Related papers: Probing electronic state-dependent conformational …
The structure and photoexcitation dynamics of high lying doubly excited states of the strontium atom with high angular momenta are studied in the vicinity of the Sr$^+(N=5)$ threshold. The spectra recorded using resonant multiphoton…
The electronic properties of solids are determined by the crystal structure and interactions between electrons, giving rise to a variety of collective phenomena including superconductivity, strange metals and correlated insulators. The…
Transition metal doping is commonly used for altering the properties of solid-state materials to suit applications in science and technology. Partially filled $d$-shells of transition metal atoms lead to electronic states with diverse…
Resolving the locations and discriminating the spin states of individual trapped ions with high fidelity is critical for a large class of applications in quantum computing, simulation, and sensing. We report on a method for high-fidelity…
Charging of a clean two-dimensional island is studied in the regime of small concentration of electrons when they form the Wigner crystal. Two forms of electron-electron interaction potential are studied: the pure Coulomb interaction and…
We report on the implementation of quantum state tomography for an ensemble of Eu$^{3+}$ dopant ions in a \YSO crystal. The tomography was applied to a qubit based on one of the ion's optical transitions. The qubit was manipulated using…
Spontaneous symmetry breaking and formation of self-organized structures in nonlinear systems are intriguing and important phenomena in nature. Advancing such research to new nonlinear optical regimes is of much interest for both…
The quantum mechanical states of electrons in atoms and molecules are distinct orbitals, which are fundamental for our understanding of atoms, molecules and solids. Electronic orbitals determine a wide range of basic atomic properties,…
We report the sudden and spontaneous evolution of an initially correlated gas of repulsively interacting Rydberg atoms to an ultracold plasma. Under continuous laser coupling we create a Rydberg ensemble in the strong blockade regime, which…
We consider temperature-induced melting of a Wigner solid in one dimensional (1D) and two dimensional (2D) lattices of electrons interacting via the long-range Coulomb interaction in the presence of strong disorder arising from charged…
We explore how the extraordinary properties of Rydberg atoms can be employed to impact the motion of ultracold ground state atoms. Specifically, we use an off-resonant two-photon laser dressing to map features of the Rydberg states on…
We study spin-phonon coupled dynamics in the vicinity of a sloped conical intersection created by laser coupling the electronic (spin) and vibrational degrees of freedom of a pair of trapped Rydberg ions. We show that the shape of the…
Dynamic control of atomic dressing to the highly-excited Rydberg state in multi-level systems has special appeals owing to the development of flexible and precise measurement. In this study we develop an experimentally-accessible proposal…
We experimentally studied the Rydberg level shift caused by the electric field, which is generated by Rydberg atom collision induced ionization in a cesium atomic ensemble. The density of charged particles caused by collisions between…
The choice that a solid system "makes" when adopting a crystal structure (stable or metastable) is ultimately governed by the interactions between electrons forming chemical bonds. By analyzing 6 prototypical binary transition-metal…
The physics of interacting quantum wires has attracted a lot of attention recently. When the density of electrons in the wire is very low, the strong repulsion between electrons leads to the formation of a Wigner crystal. We review the rich…
In the construction of diabatic vibronic Hamiltonians for quantum dynamics in the excited-state manifold of molecules, the coupling constants are often extracted solely from information on the excited-state energies. Here, a new protocol is…
When two-dimensional electrons are subjected to a very strong magnetic field, they are believed to form a triangular Wigner crystal. We demonstrate that, in the entire crystal phase, this crystal is very well represented by a…
We study the impact of Rydberg molecule formation on the storage and retrieval of Rydberg polaritons in an ultracold atomic medium. We observe coherent revivals appearing in the retrieval efficiency of stored photons that originate from…
A Rydberg molecule is composed of an outer electron that collides on the residual ionic core. Typical states of Rydberg molecules display entanglement between the outer electron and the core. In this work we quantify the average…