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Related papers: $^{229}$Th Nuclear Spectroscopy in an Opaque Mater…

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$^{229}$Th is the only nucleus currently under investigation for the development of a nuclear optical clock (NOC) of ultra-high accuracy. The insufficient knowledge of the first nuclear excitation energy of $^{229}$Th has so far hindered…

M\"ossbauer spectroscopy is widely used in biochemistry, geology, and solid-state physics to obtain structural information on materials. Here, we extend this technique into the optical range using a vacuum ultraviolet laser to probe the…

The results of experimental studies of the low-energy isomeric state in the $^{229}$Th nucleus are presented. The work is consisted of several stages. During the first stage $^{229}$Th nuclei were excited with the inverse internal…

After nearly fifty years of searching, the vacuum ultraviolet $^{229}$Th nuclear isomeric transition has recently been directly laser excited [1,2] and measured with high spectroscopic precision [3]. Nuclear clocks based on this transition…

The first excited isomeric state of Th-229 has an exceptionally low energy of only a few eV and could form the gateway to high-precision laser spectroscopy of nuclei. The excitation energy of the isomeric state has been inferred from…

The isotope $^{229}$Th is the only nucleus known to possess an excited state $^{229m}$Th in the energy range of a few electron volts, a transition energy typical for electrons in the valence shell of atoms, but about four orders of…

The process of internal conversion from excited electronic states is investigated theoretically for the case of the vacuum-ultraviolet nuclear transition of $^{229}{\mathrm Th}$. Due to the very low transition energy, the $^{229}{\mathrm…

Atomic Physics · Physics 2017-03-22 Pavlo V. Bilous , Georgy A. Kazakov , Iain D. Moore , Thorsten Schumm , Adriana Pálffy

A new concept for narrow-band direct nuclear laser spectroscopy of $^{229\text{m}}$Th is proposed, using a single comb mode of a vacuum ultraviolet frequency comb generated from the 7th harmonic of an Yb-doped fiber laser system. In this…

Instrumentation and Detectors · Physics 2020-07-09 Lars von der Wense , Chuankun Zhang

$^{229}$Th, a crucial candidate for nuclear clocks and many other applications, is a typical heavy nucleus with an extremely low-energy isomeric state $^{229m}$Th. A detailed study of the nuclear structure of $^{229}$Th is performed here by…

Nuclear Theory · Physics 2025-08-28 Zi-Rui Chen , Long-Jun Wang , Yuanbin Wu

For the isotope $^{229}$Th we investigate the possibility of two-photon laser spectroscopy of the nuclear clock transition (148.38 nm) using intense monochromatic laser field at twice the wavelength (296.76 nm). Our estimates show that due…

The proposal for the development of a nuclear optical clock has triggered a multitude of experimental and theoretical studies. In particular the prediction of an unprecedented systematic frequency uncertainty of about $10^{-19}$ has…

Atomic Physics · Physics 2020-11-10 Lars von der Wense , Benedict Seiferle

The low-lying isomeric state of $^{229}$Th provides unique opportunities for high-resolution laser spectroscopy of the atomic nucleus. We determine the energy of this isomeric state by taking the absolute energy difference between the…

A low-energy nuclear transition in the isotope thorium-229 has been excited in thorium-doped crystals with laser light. This opens the perspective towards a highly stable and robust solid-state optical nuclear clock. The required laser…

The 7.6-eV-isomer of Thorium-229 offers the opportunity to perform high resolution laser spectroscopy of a nuclear transition. We give a brief review of the investigations of this isomer. The nuclear resonance connecting ground state and…

Optics · Physics 2017-08-23 E. Peik , K. Zimmermann , M. Okhapkin , Chr. Tamm

We describe a novel approach to directly measure the energy of the narrow, low-lying isomeric state in $^{229}$Th. Since nuclear transitions are far less sensitive to environmental conditions than atomic transitions, we argue that the…

Atomic Physics · Physics 2010-02-09 Wade G. Rellergert , D. DeMille , R. R. Greco , M. P. Hehlen , J. R. Torgerson , Eric R. Hudson

Today's most precise time and frequency measurements are performed with optical atomic clocks. However, it has been proposed that they could potentially be outperformed by a nuclear clock, which employs a nuclear transition instead of the…

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

Nuclear Experiment · Physics 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

Thorium-229 is a unique case in nuclear physics: it presents a metastable first excited state Th-229m, just a few electronvolts above the nuclear ground state. This so-called isomer is accessible by VUV lasers, which allows transferring the…

LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that…

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