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Well-ordered ultrathin films of NiO have been prepared on an Ag(001) substrate using molecular beam epitaxy. With the help of angle-resolved two-photon photoemission (2PPE) a series of image potential states (IPS) for film thicknesses of…

Materials Science · Physics 2018-02-21 K. Gillmeister , M. Kiel , W. Widdra

The transport of optically excited, hot electrons in heterostructures is analyzed by femtosecond, time-resolved two-photon photoelectron emission spectroscopy (2PPE) for epitaxial Au/Fe/MgO(001). We compare the temporal evolution of the…

Strong electron correlations in perovskite oxides give rise to rich and often unexpected electronic phenomena. In this study, we present a comprehensive surface-science investigation of epitaxial thin films of the charge-transfer insulator…

Materials Science · Physics 2025-06-02 Friederike Elisa Wührl , Antonia Rieche , Anne Oelschläger , Kathrin Dörr , Wolf Widdra

Employing femtosecond laser pulses in front and back side pumping of Au/Fe/MgO(001) combined with detection in two-photon photoelectron emission spectroscopy we analyze local relaxation dynamics of excited electrons in buried Fe, injection…

Mesoscale and Nanoscale Physics · Physics 2020-08-17 Yasin Beyazit , Jan Beckord , Ping Zhou , Jan Meyburg , Detlef Diesing , Manuel Ligges , Uwe Bovensiepen

We present angle resolved photoemission spectra for Ag(111) and Au(111) single crystals in normal emission geometry, taken at closely spaced intervals for photon energies between 8 eV and 160 eV. The most dominant transitions observed are…

Materials Science · Physics 2018-06-27 Friedrich Roth , Tiberiu Arion , Hendrik Kaser , Alexander Gottwald , Wolfgang Eberhardt

Silver films were deposited at room temperature onto H-passivated Si(111) surfaces. Their electronic properties have been analyzed by angle-resolved photoelectron spectroscopy. Submonolayer films were semiconducting and the onset of…

Materials Science · Physics 2009-11-07 A. Arranz , J. F. Sanchez-Royo , J. Avila , V. Perez-Dieste , P. Dumas , M. C. Asensio

We have studied the dynamics of electrons in single wall carbon nanotubes using femtosecond time-resolved photoemission. The lifetime of electrons excited to the pi* bands is found to decrease continuously from 130 fs at 0.2 eV down to less…

Materials Science · Physics 2009-10-31 Tobias Hertel , Gunnar Moos

We have studied the relaxation dynamics of optically excited electrons in molybdenum and rhodium by means of time resolved two-photon photoemission spectroscopy (TR-2PPE) and ab initio electron self-energy calculations performed within the…

Other Condensed Matter · Physics 2016-08-16 A. Mönnich , J. Lange , M. Bauer , M. Aeschlimann , I. A. Nechaev , V. P. Zhukov , P. M. Echenique , E. V. Chulkov

Rare-earth-ferrimagnetic oxides are emerging as attractive platforms for investigating ultrafast spin dynamics. Here, we study the photoinduced magnetization dynamics of epitaxial NiCo2O4 (NCO) thin films by time-resolved magneto-optical…

Employing time-resolved photoelectron spectroscopy we analyze the relaxation dynamics of hot electrons in the charge density wave / Mott material 1T-TaS_2. At 1.2 eV above the Fermi level we observe a hot electron lifetime of 12 +- 5 fs in…

Strongly Correlated Electrons · Physics 2020-07-01 Isabella Avigo , Friedemann Queisser , Ping Zhou , Manuel Ligges , Kai Rossnagel , Ralf Schützhold , Uwe Bovensiepen

In a high-resolution photoemission study of a Mo(110) surface state various contributions to the measured width and energy of the quasiparticle peak are investigated. Electron-phonon coupling, electron-electron interactions and scattering…

Strongly Correlated Electrons · Physics 2007-05-23 T. Valla , A. V. Fedorov , P. D. Johnson , S. L. Hulbert

In time-resolved photoemission experiments, more than one electron can be emitted from the solid by a single ultra-short pulse. We theoretically demonstrate how correlations between the momenta of outgoing electrons relate to time-dependent…

Strongly Correlated Electrons · Physics 2019-06-26 Christopher Stahl , Martin Eckstein

The two-carrier transport model as proposed for the two-dimensional electron gas formed at the interfaces of oxide heterostructures is investigated by means of a combined perturbation of near ultra-violet radiation and electrostatic field,…

Strongly Correlated Electrons · Physics 2012-08-21 A. Rastogi , J. J. Pulikkotil , S. Auluck , Z. Hossain , R. C. Budhani

In condensed matter, scattering processes determine the transport of charge carriers. In case of heterostructures, interfaces determine many dynamic properties like charge transfer and transport and spin current dynamics. Here we discuss…

Electrons in image-potential states on the surface of bulk helium represent a unique model system of a two-dimensional electron gas. Here, we investigate their properties in the extreme case of reduced film thickness: a monolayer of helium…

Mesoscale and Nanoscale Physics · Physics 2016-06-23 Nico Armbrust , Jens Güdde , Ulrich Höfer , Sarah Kossler , Peter Feulner

Concerning with the recent experiment of time-resolved two-photon photo-emission spectral measurements on semiconductors (GaAs, InP), we theoretically study real time relaxation dynamics of macroscopically photo-excited electrons, toward…

Mesoscale and Nanoscale Physics · Physics 2015-03-05 Hiromasa Ohnishi , Norikazu Tomita , Keiichiro Nasu

We used femtosecond optical pump-probe spectroscopy to study the photoinduced change in reflectivity of thin films of the electron-doped cuprate La$_{2-x}$Ce$_x$CuO$_4$ (LCCO) with dopings of x$=$0.08 (underdoped) and x$=$0.11 (optimally…

Superconductivity · Physics 2017-03-16 I. M. Vishik , F. Mahmood , Z. Alpichshev , J. Higgins , R. L. Greene , N. Gedik

The time of life of fermionic quasiparticles, the distribution of which in the momentum-energy space can be measured by angle resolved photoemission (ARPES), is the first quantity to look for fingerprints of interaction responsible for the…

The magnetic properties of Zn$_{1-x}$Co$_x$O ($x=0.07$ and 0.10) thin films, which were homo-epitaxially grown on a ZnO(0001) substrates with varying relatively high oxygen pressure, have been investigated using x-ray magnetic circular…

We report a first-principles description of inelastic lifetimes of excited electrons in real Cu and Al, which we compute, within the GW approximation of many-body theory, from the knowledge of the self-energy of the excited quasiparticle.…

Materials Science · Physics 2009-10-31 I. Campillo , J. M. Pitarke , A. Rubio , E. Zarate , P. M. Echenique
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