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Polar polyatomic molecules provide an ideal but largely unexplored platform to encode qubits in rotational states. Here, we trap cold (100-600 mK) formaldehyde (H$_2$CO) inside an electric box and perform a Ramsey-type experiment to observe…

Atomic Physics · Physics 2025-04-01 Maximilian Löw , Martin Ibrügger , Gerhard Rempe , Martin Zeppenfeld

In weakly bound diatomic molecules, energy levels are closely spaced and thus more susceptible to mixing by magnetic fields than in the constituent atoms. We use this effect to control the strengths of forbidden optical transitions in…

Atomic Physics · Physics 2015-12-22 B. H. McGuyer , M. McDonald , G. Z. Iwata , W. Skomorowski , R. Moszynski , T. Zelevinsky

Permanent electric dipole moments (EDMs) violate parity and time reversal symmetry. Within the Standard Model (SM) they are many orders of magnitude below present experimental sensitivity. Many extensions of the SM predict much larger EDMs,…

High Energy Physics - Experiment · Physics 2012-04-12 Gerco Onderwater

In the development of atomic clocks, some atomic transition frequencies are measured with remarkable precision. These measured spectra may include effects of a new force mediated by a weakly interacting boson. Such effects might be…

High Energy Physics - Phenomenology · Physics 2017-12-27 Kyoko Mikami , Minoru Tanaka , Yasuhiro Yamamoto

Searches for intrinsic electric dipole moments (EDMs) of nucleons, atoms and molecules are precision flavor-diagonal probes of new $CP$-odd physics, as motivated by the need to explain the matter-antimatter asymmetry in the universe. We…

High Energy Physics - Phenomenology · Physics 2026-03-19 Maxim Pospelov , Adam Ritz

Oriented external electric fields are ubiquitous in chemistry; however, the effects of fields applied in different directions on molecular systems remain underexplored. A major challenge is that an applied field exerts a torque on a…

Chemical Physics · Physics 2026-05-12 Duc Anh Lai , Devin A. Matthews

Searches for the nuclear magnetic quadrupole moment (MQM) and nuclear Schiff moment (NSM) have high discovery potential for violations of time ($T$) and parity ($P$) reversal symmetries beyond the Standard Model. Molecules containing heavy…

Atomic Physics · Physics 2025-09-16 Xing Fan , Lan Cheng

We are pursuing an experiment to measure the electric dipole moment of the electron using the molecule PbO. This measurement requires the ability to prepare quantum states with orientation of the molecular axis and, simultaneously,…

Atomic Physics · Physics 2013-05-29 S. Bickman , P. Hamilton , Y. Jiang , D. DeMille

High-precision measurements of violations of fundamental symmetries in atoms are a very effective means of testing the standard model of elementary particles and searching for new physics beyond it. Such studies complement measurements at…

Atomic Physics · Physics 2009-08-18 J. S. M. Ginges , V. V. Flambaum

Hyperfine-induced electric dipole contributions may significantly increase probabilities of otherwise very weak electric octupole and magnetic quadrupole atomic clock transitions (e.g. transitions between $s$ and $f$ electron orbitals).…

Atomic Physics · Physics 2016-06-01 V. A. Dzuba , V. V. Flambaum

Heavy polar molecules can be used to measure the electric dipole moment of the electron, which is a sensitive probe of physics beyond the Standard Model. The value is determined by measuring the precession of the molecule's spin in a plane…

Atomic Physics · Physics 2010-01-29 M. R. Tarbutt , J. J. Hudson , B. E. Sauer , E. A. Hinds

Recently the YbOH molecule has been suggested as a candidate to search for the electron electric dipole moment (eEDM) which violates spatial parity (P) and time-reversal (T) symmetries [I. Kozyryev and N. R. Hutzler, Phys. Rev. Lett. 119,…

Atomic Physics · Physics 2021-02-15 D. E. Maison , V. V. Flambaum , N. R. Hutzler , L. V. Skripnikov

The present constraint on the space parity ($\mathcal{P}$) and time reflection invariance ($\mathcal{T}$) violating electron electric dipole moment ($e$EDM) is based on the observation of the electron spin precession in an external electric…

Atomic Physics · Physics 2021-04-07 D. V. Chubukov , L. V. Skripnikov , A. N. Petrov , V. N. Kutuzov , L. N. Labzowsky

This article reviews the current state of the art in the field of cold and ultracold molecules and demonstrates that chemical reactions, inelastic collisions and dissociation of molecules at subKelvin temperatures can be manipulated with…

Atomic Physics · Physics 2015-06-26 R. V. Krems

The electric dipole moment of an electron (eEDM) is one of the sensitive probes of physics beyond the standard model. The possible existence of the eEDM gives rise to an experimentally observed energy shift, which is proportional to the…

Computational Physics · Physics 2017-01-18 A. Sunaga , M. Abe , M. Hada , B. P. Das

Electrical control of spins at the nanoscale offers significant architectural advantages in spintronics, because electric fields can be confined over shorter length scales than magnetic fields. Thus, recent demonstrations of electric-field…

Mesoscale and Nanoscale Physics · Physics 2021-10-15 Junjie Liu , Jakub Mrozek , Aman Ullah , Yan Duan , José J. Baldoví , Eugenio Coronado , Alejandro Gaita-Ariño , Arzhang Ardavan

Present limit on the electron electric dipole moment ($e$EDM) is based on the electron spin precession measurement. We propose an alternative approach - observation of the $\mathcal{P}$,$\mathcal{T}$-odd Faraday effect in an external…

Atomic Physics · Physics 2019-07-30 D. V. Chubukov , L. V. Skripnikov , L. Bougas , L. N. Labzowsky

Cold molecules provide an excellent platform for quantum information, cold chemistry, and precision measurement. Certain molecules have enhanced sensitivity to beyond Standard Model physics, such as the electron's electric dipole moment…

We propose a very sensitive method for measuring the electric dipole moment of the electron using polar molecules embedded in a cryogenic solid matrix of inert-gas atoms. The polar molecules can be oriented in the $\hat{\rm{z}}$ direction…

Atomic Physics · Physics 2018-01-29 A. C. Vutha , M. Horbatsch , E. A. Hessels

A new generation of atomic sensors using ultra-narrow optical clock transitions and composite pulses are pushing quantum engineering control to a very high level of precision for applied and fundamental physics. Here, we propose a new…

Atomic Physics · Physics 2022-02-15 T. Zanon-Willette , D. Wilkowski , A. V. Taichenachev , V. I. Yudin