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High spin systems, like those that incorporate rare-earth $4f$ elements (REEs), are increasingly relevant in many fields. Although research in such systems is sparse, the large Hilbert spaces they occupy are promising for many applications.…

Mesoscale and Nanoscale Physics · Physics 2023-08-16 David W. Facemyer , Naveen K. Dandu , Alex Taekyung Lee , Vijay R. Singh , Anh T. Ngo , Sergio E. Ulloa

CuCrO2 is a manifestation of a two-dimensional triangular antiferromagnet which exhibits an incommensurate noncollinear magnetic structure similar to a classical 120 degree ordering. Using the inelastic neutron scattering technique, direct…

Strongly Correlated Electrons · Physics 2016-09-21 Kisoo Park , Joosung Oh , Jonathan C. Leiner , Jaehong Jeong , Kirrily C. Rule , Manh Duc Le , Je-Geun Park

A recent density functional theory (DFT) based analysis, complemented with Quantum Monte Carlo calculations revealed a highly spin-frustrating nature of the one-dimensional spin-$\frac{1}{2}$ compound $Cs_2CuAl_4O_8$ that comprises of…

Strongly Correlated Electrons · Physics 2019-02-12 Satyaki Kar

Spin-mechanical coupling is vital in diverse fields including spintronics, sensing and quantum transduction. Two-dimensional (2D) magnetic materials provide a unique platform for investigating spin-mechanical coupling, attributed to their…

Mesoscale and Nanoscale Physics · Physics 2024-08-07 Fan Fei , Yulu Mao , Wuzhang Fang , Wenhao Liu , Jack P. Rollins , Aswin L. N. Kondusamy , Bing Lv , Yuan Ping , Ying Wang , Jun Xiao

Molecular spintronics hinges on the detailed understanding of electronic and magnetic properties of molecules interfaced with various materials. Here we demonstrate with ab-initio simulations that the prototypical Co-phthalocyanine (CoPc)…

Mesoscale and Nanoscale Physics · Physics 2021-05-26 Ana M. Montero , Filipe S. M. Guimarães , Samir Lounis

We report neutron inelastic scattering measurements on the normal and superconducting states of single-crystalline Cs0.8Fe1.9Se2. Consistent with previous measurements on Rb(x)Fe(2-y)Se2, we observe two distinct spin excitation signals: (i)…

Frustrated triangular molecular magnets are a very important class of magnetic molecules since the absence of inversion symmetry allows an external electric field to couple directly with the spin chirality that characterizes their ground…

Mesoscale and Nanoscale Physics · Physics 2023-06-14 J. F. Nossa , M. F. Islam , Mark R. Pederson , C. M. Canali

Spectroscopic measurements with low-temperature scanning tunneling microscopes have been used very successfully for studying not only individual atomic or molecular spins on surfaces but also complexly designed coupled systems. The symmetry…

Mesoscale and Nanoscale Physics · Physics 2017-03-28 Markus Ternes

Motivated by the premise that superconductivity in iron-based superconductors is unconventional and mediated by spin fluctuations, an intense research effort has been focused on characterizing the spin excitation spectrum in the…

The magnetic and dielectric properties under high magnetic fields are studied in the single crystal of Cu3Mo2O9. This multiferroic compound has distorted tetrahedral spin chains. The effects of the quasi-one dimensionality and the…

Strongly Correlated Electrons · Physics 2013-11-13 H. Kuroe , K. Aoki , R. Kino , T. Sato , H. Kuwahara , T. Sekine , T Kihara , M. Akaki , Y. Kohama , M. Tokunaga , A. Matsuo , K. Kindo , M. Hase , K. Takehana , H. Kitazawa , K. Oka , T. Ito , H. Eisaki

We study the decay of entanglement of quantum dot electron-spin qubits under hyperfine interaction mediated decoherence. We show that two qubit entanglement of a single entangled initial state may exhibit decay characteristic of the two…

Quantum Physics · Physics 2014-06-25 Paweł Mazurek , Katarzyna Roszak , Ravindra W. Chhajlany , Paweł Horodecki

We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…

Strongly Correlated Electrons · Physics 2017-11-30 Zhe Wang , S. Reschke , D. Hüvonen , S. -H. Do , K. -Y. Choi , M. Gensch , U. Nage , T. Rõõm , A. Loidl

The ability to electrically-drive spin excitations in molecules with magnetic anisotropy is key for high-density storage and quantum-information technology. Electrons, however, also tunnel via the vibrational excitations unique to a…

Spin excitation spectrum is studied in the double-exchange model with randomness. Applying the spin wave approximation and the spectral function analysis, we examine excitation energy and linewidth using analytical as well as numerical…

Strongly Correlated Electrons · Physics 2009-11-07 Yukitoshi Motome , Nobuo Furukawa

We devise a formalism to investigate in a systematic way the spectroscopic magnetic excitations in molecular magnets. This consists in introducing a bilinear spin Hamiltonian that allows for discrete coupling parameters accounting for…

Strongly Correlated Electrons · Physics 2018-05-04 M. Georgiev , H. Chamati

We report on the spin waves and crystal field excitations in single crystal LiFePO$_4$ by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we…

Strongly Correlated Electrons · Physics 2017-03-15 Yuen Yiu , Manh Duc Le , Rasmus Toft-Peterson , Georg Ehlers , Robert McQueeney , David Vaknin

Coulomb interactions of few ($ N $) electrons confined in a disk shaped quantum dot, with a large magnetic field $B=B^*$ applied in the z-direction (orthogonal to the dot), produce a fully spin polarized ground state. We numerically study…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 P. Lucignano , B. Jouault , A. Tagliacozzo

We present a powder inelastic neutron scattering study of magnetic excitations in Ba$_2$FeReO$_6$, a member of the double perovskite family of materials which exhibit half-metallic behavior and high Curie temperatures. We find clear…

Strongly Correlated Electrons · Physics 2013-06-04 K. W. Plumb , A. M. Cook , J. P. Clancy , A. I. Kolesnikov , B. C. Jeon , T. W. Noh , A. Paramekanti , Young-June Kim

To elucidate the spin dynamics of La$_{2-x}$Sr$_x$CuO$_4$, which couples with the charge degree of freedom, the spin excitations spanning the characteristic energy ($E_{\rm cross}$ $\sim$35-40 meV) are investigated for underdoped $x$ = 0.10…

We use inelastic neutron scattering to study the temperature dependence of the spin excitations of a detwinned superconducting YBa$_2$Cu$_3$O$_{6.45}$ ($T_c=48$ K). In contrast to earlier work on YBa$_2$Cu$_3$O$_{6.5}$ ($T_c=58$ K), where…

Superconductivity · Physics 2009-11-13 Shiliang Li , Zahra Yamani , Hye Jung Kang , Kouji Segawa , Yoichi Ando , Xin Yao , H. A. Mook , Pengcheng Dai