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Raman spectroscopy reveals chemically specific information and provides label-free insight into the molecular world. However, the signals are intrinsically weak and call for enhancement techniques. Here, we demonstrate Purcell enhancement…

The use of coherent light for precision measurements has been a key driving force for numerous research directions, ranging from biomedical optics to semiconductor manufacturing. Recent work demonstrates that the precision of such…

Optics · Physics 2021-07-29 Dorian Bouchet , Stefan Rotter , Allard P. Mosk

State-preserving frequency conversion in the optical domain is a necessary component in many configurations of quantum information processing and communication. Thus far, nonlinear crystals are used for this purpose. Here, we report on a…

Quantum Physics · Physics 2022-12-28 Alireza Aghababaei , Christoph Biesek , Frank Vewinger , Simon Stellmer

Atomic-resolution scanning transmission electron microscopy (STEM) characterization requires precise tilting of the specimen to high symmetric zone axis, which is usually processed in reciprocal space by following the diffraction patterns.…

Materials Science · Physics 2024-06-04 Jiake Wei , Zhangze Xu , Wenjie Shen , Bin Feng , Ryo Ishikawa , Naoya Shibata , Yuichi Ikuhara , Xuedong Bai

We use a Langevin approach to analyze the quantum noise in Coherent Anti-Stokes Raman Spectroscopy (CARS) in several experimental scenarios: with continuous wave input fields acting simultaneously and with fast sequential pulsed lasers…

Statistical Mechanics · Physics 2009-11-10 Kunal K. Das , G. S. Agarwal , Yu. M. Golubev , M. O. Scully

The "Impulsive Stimulated Raman Scattering" (ISRS), is generally performed using ultrashort laser pulses. It shifts the frequency of the laser beam without any change of the wave surfaces and any appearance of extra lines. ISRS works with…

Astrophysics · Physics 2007-05-23 Jacques Moret-Bailly

Interference of light fields plays an important role in various high-precision measurement schemes. It has been shown that super resolving phase measurements beyond the standard coherent state limit can be obtained either by using maximally…

Quantum Physics · Physics 2013-10-08 Emanuele Distante , Miroslav Jezek , Ulrik L. Andersen

Using a model system, we demonstrate both experimentally and theoretically that coherent scattering of light can be robust in hot atomic vapors despite a significant Doppler effect. By operating in a linear regime of far-detuned light…

There has been much recent interest in quantum optical interferometry for applications to metrology, sub-wavelength imaging, and remote sensing, such as in quantum laser radar (LADAR). For quantum LADAR, atmospheric absorption rapidly…

Quantum Physics · Physics 2015-05-13 Yang Gao , Christoph F. Wildfeuer , Petr M. Anisimov , Hwang Lee , Jonathan P. Dowling

Through temporal shaping of the excitation signal, the complex-frequency scattering zeros of a lossless structure can be accessed, enabling a storage-release mechanism referred to as coherent virtual absorption. Practical demonstrations of…

We show that the increasingly popular nonlinear optical technique of time-domain coherent anti-Stokes Raman scattering (CARS), which is usually understood in terms of the semiclassical time-dependent third-order polarization, can be equally…

Optics · Physics 2014-06-03 Michele Marrocco

Multi-photon interference is at the heart of photonic quantum technologies. Arrays of integrated cavities can support bright sources of single-photons with high purity and small footprint, but the inevitable spectral distinguishability…

Superresolution refers to the estimation of parameters of an image with an accuracy beyond standard classical techniques such as direct detection. In seminal work by Lu et al., a measurement to estimate the separation distance of two point…

Quantum Physics · Physics 2022-06-30 Hari Krovi

We describe a detector that measures the mutual coherence of two optical fields directly using quantum interference, free from photon noise of the individual irradiances. Our approach utilizes Raman transition in an atomic system where the…

Quantum Physics · Physics 2008-12-16 Jungsang Kim , David J. Brady

Achieving resolution in the sub-Rayleigh regime (superresolution) is one of the rapidly developing topics in quantum optics and metrology. Recently, it was shown that perfect measurement based on spatial mode demultiplexing (SPADE) in…

Quantum Physics · Physics 2025-04-01 Konrad Schlichtholz , Łukasz Rudnicki

Three-dimensional phase contrast imaging of multiply-scattering samples in X-ray and electron microscopy is extremely challenging, due to small numerical apertures, the unavailability of wavefront shaping optics, and the highly nonlinear…

Computational Physics · Physics 2021-06-02 Philipp M Pelz , Hamish G Brown , Jim Ciston , Scott D Findlay , Yaqian Zhang , Mary Scott , Colin Ophus

A chirped-pulse quantum control scheme applicable to Coherent Anti-Stokes Raman Scattering spectroscopy, named as C-CARS, is presented aimed at maximizing the vibrational coherence in molecules. It implies chirping of three incoming pulses…

Quantum Physics · Physics 2022-12-19 Jabir Chathanathil , Dmitry Budker , Svetlana A. Malinovskaya

We present a scheme to obtain the coherently enhanced Raman scattering in atomic vapor which is induced by a spin wave initially written by a weak write laser. The enhancement of Raman scattering is dependent on the number and the spatial…

Quantum Physics · Physics 2015-05-19 Chun-Hua Yuan , L. Q. Chen , Jietai Jing , Z. Y. Ou , Weiping Zhang

Quantum channels in free-space, an essential prerequisite for fundamental tests of quantum mechanics and quantum technologies in open space, have so far been based on direct line-of-sight because the predominant approaches for…

Quantum Physics · Physics 2021-03-02 Shihan Sajeed , Thomas Jennewein

Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…

Quantum Physics · Physics 2023-05-26 Joel Jiahao Fan , Zhe-Yu Jeff Ou , Zhedong Zhang