English
Related papers

Related papers: Parquet theory for molecular systems: Formalism an…

200 papers

The $GW$ approximation to many-body perturbation theory is a reliable tool for describing charged electronic excitations, and it has been successfully applied to a wide range of extended systems for several decades using a plane-wave basis.…

Materials Science · Physics 2019-10-23 Young-Moo Byun , Serdar Öğüt

Correlated quantum many-particle systems out of equilibrium are of high interest in many fields, including correlated solids, ultracold atoms or dense plasmas. Accurate theoretical description of these systems is challenging both,…

Strongly Correlated Electrons · Physics 2026-04-02 Erik Schroedter , Michael Bonitz

Quantum dynamics simulations of reactive molecular processes are commonly performed in a low-dimensional space spanned by highly optimized reactive coordinates. Usually, these sets of reactive coordinates consist of non-linear coordinates.…

Chemical Physics · Physics 2018-01-01 Julius P. P. Zauleck , Sebastian Thallmair , Regina de Vivie-Riedle

We present a theoretical framework and implementation details for self-energy embedding theory (SEET) with the GW approximation for the treatment of weakly correlated degrees of freedom and configuration interactions solver for handing the…

Strongly Correlated Electrons · Physics 2017-10-11 Tran Nguyen Lan , Avijit Shee , Jia Li , Emanuel Gull , Dominika Zgid

The vertex function ($\Gamma$) within the Green's function formalism encapsulates information about all higher-order electron-electron interaction beyond those mediated by density fluctuations. Herein, we present an efficient approach that…

Chemical Physics · Physics 2023-03-28 Guorong Weng , Rushil Mallarapu , Vojtech Vlcek

In this paper, we propose a generic and systematic approach for study of the electronic structure for atoms or molecules. In particular, we address the issue of single particle states, or orbitals, which should be one of the most important…

Chemical Physics · Physics 2007-05-23 Liqiang Wei

The electronic band structure of SrTiO$_3$ is investigated in the all-electron QS$GW$ approximation. Unlike previous pseudopotential based QS$GW$ or single-shot $G_0W_0$ calculations, the gap is found to be significantly overestimated…

Materials Science · Physics 2018-01-31 Churna Bhandari , Mark van Schilfgaarde , Takao Kotani , Walter R. L. Lambrecht

This paper introduces a numerical scheme for time harmonic Maxwell's equations by using weak Galerkin (WG) finite element methods. The WG finite element method is based on two operators: discrete weak curl and discrete weak gradient, with…

Numerical Analysis · Mathematics 2013-12-10 Lin Mu , Junping Wang , Xiu Ye , Shangyou Zhang

Fully self-consistent GW (sc-GW) methods are now available to evaluate quasiparticle and spectral properties of various molecular and bulk systems. However, such techniques based on the full matrix of G and W are computationally demanding.…

Materials Science · Physics 2020-11-17 Yashpal Singh , Lin-Wang Wang

Calculations of excited states in Green's function formalism often invoke the diagonal approximation, in which the quasiparticle states are taken from a mean-field calculation. Here, we extend the stochastic approaches applied in the…

Computational Physics · Physics 2023-09-28 Annabelle Canestraight , Xiaohe Lei , Khaled Ibrahim , Vojtech Vlcek

The transition-matrix ($T$-matrix) approach provides a general formalism to study scattering problems in various areas of physics, including acoustics (scalar fields) and electromagnetics (vector fields), and is related to the theory of the…

Optics · Physics 2016-02-08 Eric C. Le Ru , Walter R. C. Somerville , Baptiste Auguié

New stochastic approaches for the computation of electronic excitations are developed within the many-body perturbation theory. Three approximations to the electronic self-energy are considered: $G_0W_0$, $G_0W_0^tc$, and…

Chemical Physics · Physics 2019-08-27 Vojtech Vlcek

For materials which are incorrectly predicted by density functional theory to be metallic, an iterative procedure must be adopted in order to perform GW calculations. In this paper we test two iterative schemes based on the quasi-particle…

Materials Science · Physics 2007-05-23 V. A. Popa , G. Brocks , P. J. Kelly

We present a detailed discussion of self-energy embedding theory (SEET) which is a quantum embedding scheme allowing us to describe a chosen subsystem very accurately while keeping the description of the environment at a lower cost. We…

Chemical Physics · Physics 2016-11-15 Tran Nguyen Lan , Alexei A. Kananenka , Dominika Zgid

Understanding collective phenomena calls for tractable descriptions of correlations in assemblies of strongly interacting constituents. Capturing the essence of their self-consistency is central. The parquet theory admits a maximum level of…

Strongly Correlated Electrons · Physics 2022-11-23 Frederick Green , Thomas L. Ainsworth

We introduce a quasiclassical Green function approach describing the unitary yet irreversible dynamics of quantum systems effectively acting as their own environment. Combining a variety of concepts of quantum many-body theory, notably the…

Mesoscale and Nanoscale Physics · Physics 2025-09-09 Alexander Altland , Kun Woo Kim , Tobias Micklitz

The cumulant expansion of the Green's function is a computationally efficient beyond-$GW$ approach renowned for its significant enhancement of satellite features in materials. In contrast to the ubiquitous $GW$ approximation of many-body…

Chemical Physics · Physics 2024-02-27 Pierre-François Loos , Antoine Marie , Abdallah Ammar

The coherent potential approximation (CPA) is extended to describe satisfactorily the motion of particles in a random potential which is spatially correlated and smoothly varying. In contrast to existing cluster-CPA methods, the present…

Disordered Systems and Neural Networks · Physics 2009-10-20 Roland Zimmermann , Christoph Schindler

A general semiclassical approach to quantum systems with system-bath interactions is developed. We study system decoherence in detail using a coherent state semiclassical wavepacket method which avoids singularity issues arising in the…

Quantum Physics · Physics 2009-11-07 Gregory A. Fiete , Eric J. Heller

Within the framework of the full potential projector-augmented wave methodology, we present a promising low-scaling $GW$ implementation. It allows for quasiparticle calculations with a scaling that is cubic in the system size and linear in…

Materials Science · Physics 2016-10-12 Peitao Liu , Merzuk Kaltak , Jiří Klimeš , Georg Kresse