanisms for COM formation are still debated. It was originally…

Astrophysics of Galaxies · Physics 2023-04-05 Samantha Scibelli , Yancy Shirley

We report the first detection of triply-deuterated methanol, with 12 observed transitions, towards the low-mass protostar IRAS 16293-2422, as well as multifrequency observations of 13CH3OH, used to derive the column density of the main…

Astrophysics · Physics 2007-05-23 B. Parise , A. Castets , E. Herbst , E. Caux , C. Ceccarelli , I. Mukhopadhyay , A. G. G. M. Tielens

Solid state astrochemical reaction pathways have the potential to link the formation of small nitrogen-bearing species, like NH3 and HNCO, and prebiotic molecules, specifically amino acids. To date, the chemical origin of such small…

Astrophysics of Galaxies · Physics 2017-05-26 Gleb Fedoseev , Sergio Ioppolo , Dongfeng Zhao , Thanja Lamberts , Harold Linnartz

Acetic acid (CH3COOH) was detected in the gas toward interstellar clouds, hot cores, protostars and comets. Its formation in ice mantles was proposed and acetic acid awaits detection in the infrared spectra of the ice as most other COMs…

Instrumentation and Methods for Astrophysics · Physics 2023-12-05 C. del Burgo Olivares , H. Carrascosa , B. Escribano , G. M. Muñoz Caro , R. Martín-Doménech

Gas-phase chemistry at extreme conditions (low densities and temperatures) is difficult, so the presence of interstellar grains is especially important for the synthesis of molecules that cannot form in the gas phase. Interstellar grains…

Astrophysics of Galaxies · Physics 2023-12-12 Gerard Pareras , Victoria Cabedo , Martin McCoustra , Albert Rimola

The chemical network governing interstellar sulfur has been the topic of unrelenting discussion for the past decades due to the conspicuous discrepancy between its expected and observed abundances in different interstellar environments.…

Astrophysics of Galaxies · Physics 2024-07-16 Julia C. Santos , Joan Enrique-Romero , Thanja Lamberts , Harold Linnartz , Ko-Ju Chuang

Carbon ($^3$P) atom is a reactive species that, according to laboratory experiments and theoretical calculations, condensates with interstellar ice components. This fact is of uttermost importance for the chemistry in the interstellar…

Astrophysics of Galaxies · Physics 2023-07-19 Stefano Ferrero , Cecilia Ceccarelli , Piero Ugliengo , Mariona Sodupe , Albert Rimola

The formation of CH+ in the interstellar medium has long been an outstanding problem in chemical models. In order to probe the physical conditions of the ISM in which CH+ forms, we propose the use of CH3+ observations. The pathway to…

Astrophysics of Galaxies · Physics 2015-05-18 Nick Indriolo , Takeshi Oka , T. R. Geballe , Benjamin J. McCall

Methanol is a key species in astrochemistry since it is the most abundant organic molecule in the ISM and is thought to be the mother molecule of many complex organic species. Estimating the deuteration of methanol around young protostars…

The deuterium fractionation of gas-phase molecules in hot cores is believed to reflect the composition of interstellar ices. The deuteration of methanol is a major puzzle, however, because the isotopologue ratio [CH2DOH]/[CH3OD], which is…

Solar and Stellar Astrophysics · Physics 2015-12-02 A. Faure , M. Faure , P. Theulé , E. Quirico , B. Schmitt

The first experimental study of the low-temperature kinetics of the gas-phase reaction of NH2 with formaldehyde (CH2O) has been performed. This reaction has previously been suggested as a source of formamide (NH2CHO) in interstellar…

Astrophysics of Galaxies · Physics 2022-10-05 Kevin M. Douglas , Daniel Lucas , Catherine Walsh , Niclas A. West , Mark A. Blitz , Dwayne E. Heard

Interstellar complex organic molecules (iCOMs) are assumed to be mainly formed on dust-grain surfaces. However, neutral gas-phase reactions in the interstellar medium (ISM) can play an important role. In this paper, by investigating the…

Astrophysics of Galaxies · Physics 2020-09-09 F. Tonolo , J. Lupi , C. Puzzarini , V. Barone

A prevailing theory for the interstellar production of complex organic molecules (COMs) involves formation on warm dust-grain surfaces, via the diffusion and reaction of radicals produced through grain-surface photodissociation of stable…

Astrophysics of Galaxies · Physics 2020-08-19 Mihwa Jin , Robin T. Garrod

A number of recent experimental studies have shown that solid-state complex organic molecules (COMs) can form under conditions that are relevant to the CO freeze-out stage in dense clouds. In this work, we show that alcohols can be formed…

Astrophysics of Galaxies · Physics 2019-05-16 D. Qasim , G. Fedoseev , T. Lamberts , K. -J. Chuang , J. He , S. Ioppolo , J. Kästner , H. Linnartz

We calculated reaction rate constants including atom tunneling for the hydrogen abstraction reaction CH3OH+H -> CH2OH+H2 with the instanton method. The potential energy was fitted by a neural network, that was trained to…

Chemical Physics · Physics 2020-09-10 April. M. Cooper , Johannes Kästner

Methanol ice is embedded in interstellar ice mantles present in dense molecular clouds. We aim to measure the sputtering efficiencies starting from different ice mantles of varying compositions experimentally, in order to evaluate their…

Astrophysics of Galaxies · Physics 2020-02-19 E. Dartois , M. Chabot , A. Bacmann , P. Boduch , A. Domaracka , H. Rothard