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X-ray photon correlation spectroscopy (XPCS) is a powerful tool for the investigation of dynamics covering a broad range of time and length scales. The two-time correlation function (TTC) is commonly used to track non-equilibrium dynamical…

Soft Condensed Matter · Physics 2024-06-19 Anastasia Ragulskaya , Vladimir Starostin , Fajun Zhang , Christian Gutt , Frank Schreiber

Long-term quantum coherence constitutes one of the main challenges when engineering quantum devices. However, easily accessible means to quantify complex decoherence mechanisms are not readily available, nor are sufficiently stable systems.…

Terahertz waves hold immense potential across diverse fields, including healthcare monitoring, biomedical imaging, precision navigation, high-speed communication, security screening, industrial quality control, and space exploration.…

Optics · Physics 2026-04-13 Yifan Zhao , Shahed-E- Zumrat , Szu-An Tsao , Mona Jarrahi

To manufacture faster electron devices, the industry has entered into the nanoscale dimensions and Terahertz (THz) working frequencies. The discrete nature of the few electrons present simultaneously in the active region of ultra-small…

Mesoscale and Nanoscale Physics · Physics 2024-02-13 Enrique Colomés , Javier Mateos , Tomás González , Xavier Oriols

Recent interest in developing fast spintronic devices and laser-controllable magnetic solids has sparked tremendous experimental and theoretical efforts to understand and manipulate ultrafast dynamics in materials. Studies of spin dynamics…

Optics · Physics 2022-09-21 Xinwei Li , Dasom Kim , Yincheng Liu , Junichiro Kono

Measuring fluctuations in matter's low energy excitations is the key to unveil the nature of the nonequilibrium response of materials. A promising outlook in this respect is offered by spectroscopic methods that address matter fluctuations…

Two-dimensional spectroscopy (2DS) is a powerful ultrafast technique for probing electronic and vibrational dynamics in complex microscopic systems. Extracting detailed information on system dynamics and system-bath interactions from 2DS…

Quantum Physics · Physics 2026-04-29 Yi-Xuan Yao , Hao-Yue Zhang , Cheng-Ge Liu , Rong-Hang Chen , Qing Ai , Franco Nori

Intense, single-cycle terahertz (THz) pulses offer a promising approach for understanding and controlling the properties of a material on an ultrafast time scale. In particular, resonantly exciting phonons leads to a better understanding of…

Strongly Correlated Electrons · Physics 2016-10-05 P. Bowlan , J. Bowlan , S. A. Trugman , R. Valdes Aguilar , J. Qi , X. Liu , J. Furdyna , M. Dobrowolska , A. J. Taylor , D. A. Yarotski , R. P. Prasankumar

Identifying signatures of quantum coherent behaviour in photoactive systems that are maintained in stationary states away from thermal equilibrium is an open problem of wide interest in a variety of physical scenarios, including single…

The third-order response lies at the heart of simulating and interpreting nonlinear spectroscopies ranging from two dimensional infrared (2D-IR) to 2D electronic (2D-ES), and 2D sum frequency generation (2D-SFG). The extra time and…

Chemical Physics · Physics 2022-09-21 Kenneth A. Jung , Thomas E. Markland

Decoherence remains one of the most serious challenges to the implementation of quantum technology. It appears as a result of the transformation over time of a quantum superposition state into a classical mixture due to the quantum system…

Optics · Physics 2021-07-28 Fu Li , Tian Li , Girish S. Agarwal

Terahertz time-domain spectroscopy (THz-TDS) has become a powerful tool for investigating the optical properties of thin films, offering direct access to the complex permittivity in the terahertz range. However, in transmission-based…

Non-equilibrium photon correlations of coherently excited single quantum systems can reveal their internal quantum dynamics and provide spectroscopic access. Here we propose and discuss the fundamentals of a coherent photon coincidence…

Quantum Physics · Physics 2020-11-04 Matthew Otten , Tristan Kenneweg , Matthias Hensen , Stephen K. Gray , Walter Pfeiffer

Quantum correlations are key information about the structures and dynamics of quantum many-body systems. There are many types of high-order quantum correlations with different time orderings, but only a few of them are accessible to the…

Quantum Physics · Physics 2022-06-14 Ze Wu , Ping Wang , Tianyun Wang , Yuchen Li , Ran Liu , Yuquan Chen , Xinhua Peng , Ren-Bao Liu , Jiangfeng Du

Quantum coherence is a fundamental characteristic to distinguish quantum systems from their classical counterparts. Though quantum coherence persists in isolated non-interacting systems, interactions inevitably lead to decoherence, which is…

Quantum Gases · Physics 2017-11-15 Ke-Ji Chen , Ho Kwan Lau , Hon Ming Chan , Dajun Wang , Qi Zhou

Optical two-dimensional coherent spectroscopy (2DCS) is a powerful ultrafast spectroscopic technique that can greatly benefit from the unique features of a femtosecond laser operating at a kHz repetition rate. However, isolating specific…

Optics · Physics 2024-08-08 Stephen Revesz , Rustam Gatamov , Adolfo Misiara , Hebin Li

Intense terahertz (THz) electromagnetic fields have been utilized to reveal a variety of extremely nonlinear optical effects in many materials through nonperturbative driving of elementary and collective excitations. However, such nonlinear…

High-dimensional quantum information processing has become a mature field of research with several different approaches being adopted for the encoding of $D$-dimensional quantum systems. Such progress has fueled the search of reliable…

Quantum Physics · Physics 2019-01-30 D. Martínez , M. A. Solís-Prosser , G. Cañas , O. Jiménez , A. Delgado , G. Lima

Parametric down-conversion (PDC) is the established standard for the practical generation of a multiplicity of quantum optical states. These include two-mode squeezed vacuum, heralded non-Gaussian states and entangled photon pairs. Detailed…

Quantum Physics · Physics 2014-06-18 Malte Avenhaus , Benjamin Brecht , Kaisa Laiho , Christine Silberhorn

Real-time measurement of the absolute frequency of continuous-wave terahertz (CW-THz) waves is required for characterization and frequency calibration of practical CW-THz sources. We proposed a method for real-time monitoring of the…