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Phase change materials provide a powerful platform for dynamically modulating optical responses in nanophotonic systems. While plasmonic metasurfaces have been widely employed to enhance photocatalytic efficiency and promote particular…

Molecular polaritons, hybrid light-matter states resulting from strong cavity coupling of optical transitions, may provide a new route to guide chemical reactions. However, demonstrations of cavity-modified reactivity in clean benchmark…

Chemical Physics · Physics 2024-08-20 Liying Chen , Ashley P. Fidler , Alexander M. McKillop , Marissa L. Weichman

Recent experiments have demonstrated that polariton formation provides a novel strategy for modifying local molecular processes when a large ensemble of molecules is confined within an optical cavity. Herein, a numerical strategy based on…

Chemical Physics · Physics 2025-05-16 Andres Felipe Bocanegra Vargas , Tao E. Li

Integrated photonics has been a promising platform for analog quantum simulation of condensed matter phenomena in strongly correlated systems. To that end, we explore the implementation of all-photonic quantum simulators in coupled cavity…

Two-dimensional photonic crystal membranes provide a versatile planar architecture for integrated photonics to control the propagation of light on a chip employing high quality optical cavities, waveguides, beamsplitters or dispersive…

We present the effects of resonator birefringence on the cavity-enhanced interfacing of quantum states of light and matter, including the first observation of single photons with a time-dependent polarisation state that evolves within their…

Quantum Physics · Physics 2019-03-27 Thomas D. Barrett , Oliver Barter , Dustin Stuart , Ben Yuen , Axel Kuhn

We theoretically demonstrate that chemical reaction rate constant can be significantly suppressed by coupling molecular vibrations with an optical cavity, exhibiting both the collective coupling effect and the cavity-frequency modification…

Chemical Physics · Physics 2022-01-26 Arkajit Mandal , Xinyang Li , Pengfei Huo

The observation that materials can change their properties when placed inside or near an optical resonator, has sparked a fervid interest in understanding the effects of strong light-matter coupling on molecular dynamics, and several…

Chemical Physics · Physics 2024-03-20 Ilia Sokolovskii , Gerrit Groenhof

In this article, we present a numerical study of the optical properties of a metal nanowire interacting with a localized cavity in a two dimensional photonic crystal. The nature of the modes, their wavelength and width are investigated as a…

We study the coupling between photonic molecules and waveguides in photonic crystal slab structures using finite-difference time-domain method and coupled mode theory. In a photonic molecule with two cavities, the coupling of cavity modes…

Optics · Physics 2015-04-08 Yanhui Zhao , Chenjiang Qian , Kangsheng Qiu , Yunan Gao , Xiulai Xu

Exploring the dynamics of an optically levitated dielectric micro- and nanoparticle is an exciting new subject in quantum science. Recent years have witnessed rapid advancements in attaining quantum-limited optical detection and control of…

Optics · Physics 2025-04-22 Seyed Khalil Alavi , Zijie Sheng , Haneul Lee , Hansuek Lee , Sungkun Hong

Microwave cavity resonators are crucial components of many quantum technologies and are a promising platform for hybrid quantum systems, as their open architecture enables the integration of multiple subsystems inside the cavity volume. To…

Instrumentation and Detectors · Physics 2022-02-23 Myles Ruether , Clinton A. Potts , John P. Davis , Lindsay J. LeBlanc

We present a combined analytical and numerical study for coherent terahertz control of a single molecular polariton, formed by strongly coupling two rotational states of a molecule with a single-mode cavity. Compared to the bare molecules…

Quantum Physics · Physics 2023-02-08 Li-Bao Fan , Chuan-Cun Shu , Daoyi Dong , Jun He , Niels E. Henriksen , Franco Nori

We introduce a numerical procedure which permits to drastically accelerate the design of multimode photonic crystal resonators. Specifically, we demonstrate that the optical response of an important class of such nanoscale structures is…

Several years ago, it was shown that strong coupling between an electronic transition in organic molecules and a resonant photonic structure can modify the electronic landscape of the molecules and affect their chemical behavior. Since…

We propose a cavity QED approach to describe light-matter interaction between an individual anharmonic molecular vibration and an infrared cavity field. Starting from a generic Morse oscillator with quantized nuclear motion, we derive a…

Chemical Physics · Physics 2019-10-16 Federico Hernández , Felipe Herrera

Using carefully designed hybrid metal-dielectric resonators, we study molecular optomechanics in the strong coupling regime ($g_{\rm }^2/\omega_m {>} \kappa$), which manifests in anharmonic emission lines in the sideband-resolved region of…

Mesoscale and Nanoscale Physics · Physics 2019-11-28 Mohsen Kamandar Dezfouli , Reuven Gordon , Stephen Hughes

A quantum system composed of a molecule and an atomic ensemble, confined in a microscopic cavity, is investigated theoretically. The indirect coupling between atoms and the molecule, realized by their interaction with the cavity radiation…

Chemical Physics · Physics 2020-05-05 Tamás Szidarovszky , Gábor J. Halász , Ágnes Vibók

The mechanical properties of light have found widespread use in the manipulation of gas-phase atoms and ions, helping create new states of matter and realize complex quantum interactions. The field of cavity-optomechanics strives to scale…

Optics · Physics 2015-08-24 Kejie Fang , Matthew H. Matheny , Xingsheng Luan , Oskar Painter

We investigate the chemical reactivity of molecular populations confined inside a nanofluidic Fabry-P{\'e}rot cavity. Due to strong light-matter interactions developing between a resonant electromagnetic cavity-mode and the electric dipole…

Mesoscale and Nanoscale Physics · Physics 2021-04-21 L Mauro , K Caicedo , G Jonusauskas , Rémi Avriller
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