Related papers: Unlocking Quantum Control and Multi-Order Correlat…
We show that the nonlinear optical response probed by two-dimensional coherent spectroscopy (2DCS) can discriminate between excitonic and lattice driven order. In the excitonic regime of a realistic model of Ta$_2$NiSe$_5$, the third order…
The terahertz (THz) spectral domain offers a myriad of applications spanning chemical spectroscopy, medicine, security and imaging[1]. It has also recently become a playground for fundamental studies of light-matter interactions [2-6]. THz…
We present a method to measure quadratic Terahertz optical nonlinearities in Terahertz time-domain spectroscopy. We use a rotating linear polarizer (a polarizing chopper) to modulate the amplitude of the incident THz pulse train. We use a…
In this work, we consider Terahertz (THz) communications with low-resolution uniform quantization and spatial oversampling at the receiver side, corresponding to a single-input multiple-output (SIMO) transmission. We fairly compare…
Coherent multidimensional optical spectroscopy techniques are broadly applied across the electromagnetic spectrum ranging from NMR to the UV. These reveal properties of matter through correlation plots of signal fields generated in response…
Terahertz (THz) technology is critical for quantum material physics, biomedical imaging, ultrafast electronics, and next-generation wireless communications. However, standing in the way of widespread applications is the scarcity of…
The precision measurement of real-time electron temporal profiles is crucial for advancing electron and X-ray devices used in ultrafast imaging and spectroscopy. While high temporal resolution and large temporal window can be achieved…
We present a single-shot detection method of terahertz-correlated second harmonic generation in plasma-based sources by directly mixing an optical probe into femtosecond laser-induced plasma filaments in air. The single-shot second harmonic…
Slow data acquisition in terahertz time-domain spectroscopy (THz-TDS) has hindered the technique's ability to resolve "fast" dynamics occurring on the microsecond timescale. This timescale, arguably too slow to be accessed via standard…
Mode-resolved dual-comb spectroscopy (DCS) is an emerging spectroscopic tool with the potential to simultaneously achieve a broad spectral coverage and ultrahigh spectral resolution in terahertz (THz) spectroscopy. However, the need for two…
Terahertz (THz) nonlinear optics offer powerful tools to investigate and manipulate electronic dynamics in condensed matter. Confining high-peak-power THz pulses within near field can effectively generates extremely localized…
Advancements in quantum optics and squeezed light generation have transformed various domains of quantum science and technology. However, real-time quantum dynamics remain an underexplored frontier. Here, we extend quantum optics into the…
Long lived coherent quasiparticles are a promising foundation for novel quantum technologies, where maintaining quantum coherence is crucial. Decoherence, driven by finite emitter lifetimes, remains a central challenge in quantum computing.…
Hyperentangled photonic states - exhibiting nonclassical correlations in several degrees of freedom - offer improved performance of quantum optical communication and computation schemes. Experimentally, a hyperentanglement of…
Metastable phases present a promising route to expand the functionality of complex materials. Of particular interest are light-induced metastable phases that are inaccessible under equilibrium conditions, as they often host new, emergent…
Nonlinear processes can offer pathways to next-generation sensors and frequency mixing devices to overcome modern imaging, detection, and communication challenges. In this article, we report on strong second and third-order nonlinear…
Strong field driven electric currents in condensed matter systems open new frontiers in petahertz electronics. In this regime new challenges arise as the role of the band structure and the quantum nature of electron-hole dynamics have yet…
Since its first demonstration in 1995, terahertz time-domain imaging has attracted an increasingly growing interest for its ability to reveal spectral fingerprints of materials, probe changes in refractive index and absorption, as well as…
Recent experiments on cuprates have shown the possibility of opening a gap above the superconducting critical temperature, in the so-called phase-fluctuating state, by enhancing the phase coherence of preformed Cooper pairs. Quench-drive…
Two-dimensional electronic spectroscopy (2DES) can be implemented with different geometries, e.g., BOXCARS, collinear and pump-probe geometries. The pump-probe geometry has its advantage of overlapping only two beams and reducing phase…