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Coherent Raman scattering provides highly sensitive vibrational analysis through nonlinear light-matter interactions. However, its application to metal interfaces has remained challenging because the intrinsically large non-resonant…

We study coherent anti-Stokes Raman spectroscopy in air-filled anti-resonance hollow-core photonic crystal fiber, otherwise known as 'revolver' fiber. We compare the vibrational coherent anti-Stokes Raman signal of N$_2$, at 2331 cm$^{-1}$,…

We present a new collection of processing techniques, collectively "factorized Kramers--Kronig and error correction" (fKK-EC), for (a) Raman signal extraction, (b) denoising, and (c) phase- and scale-error correction in coherent anti-Stokes…

Signal Processing · Electrical Eng. & Systems 2020-12-10 Charles H. Camp , John S. Bender , Young Jong Lee

Diffuse speckle contrast analysis (DSCA), also called speckle contrast optical spectroscopy(SCOS), has emerged as a groundbreaking optical imaging technique for tracking dynamic biological processes, including blood flow and tissue…

We experimentally demonstrate efficient Raman conversion to respective Stokes and anti-Stokes fields in both pulsed and continuous modes with a Rb-87 atomic vapor cell. The conversion efficiency is about 40-50% for the Stokes field and…

Atomic Physics · Physics 2012-10-19 Bing Chen , Kai Zhang , Chun-Hua Yuan , Chengling Bian , Cheng Qiu , L. Q. Chen , Z. Y. Ou , Weiping Zhang

Light detection and ranging (LiDAR) is widely used in autonomous systems and industrial metrology; however, the simultaneous acquisition of three-dimensional (3D) structure and broadband spectral information remains challenging, as…

The principle and experimental realization of a novel Raman spectroscopic technique entitled stimulated Raman phase shift (SRPS) spectroscopy was demonstrated. This technique depends on the measurement of the stimulated Raman scattering…

Optics · Physics 2024-03-07 Meng Qi , Wenrong Wang , Yuan-ji Li , Jin-xia Feng , Kuan-shou Zhang

The Herschel SPIRE Fourier transform spectrometer (FTS) performs spectral imaging in the 447-1546 GHz band. It can observe in three spatial sampling modes: sparse mode, with a single pointing on sky, or intermediate or full modes with 1 and…

Femtosecond, broadband stimulated Raman spectroscopy is a popular approach to measuring molecular dynamics with excellent signal-to-noise and spectral resolution. We present a new method for broadband stimulated Raman spectroscopy that…

Optics · Physics 2025-08-19 Nathan G. Drouillard , TJ Hammond

Thanks to their highly coherent emission and compact form factor, single axial mode diamond Raman lasers have been identified as a valuable asset for applications including integrated quantum technology, high resolution spectroscopy or…

Optics · Physics 2022-08-17 Georgios Stoikos , Eduardo Granados

We show that coherent anti-Stokes Raman lineshapes do not follow known spectral profiles if the time asymmetry of realistic laser pulses is taken into account. Examples are given for nanosecond and picosecond laser pulses commonly employed…

Optics · Physics 2015-06-22 Michele Marrocco , Emil Nordström , Per-Erik Bengtsson

We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously…

Spatial transcriptomics (ST) is a novel technique that simultaneously captures pathological images and gene expression profiling with spatial coordinates. Since ST is closely related to pathological features such as disease subtypes, it may…

Computer Vision and Pattern Recognition · Computer Science 2025-03-11 Kazuya Nishimura , Ryoma Bise , Yasuhiro Kojima

We present a new interferometric technique for measuring Coherent Anti-Stokes Raman Scattering (CARS) and Second Harmonic Generation (SHG) signals. Heterodyne detection is employed to increase the sensitivity in both CARS and SHG signal…

Optics · Physics 2009-11-10 C. Vinegoni , J. S. Bredfeldt , D. L. Marks , S. A. Boppart

Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…

Space-time (ST) wave packets are coherent pulsed beams that propagate diffraction-free and dispersion-free by virtue of tight correlations introduced between their spatial and temporal spectral degrees of freedom. Less is known of the…

The process in which Raman scattering produces correlated Stokes and anti-Stokes radiation is known as Stokes--anti-Stokes (SaS) scattering. It has been shown recently that this process can generate entangled photon pairs, making it a…

Quantum Physics · Physics 2025-09-30 Raul Corrêa , Marcelo F. Santos , Carlos H. Monken , Ado Jorio

Spontaneous vibrational Raman scattering is a ubiquitous form of light-matter interaction whose description necessitates quantization of the electromagnetic field. It is usually considered as an incoherent process because the scattered…

Quantum Physics · Physics 2023-07-18 Valeria Vento , Santiago Tarrago Velez , Anna Pogrebna , Christophe Galland

Fourier-transform spectroscopy (FTS) has been widely used as a standard analytical technique over the past half-century. FTS is a simple and robust autocorrelation-based technique that is compatible with both temporally coherent and…

Instrumentation and Detectors · Physics 2018-11-21 Kazuki Hashimoto , Takuro Ideguchi

We demonstrate a method to double the collection efficiency in Laser Tweezers Raman Spectroscopy (LTRS) by collecting both the forward and back-scattered light in a single-shot multitrack measurement. Our method can collect signals at…

Optics · Physics 2021-06-09 Tobias Dahlberg , Magnus Andersson
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