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In this work, we show the short-time existence of solutions of the evolution equations that represent the solid state dewetting of thin films through evaporation-condensation as a two dimensional sharp interface variational model. The…

Analysis of PDEs · Mathematics 2025-08-12 M. S. Indulekha

Dewetting of ultra-thin polymer films near the glass transition exhibits unexpected front morphologies [G. Reiter, Phys. Rev. Lett., 87, 186101 (2001)]. We present here the first theoretical attempt to understand these features, focusing on…

Soft Condensed Matter · Physics 2009-11-07 F. Saulnier , E. Raphael , P. -G. de Gennes

We report on the dewetting of a monolayer on a solid substrate, where mass transport occurs via surface diffusion. For a wide range of parameters, a labyrinthine pattern of bilayer islands is formed. An irreversible regime and a…

Soft Condensed Matter · Physics 2009-11-13 Olivier Pierre-Louis , Anna Chame , Yukio Saito

The stability of thin liquid coatings is of fundamental interest in every- day life. Homogeneous and non-volatile liquid coatings may dewet either by heterogeneous nucleation, thermal nucleation, or spinodal dewetting. Wetting and dewetting…

Soft Condensed Matter · Physics 2008-05-29 Karin Jacobs , Ralf Seemann , Stephan Herminghaus

This study reveals the influence of the surface energy and solid/liquid boundary condition on the breakup mechanism of dewetting ultra-thin polymer films. Using silane self-assembled monolayers, SiO$_2$ substrates are rendered hydrophobic…

Soft Condensed Matter · Physics 2017-05-03 Matthias Lessel , Joshua D. McGraw , Oliver Bäumchen , Karin Jacobs

Solidification is an important process in many alloy processing routes. The solidified microstructure of alloys is usually made up of dendrites, eutectics or a combination of both. The evolving morphologies are largely determined by the…

Materials Science · Physics 2024-12-17 Marco Seiz , Michael Kellner , Britta Nestler

We develop a sharp-interface model for solid-state dewetting of double-bubble thin films using an energy variational approach based on a newly proposed interfacial energy. This model characterizes the dynamic evolution of interfaces in…

Numerical Analysis · Mathematics 2025-03-06 Meng Li , Nan Wang , Ruofan Zhao , Chunjie Zhou

We propose an accurate and energy-stable parametric finite element method for solving the sharp-interface continuum model of solid-state dewetting in three-dimensional space. The model describes the motion of the film\slash vapor interface…

Numerical Analysis · Mathematics 2023-07-04 Weizhu Bao , Quan Zhao

In this work, we consider the solid-state dewetting of an axisymmetric thin film on a curved-surface substrate, with the assumption that the substrate morphology is also axisymmetric. Under the assumptions of axisymmetry, the surface…

Numerical Analysis · Mathematics 2025-01-03 Zhenghua Duan , Meng Li , Chunjie Zhou

Dewetting of thin polystyrene films deposited onto silicone wafers at temperatures close to the glass transition exhibits unusual dynamics and front morphologies. Here, we present a new theoretical approach of these phenomena taking into…

Soft Condensed Matter · Physics 2007-05-23 Elie Raphael , Thomas Vilmin

We have studied the breakup and subsequent fluid flow in very thin films of partially wetting liquid on solid substrates, using molecular dynamics simulations. The liquid is made of short chain molecules interacting with Lennard-Jones…

Soft Condensed Matter · Physics 2009-10-31 Joel Koplik , Jayanth R. Banavar

The dewetting of thin nanofilms is significantly impacted by thermal fluctuations, liquid-solid slip, and disjoining pressure, which can be described by lubrication equations augmented by appropriately scaled noise terms, known as…

Fluid Dynamics · Physics 2024-10-29 Yixin Zhang

We report on three key processes involving atomic step motion during the dewetting of thin solid films: (i) the growth of an isolated island nucleated far from a hole, (ii) the spreading of a monolayer rim, and (iii) the zipping of a…

Materials Science · Physics 2015-05-18 O. Pierre-Louis , A. Chame , M. Dufay

The performance of solution-processed solar cells strongly depends on the geometrical structure and roughness of the photovoltaic layers formed during film drying. During the drying process, the interplay of crystallization and…

We consider the dynamic wetting and dewetting processes of films and droplets of complex liquids on planar surfaces, focusing on the case of colloidal suspensions, where the particle interactions can be sufficiently attractive to cause…

Fluid Dynamics · Physics 2024-11-20 J. Zhang , D. N. Sibley , D. Tseluiko , A. J. Archer

Dewetting of ultrathin (< 100 nm) polymer films, by heating above the glass transition, produces droplets of sizes of the order of microns and mean separations between droplets of the order of tens of microns. These relatively large length…

Soft Condensed Matter · Physics 2011-06-06 Ankur Verma , Ashutosh Sharma

We consider a two-dimensional sharp-interface model for solid-state dewetting of thin films with anisotropic surface energies on curved substrates, where the film/vapor interface and substrate surface are represented by an evolving and a…

Numerical Analysis · Mathematics 2024-10-02 Weizhu Bao , Yifei Li , Quan Zhao

The nucleation mechanisms during solution deposition of organic semiconductor thin films determine the grain morphology and may influence the crystalline packing in some cases. Here, in-situ optical spectromicroscopy in reflection mode is…

Materials Science · Physics 2016-08-02 Yang Li , Jing Wan , Detlef-M. Smilgies , Nicole Bouffard , Richard Sun , Randall L. Headrick

We propose a sharp interface model for simulating solid-state dewetting where the surface energy is (weakly) anisotropic. The morphology evolution of thin films is governed by surface diffusion and contact line migration. The mathematical…

Materials Science · Physics 2015-06-22 Yan Wang , Wei Jiang , Weizhu Bao , Dave J. Srolovitz

The crystal growth of isotactic polystyrene (it-PS) is investigated in very thin, 11 nm thick films. The it-PS crystals grown in the thin films show quite different morphology from that in the bulk. With decreasing crystallization…

Soft Condensed Matter · Physics 2016-08-31 Ken Taguch , Hideki Miyaji , Kunihide Izumi , Akitaka Hoshino , Yoshihisa Miyamoto , Ryohei Kokawa