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The spin dynamics and magnetic excitations of the slightly distorted triangular s = 3/2 system alpha-CaCr2O4 are investigated by means of Raman spectroscopy and electron spin resonance (ESR) to elucidate its peculiar magnetic properties.…

Assemblies of interacting quantum particles often surprise us with properties that are difficult to predict. One of the simplest quantum many-body systems is the spin 1/2 Heisenberg antiferromagnetic chain, a linear array of interacting…

Strongly Correlated Electrons · Physics 2013-07-02 M. Mourigal , M. Enderle , A. Klöpperpieper , J. -S. Caux , A. Stunault , H. M. Rønnow

We use neutron spectroscopy to determine the nature of the magnetic excitations in superconducting BaFe$_{1.9}$Ni$_{0.1}$As$_{2}$ ($T_{c}=20$ K). Above $T_{c}$ the excitations are gapless and centered at the commensurate antiferromagnetic…

Motivated by a recent experimental study on the quantum Ising magnet $\text{K}_2\text{Co}(\text{SeO}_3)_2$ that presented spectroscopic evidence of zero-field supersolidity (Chen et al., arXiv:2402.15869), we simulate the excitation…

Strongly Correlated Electrons · Physics 2025-07-15 Yi Xu , Juraj Hasik , Boris Ponsioen , Andriy H. Nevidomskyy

Molecular nanomagnets show clear signatures of coherent behavior and have a wide variety of effective low-energy spin Hamiltonians suitable for encoding qubits and implementing spin-based quantum information processing. At the nanoscale,…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Mircea Trif , Filippo Troiani , Dimitrije Stepanenko , Daniel Loss

The magnetic properties and the spin dynamics of two molecular magnets have been investigated by magnetization and d.c. susceptibility measurements, Electron Paramagnetic Resonance (EPR) and proton Nuclear Magnetic Resonance (NMR) over a…

Materials Science · Physics 2017-12-06 P. Khuntia , M. Mariani , M. C. Mozzati , L. Sorace , F. Orsini , A. Lascialfari , F. Borsa , M. Andruh , C. Maxim

We demonstrate that spin-charge separation can occur in two dimensions and note its confluence with superconductivity, topology, gauge theory, and fault-tolerant quantum computation. We construct a microscopic Ising-like model and, at a…

Strongly Correlated Electrons · Physics 2011-06-07 Chetan Nayak , Kirill Shtengel

It has been shown that the crystal-field interactions can produce a non- magnetic singlet ground state for the highly-correlated d6 system situated in the quasi-octahedral crystal field (CEF) surrounding provided the spin-orbit interactions…

Strongly Correlated Electrons · Physics 2009-10-31 R. J. Radwanski , Z. Ropka

Spin excitations of magnetoelectric LiNiPO$_4$ are studied by infrared absorption spectroscopy in the THz spectral range as a function of magnetic field through various commensurate and incommensurate magnetically ordered phases up to…

The low-energy excitations of Cr, i.e. the Fincher-Burke (FB) modes, have been investigated in the transversely polarized spin-density-wave phase by inelastic neutron scattering using a single-(Q+-) crystal with a propagation vector (Q+-)…

Materials Science · Physics 2009-11-10 H. Hiraka , P. Boni , K. Yamada , S. Park , S-. H. Lee , G. Shirane

The Kitaev candidate material Na$_2$Co$_2$TeO$_6$ is proposed to be proximate to a quantum spin liquid state but a suitable spin model and the nature of its ground states are still under debate. Our high-frequency/high-field electron spin…

Strongly Correlated Electrons · Physics 2025-09-08 Luca Bischof , Jan Arneth , Raju Kalaivanan , Raman Sankar , Kwang-Yong Choi , Rüdiger Klingeler

Close to the quantum critical point of the transverse-field Ising spin-chain model, an exotic dynamic spectrum was predicted to emerge upon a perturbative longitudinal field. The dynamic spectrum consists of eight particles and is governed…

Strongly Correlated Electrons · Physics 2020-09-25 Kirill Amelin , Johannes Engelmayer , Johan Viirok , Urmas Nagel , Toomas Rõõm , Thomas Lorenz , Zhe Wang

We present terahertz spectroscopic measurements of quantum spin dynamics in the honeycomb magnet K$_2$Co$_2$TeO$_6$ as a function of temperature, polarization and in an external magnetic field applied in the honeycomb plane. Magnetic…

Strongly Correlated Electrons · Physics 2025-08-01 Patrick Pilch , Laur Peedu , Urmas Nagel , Toomas Rõõm , Changqing Zhu , Yurii Skourski , Xianghan Xu , Robert J. Cava , Zhe Wang

Although BiFeO$_3$ is one of the most studied multiferroic materials, recent magnetization and neutron scattering studies have revealed a new magnetic phase in this compound - the transverse conical phase. To study the collective spin…

Materials Science · Physics 2024-02-05 B. Tóth , D. G. Farkas , K. Amelin , T. Rõõm , U. Nagel , L. Udvardi , L. Szunyogh , L. Rózsa , T. Ito , S. Bordács

We report on the observation of Kondo and split Kondo peaks in single-molecule transistors containing a single spin transition molecule with a Fe2+ ion. Coulomb blockade characteristics reveal a double quantum dot behavior in a parallel…

Mesoscale and Nanoscale Physics · Physics 2010-04-27 A. Bernand-Mantel , J. S. Seldenthuis , A. Beukman , H. S. J. van der Zant , V. Meded , R. Chandrasekhar , K. Fink , M. Ruben , F. Evers

Elementary excitations in condensed matter capture the complex many-body dynamics of interacting basic entities in a simple quasiparticle picture. In magnetic systems the most established quasiparticles are magnons, collective excitations…

Strongly Correlated Electrons · Physics 2019-05-07 M. Pregelj , A. Zorko , M. Gomilšek , M. Klanjšek , O. Zaharko , J. S. White , H. Luetkens , F. Coomer , T. Ivek , D. R. Góngora , H. Berger , D. Arčon

Molecular magnets are attractive as spin qubits due to their chemical tunability, addressability through electron-spin resonance techniques, and long coherence times. Clock transitions (CTs), for which the system is immune to the effect of…

X-ray magnetic circular dichroism spectroscopy has been used to characterize the electronic structure and magnetic moment of Cr$_2^+$. Our results indicate that the removal of a single electron from the $4s\sigma_g$ bonding orbital of…

We establish a correspondence between the electric dipole matrix elements of a polyatomic symmetric top molecule in a state with nonzero projection of the total angular momentum on the symmetry axis of the molecule and the magnetic dipole…

Quantum Gases · Physics 2015-03-20 Michael L Wall , Kenji Maeda , Lincoln D Carr

We formulate the theory for a diatomic molecule in a spatially degenerate electronic state interacting with a non-resonant laser field and investigate its rovibrational structure in the presence of the field. We report on \textit{ab initio}…