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In this paper we make a detailed study of the role of coherent tunneling, on the photocurrent and power delivered by a quantum dot molecule (QDM) in the presence of solar light. We focus our analysis on the coherence driven by tunneling and…

Quantum Physics · Physics 2022-07-15 J. Lira , J. M. Villas-Boas , L. Sanz , A. M. Alcalde

Artificially reproducing the biological light reactions responsible for the remarkably efficient photon-to-charge conversion in photosynthetic complexes represents a new direction for the future development of photovoltaic devices. Here, we…

Quantum Physics · Physics 2013-12-25 C. Creatore , M. A. Parker , S. Emmott , A. W. Chin

The high quantum efficiency of photosynthetic complexes has inspired researchers to explore new routes to utilize this process for photovoltaic devices. Quantum coherence has been demonstrated to play a crucial role within this process.…

Chemical Physics · Physics 2015-06-23 Yiteng Zhang , Sangchul Oh , Fahhad H. Alharbi , Greg Engel , Sabre Kais

It is thought that nature already exploits quantum mechanical properties to increase the efficiency of solar energy harvesting devices. So, the operation of these devices can be enhanced by clever design of a nanoscopic, quantum mechanical…

Mesoscale and Nanoscale Physics · Physics 2024-07-17 Baharak Mohamad Jafari Navadel , Esfandyar Faizi , Baharam Ahansaz , Jaber Jahanbin Sardroodi

We study how much the efficiency of a solar cell as a quantum heat engine could be enhanced by quantum coherence. In contrast to the conventional approach that a quantum heat engine is in thermal equilibrium with both hot and cold…

Quantum Physics · Physics 2020-05-28 Sangchul Oh

In this work, we propose an efficient quantum-enhanced solid-state photocell based on GaN quantum dots. We exploit the strong built-in electric field in GaN QDs and excitonic dipole-dipole coupling between adjacent QDs to break detailed…

Solar cells employing quantum wells can enhance the light absorption but suffer from the difficulty in photogenerated carrier extraction. Here, we analyzed the spectral response and the photocarrier collection mechanism of p-i-n multiple…

Applied Physics · Physics 2020-06-02 Kasidit Toprasertpong , Tomoyuki Inoue , Yoshiaki Nakano , Masakazu Sugiyama

For efficient photovoltaic conversion, it is important to understand how quantum entropy-related quantities evolve during the photovoltaic process. In this study, using a double quantum dot (DQD) photocell model, we explored the dynamic…

Mesoscale and Nanoscale Physics · Physics 2024-02-13 Lin-Jie Chen , Shun-Cai Zhao , Ya-Fang Tian

In this work, it is investigated the behavior of the efficiency at maximum power of a quantum dot molecule, acting as a device for photovoltaic conversion. A theoretical approach using a master equation, considering the effect of the energy…

Mesoscale and Nanoscale Physics · Physics 2022-05-16 J. Lira , L. Sanz , A. M. Alcalde

Understanding the carrier excitation and transport processes at the single-charge level plays a key role in quantum-dot-based solar cells and photodetectors. Here, we report on Coulomb-induced giant photocurrent enhancement of positive…

Mesoscale and Nanoscale Physics · Physics 2019-02-13 Kai Peng , Shiyao Wu , Xin Xie , Jingnan Yang , Chenjiang Qian , Feilong Song , Sibai Sun , Jianchen Dang , Yang Yu , Shushu Shi , Jiongji He , Xiulai Xu

We show that quantum coherence can increase the quantum efficiency of various thermodynamic systems. For example, we can enhance the quantum efficiency for a quantum dot photocell, a laser based solar cell and the photo-Carnot quantum heat…

Quantum Physics · Physics 2011-02-03 Kimberly Chapin , Konstantin Dorfman , Anatoly Svidzinsky , Marlan Scully

We investigate the quantum thermodynamics of two quantum systems, a two-level system and a four-level quantum photocell, each driven by photon pulses as a quantum heat engine. We set these systems to be in thermal contact only with a cold…

Quantum Physics · Physics 2020-07-15 Sangchul Oh , Jungjun Park , Hyunchul Nha

To absorb the photons below the band-gap energy effectively, we proposed a quantum dot (QD) photocell modeled by multi-level system for the quantum yields and photo-to-charge efficiency limits. The theoretical results show the quantum…

Mesoscale and Nanoscale Physics · Physics 2024-02-26 Shun-Cai Zhao , Jing-Yi Chen

Nowadays, harmful effects of climate change are becoming increasingly apparent. A vital issue that must be addressed is the generation of energy from non-renewable and often polluting sources. For this reason, the development of renewable…

Computational Engineering, Finance, and Science · Computer Science 2025-01-03 Tomasz Weron

Motivated by recent experiments on the generation of coherent light in engineered hybrid quantum systems, we investigate gain in a microwave photonic cavity coupled to quantum dot structures, and develop concrete directions for achieving a…

Quantum Physics · Physics 2017-12-25 Bijay Kumar Agarwalla , Manas Kulkarni , Shaul Mukamel , Dvira Segal

Obtaining the physical mechanism of photoelectric transfer in quantum-dot (QD) photocells may be one strategy to boost the photovoltaic conversion efficiency. In this work, we attempted to formulate a novel theoretical approach to evaluate…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Sheng-Nan Zhu , Shun-Cai Zhao , Lin-Jie Chen

With advanced micro- and nano-photonic structures, the vacuum photon-photon coupling rate is anticipated to approach the intrinsic loss rate and lead to unconventional quantum effects. Here, we investigate the classical-to-quantum…

Quantum Physics · Physics 2022-04-11 Yue-Xun Huang , Ming Li , Ke Lin , Yan-Lei Zhang , Guang-Can Guo , Chang-Ling Zou

The photoexcitation life-cycle from incident photon (and creation of photoexcited electron hole pair) to ultimate extraction of electrical current is a complex multi-physics process spanning across a range of spatio-temporal scales of…

Mesoscale and Nanoscale Physics · Physics 2025-01-29 Qiong Ma , Roshan Krishna Kumar , Su-Yang Xu , Frank H. L. Koppens , Justin C. W. Song

Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 K. Beltako , F. Michelini , N. Cavassilas , L. Raymond

We propose a dynamic mechanism for the reversible regulation of photosynthesis in varying light environments. We employ a three-level quantum model to take into account the correlations between charge donors and charge acceptors immediately…

Biological Physics · Physics 2024-11-13 Guang Yang , Gen Tatara
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