Related papers: Clocking and controlling attosecond currents in a …
This perspective introduces attosecond path qubits: measurement-defined two-level subsystems that arise naturally in strong-field physics from the coherent interference of distinguishable quantum pathways. These effective qubits are…
We investigate quasi one-dimensional atomic chains on Si(553)-Au with a scanning tunneling microscope (STM). The observed periodicity at the Si step edge can be altered by the STM and depends on the magnitude of the tunneling current. In a…
Light as a carrier of information and energy plays a fundamental role in both general relativity and quantum physics, linking these areas that are still not fully compliant with each other. Its quantum nature and spatio-temporal structure…
The theory of inelastic electron tunneling spectroscopy (IETS) and motions of single adsorbed atoms and molecules on metal surfaces induced by vibrational excitation with a scanning tunneling microscope (STM) is reviewed. The theory of…
This paper presents results of numerical simulations of electron tunneling through water that extend our previous calculations on such systems in several ways. First, a tip-substrate configuration is used; second, calculations are carried…
Entanglement is one of the most intriguing aspects of quantum mechanics and lies at the heart of the ongoing Second Quantum Revolution, where it is a resource that is used in quantum key distribution, quantum computing and quantum…
In scanning tunneling microscopy (STM) experiments of molecules on insulating films, tunneling through molecular resonances implies transiently charging the molecule. The transition back to the charge ground state by tunneling through the…
Coupling phase-stable single-cycle terahertz (THz) pulses to scanning tunneling microscope (STM) junctions enables spatio-temporal imaging with femtosecond temporal and \r{A}ngstrom spatial resolution. The time resolution achieved in such…
Tunneling is one of the most bizarre phenomena in quantum mechanics. An attempt to understand it led to the next natural question of how long does a particle need to tunnel a barrier. The latter gave rise to several definitions such as the…
Electric control of individual atoms or molecules in a solid-state system offers a promising way to bring quantum mechanical functionalities into electronics. This idea has recently come into the reach of the established domain of silicon…
We develop a theoretical framework for probing superconductivity with momentum resolution using the quantum twisting microscope (QTM), a planar tunneling device where a graphene tip is rotated relative to a two-dimensional sample. Because…
The physical properties of ultrathin NaCl overlayers on the stepped Cu(311) surface have been characterized using scanning tunneling microscopy (STM) and spectroscopy, and density functional calculations. Simulations of STM images and…
Atomic motion dynamics during structural changes or chemical reactions have been visualized by picosecond and femtosecond pulsed electron beams via ultrafast electron diffraction and microscopy. Imaging the even faster dynamics of electrons…
Attosecond streaking is one of the most fundamental processes in attosecond science allowing for a mapping of temporal (i.e. phase) information on the energy domain. We show that on the single-particle level attosecond streaking time shifts…
This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…
We report on a fully nonequilibrium theory of the scanning tunneling microscopy (STM) through resonances induced by impurity atoms adsorbed on metal surfaces. The theory takes into account the effect of the tunneling current and finite bias…
Quantum mechanical tunneling of atoms is increasingly found to play an important role in many chemical transformations. Experimentally, atom-tunneling can be indirectly detected by temperature-independent rate constants at low temperature…
We introduce a novel control mode for Scanning Tunneling Microscopy (STM) that leverages di/dz feedback. By superimposing a high-frequency sinusoidal modulation on the control signal, we extract the amplitude of the resulting tunneling…
Recent experiments on measuring time-delays during tunnelling of cold atoms through an optically created potential barrier are reinvigorating the controversial debate regarding possible time-delays during light-induced tunnelling of an…
Attosecond science has demonstrated that electrons can be controlled on the sub-cycle time scale of an optical wave, paving the way toward optical frequency electronics. Using controlled few-cycle optical waveforms, the study of sub-cycle…