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We investigate the attosecond transient absorption spectroscopy (ATAS) in gapped graphene by numerically solving the four-band density matrix equations. Our results reveal that, in contrast to pristine graphene, whose fishbone-shaped…

Mesoscale and Nanoscale Physics · Physics 2025-06-30 Jiayu Yan , Hongxuan Er , Wei Dang , Jiahuan Ren , Chao Chen , Dianxiang Ren , Fulong Dong

We investigate the attosecond transient absorption spectroscopy (ATAS) of graphene by numerically solving four-band density-matrix equations, which demonstrates apparent fish bone resonance structures. To gain insight into these interesting…

Mesoscale and Nanoscale Physics · Physics 2023-01-04 Fulong Dong , Jie Liu

We extend the first-principles analysis of attosecond transient absorption spectroscopy to two-dimensional materials. As an example of two-dimensional materials, we apply the analysis to monolayer hexagonal boron nitride (h-BN) and compute…

Materials Science · Physics 2019-07-19 Shunsuke A. Sato , Hannes Hübener , Umberto De Giovannini , Angel Rubio

Attosecond transient-absorption spectroscopy (ATAS) is an established method for exploring electron dynamics on the subfemtosecond time-scale. ATAS spectra contain certain ubiquitous features, such as oscillating fringes, light-induced…

Atomic Physics · Physics 2017-08-02 Jørgen Johansen Rørstad , Jens E. Bækhøj , Lars Bojer Madsen

Attosecond transient absorption spectroscopy (ATAS) has emerged as a powerful technique within the field of attosecond science, combining extremely high temporal and excellent spectral resolution. So far, ATAS has been implemented in…

Probing vibronic coherence in molecules has been a central topic in ultrafast science, as it is an essential prerequisite to monitoring electronic motion. While experiments have demonstrated that attosecond transient absorption spectroscopy…

Atomic Physics · Physics 2023-08-02 C. H. Yuen , C. D. Lin

We apply attosecond transient absorption spectroscopy (ATAS) to explore the effects of a nonzero permanent dipole on electron dynamics at the subfemtosecond scale, exemplified in the polar LiF molecule. In contrast with nonpolar systems, a…

Atomic Physics · Physics 2018-11-14 Jørgen Johansen Rørstad , Nikolaj S. W. Ravn , Lun Yue , Lars Bojer Madsen

We perform the first-principles many-body GW and Bethe-Salpeter equation (BSE) calculations on the two-dimensional hexagonal boron nitride (2D-hBN) to explore the effects of opposite atoms on the electronic structure and linear one-photon…

Materials Science · Physics 2023-01-04 You-Zhao Lan

Hexagonal boron nitride ($\it h$-BN) exhibits dominant $\pi$-bands near the Fermi level, similar to graphene. However, unlike graphene, where tight-binding (TB) models accurately reproduce band edges near the $K$ and $K^{\prime}$ points in…

Materials Science · Physics 2024-09-04 Srivani Javvaji , Fengping Li , Jeil Jung

A theoretical study of the exciton binding energy in the two-dimensional hexagonal boron nitride monolayer is presented within the tight-binding approximation (TBA). A self-consistent equation for the interband electron-hole propagators is…

Materials Science · Physics 2018-03-28 Zoran Rukelj , Vito Despoja

Tracing ultrafast processes induced by interaction of light with matter is often very challenging. In molecular systems, the initially created electronic coherence becomes damped by the slow nuclear rearrangement on a femtosecond timescale…

Chemical Physics · Physics 2021-09-20 Nikolay V. Golubev , Jiří Vaníček , Alexander I. Kuleff

Attosecond transient absorption spectroscopy (ATAS) is becoming an indispensable and powerful tool in the emerging field of attochemistry, while the interpretation of measurements often requires full considerations of the coupling among…

Group theory and density functional theory methods are combined to obtain compact and accurate $k\cdot p$ Hamiltonians that describe the bandstructures around the $K$ and $\Gamma$ points for the 2D material hexagonal boron arsenide (h-BAs)…

Mesoscale and Nanoscale Physics · Physics 2019-05-28 Mathias Rosdahl Brems , Morten Willatzen

Being a flexible wide band gap semiconductor, hexagonal boron nitride (h-BN) has great potential for technological applications like efficient deep ultraviolet light sources, building block for two-dimensional heterostructures and room…

BAs is III-V semiconductor with ultra-high thermal conductivity, but many of its electronic properties are unknown. This work applies predictive atomistic calculations to investigate the properties of BAs heterostructures, such as strain…

Materials Science · Physics 2019-09-05 Kyle Bushick , Sieun Chae , Zihao Deng , John Heron , Emmanouil Kioupakis

Monolayer of hexagonal boron nitride (h-BN), commonly known as "white graphene" is a promising wide bandgap semiconducting material for deep-ultaviolet optoelectronic devices. In this report, the light absorption of a single layer hexagonal…

Mesoscale and Nanoscale Physics · Physics 2011-09-26 Aniruddha Konar , Raj Jana , Tian Fang , Guowang Li , William O'Brien , Debdeep Jena

Atomically thin hexagonal boron nitride (h-BN), especially monolayer, has garnered increasing attention due to its intriguing optical and light-matter-interaction properties. However, its intrinsic optical properties and electronic band…

We investigate the ultrafast electron dynamics of a model of a wide-bandgap material with inner, valence, and conduction bands excited by an intense few-femtosecond pump and monitored by a delayed attosecond extreme-ultraviolet probe pulse.…

Optics · Physics 2026-05-08 Stefano M. Cavaletto , Lars Bojer Madsen

The mechanism underlying high harmonic generation (HHG) in gases has been well clarified, characterizing attosecond pulse trains (APT) in the time domain, significantly advances the synthesis of isolated attosecond pulse (IAP). However, the…

Optics · Physics 2025-07-25 Qing-Guo Fan , Kang Lai , Wen-hao Liu , Zhi Wang , Lin-Wang Wang , Jun-Wei Luo

Hexagonal boron nitride (hBN) has emerged as a promising two-dimensional (2D) material for many applications in photonics. Although its linear and nonlinear optical properties have been extensively studied, its interaction with…

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