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We study many-body correlations in the ground states of a general quantum system of bosons or fermions by including an additional Jastrow function in our ecently proposed variational coupled-cluster method. Our approach combines the…

Strongly Correlated Electrons · Physics 2009-11-13 Y. Xian

We present an implementation and benchmark of new approximations in multireference algebraic diagrammatic construction theory for simulations of neutral electronic excitations and UV/Vis spectra of strongly correlated molecular systems…

Chemical Physics · Physics 2021-12-02 Ilia M. Mazin , Alexander Yu. Sokolov

Among many current data processing systems, the objectives are often not the reproduction of data, but to compute some answers based on the data resulting from queries. The similarity identification task is to identify the items in a…

Signal Processing · Electrical Eng. & Systems 2020-01-23 Hanwei Wu , Qiwen Wang , Markus Flierl

In this work, we present a brief overview of the fermionic mode optimization within the framework of tensor network state methods [PRL 117,210402(2016)], and demonstrate that it has the potential to compress the multireference character of…

Chemical Physics · Physics 2022-04-29 Mihály Máté , Klára Petrov , Szilárd Szalay , Örs Legeza

Benefited from the advances of deep learning (DL) techniques, deep joint source-channel coding (JSCC) has shown its great potential to improve the performance of wireless transmission. However, most of the existing works focus on the…

Information Theory · Computer Science 2022-11-22 Kaiyi Chi , Qianqian Yang , Zhaohui Yang , Yiping Duan , Zhaoyang Zhang

In a recent paper, we proposed the adaptive shift method for correcting the undersampling bias of the initiator-FCIQMC. The method allows faster convergence with the number of walkers to the FCI limit than the normal initiator method,…

Computational Physics · Physics 2021-02-03 Khaldoon Ghanem , Kai Guther , Ali Alavi

In multi-core quantum computing architectures, waveguide-mediated interconnects are essential for facilitating fast, high-fidelity quantum state transfer between qubits located in different chips. However, optimizing these systems typically…

A method is presented for calculating binding energies and other properties of extended interacting systems using the projected density of transitions (PDoT) which is the probability distribution for transitions of different energies…

Strongly Correlated Electrons · Physics 2009-10-31 Roger Haydock

We introduce a multireference selected quantum Krylov (MRSQK) algorithm suitable for quantum simulation of many-body problems. MRSQK is a low-cost alternative to the quantum phase estimation algorithm that generates a target state as a…

Chemical Physics · Physics 2019-11-14 Nicholas H. Stair , Renke Huang , Francesco A. Evangelista

A method is suggested to build simple multiconfigurational wave functions specified uniquely by an energy cutoff $\Lambda$. These are constructed from a model space containing determinants with energy relative to that of the most stable…

Chemical Physics · Physics 2015-06-19 Francesco A. Evangelista

We review a recent approach for the simulation of many-body interacting systems based on an efficient generalization of the Lanczos method for Quantum Monte Carlo simulations. This technique allows to perform systematic corrections to a…

Strongly Correlated Electrons · Physics 2007-05-23 Sandro Sorella

Cross-correlated contrast source inversion (CC-CSI) is a non-linear iterative inversion method that is proposed recently for solving the inverse scattering problems. In CC-CSI, a cross-correlated error is constructed and introduced to the…

Signal Processing · Electrical Eng. & Systems 2019-06-27 Shilong Sun , Bert Jan Kooij , Alexander G. Yarovoy

The multi-configuration Dirac-Hartree-Fock method was employed to calculate the total and excitation energies, oscillator strengths and hyperfine structure constants for low-lying levels of Sm I. In the first-order perturbation…

Atomic Physics · Physics 2015-09-16 Fuyang Zhou , Yizhi Qu , Jiguang Li , Jianguo Wang

We investigate the existence of holomorphic Hartree-Fock solutions using a revised SCF algorithm. We use this algorithm to study the Hartree-Fock solutions for H$_{2}$ and H$_{4}^{2+}$ and report the emergence of holomorphic solutions at…

Chemical Physics · Physics 2015-11-20 Hugh G. A. Burton , Alex J. W. Thom

In this work, we investigate the fidelity of orbital optimization in variational Monte Carlo to improve diffusion Monte Carlo results on correlated magnetic systems, using CrSBr as a model system. We compare the performance of different…

Strongly Correlated Electrons · Physics 2026-04-27 Cody A. Melton , Jaron T. Krogel

We present an efficient implementation of a one-step relativistic second-order multireference perturbation theory based on the multireference driven similarity renormalization group (MR-DSRG) using the exact two-component (X2C) Hamiltonian,…

Chemical Physics · Physics 2026-05-13 Zijun Zhao , Francesco A. Evangelista

In this work, we investigate the possibility of improving multireference-driven coupled cluster (CC) approaches with an algorithm that iteratively combines complete active space (CAS) calculations with tailored CC and externally corrected…

Chemical Physics · Physics 2025-03-06 Robin Feldmann , Max Mörchen , Jakub Lang , Michał Lesiuk , Markus Reiher

Calculations of the binding energy of the transition metal oxide molecules TiO and MnO are presented, using a recently developed phaseless auxiliary field quantum Monte Carlo approach. This method maps the interacting many-body problem onto…

Strongly Correlated Electrons · Physics 2007-05-23 W. A. Al-Saidi , Henry Krakauer , Shiwei Zhang

We use the multiconfiguration Dirac-Hartree-Fock (MCDHF) method combined with the relativistic configuration interaction (RCI) approach (GRASP2K) to provide a consistent set of transition energies and radiative transition data for the lower…

Atomic Physics · Physics 2020-01-08 K. Wang , P. Jönsson , G. Del Zanna , M. Godefroid , Z. B. Chen , C. Y. Chen , J. Yan

Direct sampling from a Slater determinant is combined with an autoregressive deep neural network as a Jastrow factor into a fully autoregressive Slater-Jastrow ansatz for variational quantum Monte Carlo, which allows for uncorrelated…

Strongly Correlated Electrons · Physics 2023-06-22 Stephan Humeniuk , Yuan Wan , Lei Wang
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