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Hyperfine-structure constants of odd Ra$^{+}$ due to the interactions of nuclear magnetic dipole, electric quadrupole, and magnetic octupole moments with the electrons are investigated in the framework of relativistic coupled-cluster method…

Atomic Physics · Physics 2021-03-16 Fei-Chen Li , Yong-Bo Tang , Hao-Xue Qiao , Ting-Yun Shi

Electric dipole moment (EDM) measurements using paramagnetic molecules have significantly advanced over the last decade. Traditionally, these experiments have been analyzed in terms of the electron EDM. However, paramagnetic molecules are…

High Energy Physics - Phenomenology · Physics 2026-05-20 Wouter Dekens , Jordy de Vries , Lemonia Gialidi , Javier Menéndez , Heleen Mulder , Beatriz Romeo

We investigate the microwave spectra of ultracold alkali metal dimers in magnetic, electric and combined fields, taking account of the hyperfine structure due to the nuclear spins. We consider the molecules 41K87Rb and 7Li133Cs, which are…

Chemical Physics · Physics 2015-05-14 Hong Ran , J. Aldegunde , Jeremy M. Hutson

The energy splitings for $J = 1$, $F=3/2$, $|M_F|=3/2$ hyperfine levels of the $^3\Delta_1$ electronic state of $^{180}$Hf$^{19}$F$^+$ ion are calculated as functions of the external variable electric and magnetic fields within two…

Atomic Physics · Physics 2018-05-16 A. N. Petrov

In this paper, dye sensitized solar cell based on nano dye molecule N3 are investigated by using density functional computations. The main focus is on the N3 dye molecule and corresponding complexes formed at the interface between…

Materials Science · Physics 2017-05-02 E. Shomali , I. Abdolhosseini Sarsari , S. Javad Hashemifar , M. Alaei

We investigate the $2\,^3\!S_1$--$2\,^3\!P_J$ ($J = 0, 1, 2$) transitions in $\rm^6Li^+$ using the optical Ramsey technique and achieve the most precise values of the hyperfine splittings of the $2\,^3\!S_1$ and $2\,^3\!P_J$ states, with…

The electric dipole moment (EDM) of paramagnetic atoms is sensitive to the intrinsic EDM contribution from that of its constituent electrons and a scalar--pseudo-scalar (S-PS) electron-nucleus interactions. The electron EDM and the S-PS EDM…

Atomic Physics · Physics 2008-07-16 H. S. Nataraj , B. K. Sahoo , B. P. Das , D. Mukherjee

Triatomic molecule RaOH combines the advantages of laser-coolability and the spectrum with close opposite-parity doublets. This makes it a promising candidate for experimental study of the $\mathcal{P}$,$\mathcal{T}$-violation. Previous…

Atomic Physics · Physics 2021-03-17 Anna Zakharova , Alexander Petrov

We investigate two-dimensional electric dipole sheets in the superlattice made of BaTiO$_{3}$ and BaZrO$_{3}$ using first-principles-based Monte-Carlo simulations and density functional calculations. Electric dipole domains and complex…

Materials Science · Physics 2015-06-22 Zhijun Jiang , Bin Xu , Fei Li , Dawei Wang , C. -L. Jia

Fully numerical mesh solutions of 2D quantum equations of Schroedinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of atoms and…

Atomic Physics · Physics 2015-06-26 Mikhail V. Ivanov , Peter Schmelcher

An algorithm for the calculation of hyperfine structure and spectra of diatomic molecules based on the variational nuclear motion is presented. Hyperfine coupling terms considered are Fermi-contact, nuclear spin-electron spin dipole-dipole,…

Chemical Physics · Physics 2022-02-15 Qianwei Qu , Sergei N. Yurchenko , Jonathan Tennyson

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. In homonuclear molecular ions the electric dipole $E1$ transitions are…

Atomic Physics · Physics 2021-01-20 P. Danev , D. Bakalov , V. I. Korobov , S. Schiller

Measuring the hyperfine structure (HFS) of long-lived $^3P_2$ states of divalent atoms may offer the opportunity of extracting relatively unexplored nuclear magnetic octupole and electric hexadecapole moments. Here, using relativistic…

Atomic Physics · Physics 2009-11-13 K. Beloy , A. Derevianko , W. R. Johnson

A theoretical model of hyperfine spectra of nuclear spin conversion of molecular isomers has been developed. The model takes into account the nuclear spin-spin and spin-rotation interactions, as well as the saturation of intramolecular…

Chemical Physics · Physics 2009-11-06 Pavel L. Chapovsky

We identify a potential means to extract the $^{229g}$Th $\rightarrow$ $^{229m}$Th nuclear excitation energy from precision microwave spectroscopy of the $5F_{5/2,7/2}$ hyperfine manifolds in the ion $^{229g}$Th$^{3+}$. The hyperfine…

Atomic Physics · Physics 2014-02-14 K. Beloy

A method for precise calculation of the energy corrections due to second order electric quadrupole interactions, as well as mixed electric quadrupole-vacuum polarization in the framework of the dynamic hyperfine structure in heavy muonic…

Atomic Physics · Physics 2019-04-10 Niklas Michel , Natalia S. Oreshkina

We have applied the Finite Element Method to the self-consistent electronic structure calculations of molecules and solids for the first time. In this approach all the calculations are performed in "real space" and the use of non-uniform…

mtrl-th · Physics 2009-10-28 Eiji Tsuchida , Masaru Tsukada

The electric dipole moment of an electron (eEDM) is one of the sensitive probes of physics beyond the standard model. The possible existence of the eEDM gives rise to an experimentally observed energy shift, which is proportional to the…

Computational Physics · Physics 2017-01-18 A. Sunaga , M. Abe , M. Hada , B. P. Das

The relativistic coupled-cluster (RCC) method is a powerful many-body method, particularly in the evaluation of electronic wave functions of heavy atoms and molecules, and can be used to calculate various atomic and molecular properties.…

Atomic Physics · Physics 2019-12-09 Nanako Shitara , B. K. Sahoo , T. Watanabe , B. P. Das

We calculate for the first time the electric dipole moment (EDM) of the $^6$Li nucleus within the alpha + p + n three-body cluster model using the Gaussian expansion method, assuming the one meson exchange P, CP-odd nuclear forces. It is…

Nuclear Theory · Physics 2015-05-28 Nodoka Yamanaka , Emiko Hiyama