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Neutron-rich nuclei in the vicinity of the $N=40$ island of inversion are characterized by shell evolution and exhibit deformed ground states. In several nuclei isomeric states have been observed and attributed to excitations to the…

We present a new method for determining the intrinsic natural linewidth or lifetime of exceptionally long-lived optical excited states. Such transitions are key to the performance of state-of-the-art atomic clocks, have potential…

Atomic Physics · Physics 2021-06-02 Juan A. Muniz , Dylan J. Young , Julia R. K. Cline , James K. Thompson

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

Nuclear Experiment · Physics 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

The lifetime of the isomeric state in fully stripped 94Ru44+ ions has been measured using isochronous mass spectrometry (IMS) at the experimental Cooler Storage Ring (CSRe) of the Heavy Ion Research Facility in Lanzhou (HIRFL). Previously,…

Instrumentation and Detectors · Physics 2025-09-22 Qi Zeng , Bushi Huang , Tingwei Peng , Hongfu Li , Xing XuYuanming Xing , Huaiqiang Zhang , Jiankun Zhao , Xu Zhou

Today's most precise time and frequency measurements are performed with optical atomic clocks. However, it has been proposed that they could potentially be outperformed by a nuclear clock, which employs a nuclear transition instead of the…

LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that…

We performed at ISOLDE the spectroscopy of the decay of the 8- isomer in 136Cs by and conversion-electron detection. For the first time the excitation energy of the isomer and the multipolarity of its decay have been measured. The half-life…

We present absolute frequency measurements of the ${}^{1}\text{P}_1 \leftarrow {}^{1}\text{S}_0$ ($229$nm) and ${}^{3}\text{P}_1 \leftarrow {}^{1}\text{S}_0$ ($326$nm) transitions for all naturally occurring isotopes of cadmium. The isotope…

Peik and Tamm [Europhys. Lett. 61, 181 (2003)] proposed a nuclear clock based on the isomeric transition between the ground state and the first excited state of thorium-229. This transition was recognized as a potentially sensitive probe of…

Atomic Physics · Physics 2021-01-19 Pavel Fadeev , Julian C. Berengut , Victor V. Flambaum

The low-lying isomeric state of $^{229}$Th provides unique opportunities for high-resolution laser spectroscopy of the atomic nucleus. We determine the energy of this isomeric state by taking the absolute energy difference between the…

The isomeric and {\beta} decays of the N = Z +2 nucleus 96Ag were investigated at NSCL. A cascade of {\gamma}-ray transitions originating from the de-excitation of a {\mu}s isomer was observed for the first time and was found in coincidence…

We observe a weakly allowed optical transition of atomic ytterbium from the ground state to the metastable state $4f^{13}5d6s^2 \: (J=2)$ for all five bosonic and two fermionic isotopes with resolved Zeeman and hyperfine structures. This…

Atomic Physics · Physics 2023-04-18 Taiki Ishiyama , Koki Ono , Tetsushi Takano , Ayaki Sunaga , Yoshiro Takahashi

We estimate the range of the radiative lifetime and energy of the anomalous, low-energy $3/2^+(7.8 \pm 0.5$ eV) state in the $^{229}$Th nucleus. Our phenomenological calculations are based on the available experimental data for the…

Atomic Physics · Physics 2015-12-09 E. V. Tkalya , Christian Schneider , Justin Jeet , Eric R. Hudson

The endohedral fullerene $^{15}\mathrm{N@C}_{60}$ has narrow electron paramagnetic resonance lines which have been proposed as the basis for a condensed-matter portable atomic clock. We measure the low-frequency spectrum of this molecule,…

State-resolved laser spectroscopy at the 10$^{-12}$ precision level recently reported in $arXiv$:2406.18719 determined the fractional change in nuclear quadrupole moment between the ground and isomeric state of $^{229}\rm{Th}$, $\Delta…

The lifetime of the 3163 keV, 7/2$^-$ isomeric state in $^{35}Cl$ that decays by a stretched M2 transition to the $3/2^+$ ground state, has been re-measured using the Doppler Shift Attenuation Method, by gating on the 1185 keV transition…

Contemporary data are analyzed concerning the half-lives of the $^{229m}$Th isomer in neutral atoms and various ions. It is explicitly shown that the isomer lifetime may strongly depend on the plain environmental physical conditions like…

Nuclear Theory · Physics 2018-03-14 F. F. Karpeshin , M. B. Trzhaskovskaya , L. F. Vitushkin

A high-precision measurement of the electron-capture (EC) decay $Q$ value for the ground-state-to-ground-state (gs-to-gs) transition of $^{113}$Sn to $^{113}$In has been performed using the JYFLTRAP double Penning trap mass spectrometer.…

The first excited isomeric state of $^{229}$Th possesses the lowest energy among all known excited nuclear states. The expected energy is accessible with today's laser technology and in principle allows for a direct optical laser excitation…

Nuclear Experiment · Physics 2018-01-17 Benedict Seiferle , Lars von der Wense , Peter G. Thirolf
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