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We develop the machine learning capability to predict a time sequence of in-situ transmission electron microscopy (TEM) video frames based on the combined long-short-term-memory (LSTM) algorithm and the features de-entanglement method. We…

Materials Science · Physics 2022-05-24 Wenkai Fu , Steven R. Spurgeon , Chongmin Wang , Yuyan Shao , Wei Wang , Amra Peles

Over three decades of reverberation mapping (RM) studies on local broad-line active galactic nuclei (AGNs) have measured reliable black-hole (BH) masses for $> 100$ AGNs. These RM measurements reveal a significant correlation between the…

Theoretical description of oscillations of electron liquid in large metallic nanospheres (with radius of few tens nm) is formulated within random-phase-approximation semiclassical scheme. Spectrum of plasmons is determined including both…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 W. Jacak , J. Krasnyj , J. Jacak , R. Gonczarek , A. Chepok , L. Jacak , D. Z. Hu , D. Schaadt

We study the distance dependence of the rate of electronic excitation energy transfer from a dye molecule to a metal nanoparticle. Using the spherical jellium model, we evaluate the rates corresponding to the excitation of l = 1, 2, and 3…

Chemical Physics · Physics 2009-11-13 R. S. Swathi , K. L. Sebastian

Using benzene sandwiched between two Au leads as a model system, we investigate from first principles the change in molecular conductance caused by different atomic structures around the metal-molecule contact. Our motivation is the…

Materials Science · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

We study the metallicities and abundance ratios of early-type galaxies in cosmological semi-analytic models (SAMs) within the hierarchical galaxy formation paradigm. To achieve this we implemented a detailed galactic chemical evolution…

Cosmology and Nongalactic Astrophysics · Physics 2015-05-13 Matías Arrigoni , Scott C. Trager , Rachel S. Somerville , Brad K. Gibson

Starting from first principles, we theoretically model the nonlinear temporal dynamics of gold-based plasmonic devices resulting from the heating of their metallic components. At optical frequencies, the gold susceptibility is determined by…

Noble-metal nanoparticles for photocatalysis have become a major research object in recent years due to their plasmon-enhanced strong light-matter interaction. The dynamics of the hot electrons in the noble metal are crucial for the…

The combination of nanodiamonds with plasmonic metal particles is being explored for synergic effects that can enhance biosensing and antibacterial treatments, energy harvesting, photocatalysis, and quantum centres. Here we systematically…

The origin of the anomalously compliant behavior of nanoporous gold is studied by comparing the elasticity obtained from molecular dynamics (MD) and finite element method (FEM) simulations. Both models yield a compliance, which is much…

Materials Science · Physics 2016-11-29 B. -N. D. Ngô , B. Roschning , K. Albe , J. Weissmüller , J. Markmann

We demonstrated a biosensing approach which, for the first time, combines the high-sensitivity of whispering gallery modes (WGM) with a metallic nanoparticle based assay. We provided a computational model based on generalized Mie theory to…

Gold (Au) nanoparticles particularly nanorods are actively exploited as imaging probes because of their special nonblinking and nonbleaching absorption, scattering and emitting properties that arise from the excitation of surface plasmons.…

Optics · Physics 2011-09-30 Tao Li , Qiang Li , Xiao-Jun Chen , Yi Xu , Qiaofeng Dai , Hai-Ying Liu , Sheng Lan , Li-Jun Wu

We present a modeling of the nonlinear optical response of a metal surface in order to account for recent experimental results from two-color Sum-Frequency Generation experiments on gold. The model allows calculating the surface and bulk…

Chemical Physics · Physics 2019-05-16 Bertrand Busson , Laetitia Dalstein

We develop and evaluate point and interval estimates for the random effects $\theta_i$, having made observations $y_i|\theta_i\stackrel{\m athit{ind}}{\sim}N[\theta_i,V_i],i=1,...,k$ that follow a two-level Normal hierarchical model.…

Methodology · Statistics 2011-08-17 Carl Morris , Ruoxi Tang

Large reflection losses at interfaces in light emitting semiconductor devices cause a significant reduction in their light emission and energy efficiencies. Metal nanoparticle (NP) surface coatings have been demonstrated to increase the…

Plasmonic devices, fundamental to modern nanophotonics, exploit resonant interactions between light and free electrons in metals to achieve enhanced light trapping and electromagnetic field confinement. However, modeling their complex,…

Computational Engineering, Finance, and Science · Computer Science 2025-08-07 Emmanuel A. Bamidele

This paper provides new insights concerning the simulation of plasmon driven chemical reactions using real-time TDDFT based on the tight-binding electronic structure code DFTB+, with applications to the dissociation of H$_2$ on octahedral…

Chemical Physics · Physics 2023-03-21 Sajal Kumar Giri , George C. Schatz

Electrical resistivity in good metals, particularly noble metals such as gold (Au), silver (Ag), or copper, increases linearly with temperature ($T$) for $T > \Theta_{\mathrm{D}}$, where $\Theta_{\mathrm{D}}$ is the Debye temperature. This…

Passive and active targets, implanted with gold nanoprisms, were designed to achieve enhanced and uniform power absorption during two-sided illumination by short laser pulses. The target length was adjusted to match the short laser…

In this work we study the strong confinement effects on the electromagnetic response of metallic nanoparticles. We calculate the field enhancement factor for nanospheres of various radii by using optical constants obtained from both…

Mesoscale and Nanoscale Physics · Physics 2018-02-20 Mario Zapata-Herrera , Jefferson Flórez , Angela Camacho , Hanz Y. Ramirez