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The electrostatic complexation between DOTAP-DOPC unilamellar liposomes and an oppositely charged polyelectrolyte (NaPA) has been investigated in a wide range of the liposome surface charge density. We systematically characterized the…

Soft Condensed Matter · Physics 2015-03-11 Simona Sennato , Laura Carlini , Domenico Truzzolillo , Federico Bordi

In the development of low cost, sustainable, and energy-dense batteries, chloride-based compounds are promising catholyte materials for solid-state batteries owing to their high Na-ion conductivities and oxidative stabilities. The ability…

Screening of a surface charge by electrolyte and the resulting interaction energy between charged objects is of fundamental importance in scenarios from bio-molecular interactions to energy storage. The conventional wisdom is that the…

Chemical Physics · Physics 2017-01-30 Alpha A. Lee , Carla Perez-Martinez , Alexander M. Smith , Susan Perkin

The study of Quantum Chromodynamics (QCD) at ultra-relativistic energies can be performed in a controlled environment through lepton-hadron deep inelastic scatterings. In such collisions, the high-energy partonic emissions that follow from…

High Energy Physics - Phenomenology · Physics 2025-01-23 Liliana Apolinário , Raghav Kunnawalkam Elayavalli , Nuno Olavo Madureira

The physical and chemical properties of metal nanoparticles differ significantly from those of free metal atoms as well as from the properties of bulk metals, and therefore, they may be viewed as a transition regime between the two physical…

Adaptation and Self-Organizing Systems · Physics 2007-05-23 Horacio G. Rotstein , Amy Novick-Cohen , Rina Tannenbaum

We scrutinize the effect of polyvalent ions on polymer-DNA interactions. We extend a recently developed test charge theory to the case of a stiff polymer interacting with a DNA molecule in an electrolyte mixture. The theory accounts for…

Soft Condensed Matter · Physics 2017-03-08 Sahin Buyukdagli

Monte Carlo simulations were employed to study two charged rods confined between two unlike charged plates, all immersed in a model electrolyte. Recently, it was shown that two rods immersed in a multivalent counterion solution may show…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 G. Odriozola , F. Jiménez-Ángeles , M. Lozada-Cassou

Interplay of Coulomb interaction energy, free ion entropy, and conformational elasticity is a fascinating aspect in polyelectrolytes (PEs). We develop a theory for complexation of two oppositely charged PEs, a process known to be the…

Soft Condensed Matter · Physics 2022-09-15 Soumik Mitra , Arindam Kundagrami

Ion concentration polarization (CP, current-induced concentration gradient adjacent to a charge-selective interface) has been well studied for single-phase mixed conductors (e.g., liquid electrolyte), but multiphase CP has been rarely…

Materials Science · Physics 2022-12-21 Huanhuan Tian , Ju Li , Martin Bazant

We study a model nanopore sensor with which a very low concentration of analyte molecules can be detected on the basis of the selective binding of the analyte molecules to the binding sites on the pore wall. The bound analyte ions partially…

Applied Physics · Physics 2018-01-17 Eszter Mádai , Mónika Valiskó , András Dallos , Dezső Boda

The adsorption of highly \textit{oppositely} charged flexible polyelectrolytes onto a charged spherical surface is investigated by means of Monte Carlo simulations in a fashion which resembles the layer-by-layer deposition technique…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina , Christian Holm , Kurt Kremer

The self-assembly of copolymeric vesicles and micelles in micromixers is studied by External Potential Dynamics (EPD) simulations -- a dynamic density functional approach that explicitly accounts for the polymer architecture both at the…

Soft Condensed Matter · Physics 2018-04-10 Simon Kessler , Klaus Drese , Friederike Schmid

We study the adsorption-desorption transition of polyelectrolyte chains onto planar, cylindrical and spherical surfaces with arbitrarily high surface charge densities by massive Monte Carlo computer simulations. We examine in detail how the…

Soft Condensed Matter · Physics 2016-10-05 Sidney J. de Carvalho , Ralf Metzler , Andrey G. Cherstvy

Charged colloidal monolayers at the interface between water and air (or oil) are used in a large number of chemical, physical and biological applications. Although a considerable experimental and theoretical effort has been devoted in the…

Soft Condensed Matter · Physics 2018-12-03 Aviv Karnieli , Tomer Markovich , David Andelman

It is well established that when multivalent counterions or salts are added to a solution of highly-charged polyelectrolytes (PEs), correlation effects can cause charge inversion of the PE, leading to electrophoretic mobility (EM) reversal.…

Soft Condensed Matter · Physics 2023-06-14 Hossein Vahid , Alberto Scacchi , Maria Sammalkorpi , Tapio Ala-Nissila

Polyelectrolyte (PE) hydrogels can dynamically respond to external stimuli, such as changes in pH and temperature, which benefits their use for smart materials and nanodevices with tunable properties. We investigate equilibrium…

Soft Condensed Matter · Physics 2026-04-07 Jiaxing Yuan , Tine Curk

The rapid charging and/or discharging of electrochemical cells can lead to localized depletion of electrolyte concentration. This depletion can significantly impact the system's time dependent resistance. For systems with porous electrodes,…

Chemical Physics · Physics 2017-12-27 James W. Palko , Ali Hemmatifar , Juan G. Santiago

Introducing nanorods into a polymeric matrix can enhance the physical and mechanical properties of the resulting material. In this paper, we focus on understanding the dispersion and orientation patterns of nanorods in an unentangled…

Soft Condensed Matter · Physics 2023-04-05 Navid Afrasiabian , Venkat Balasubramanian , Colin Denniston

Nanomaterial surface states can effectively modify or even dominate their physical and chemical properties due to large surface-to-volume ratios. Such surface effects are highly dependent on particle size and ligand coverage, yet the…

Materials Science · Physics 2020-07-17 Guolei Xiang , Yan Tang , Zigeng Liu , Wei Zhu , Haitao Liu , Jiaou Wang , Guiming Zhong , Jun Li , Xun Wang

Recent measurements suggest the possibility to exploit ionic liquids (ILs) as smart lubricants for nano-contacts, tuning their tribological and rheological properties by charging the sliding interfaces. Following our earlier theoretical…

Materials Science · Physics 2015-10-28 Rosario Capozza , Andrea Benassi , Andrea Vanossi , Erio Tosatti
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