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The domain dynamics and spin-spin correlation of 2D ferromagnets Cr2X2Te6 (X=Si, Ge) are investigated by a composite magnetoelectric method. The magnetic field-temperature phase diagrams for both in-plane and out-of-plane magnetic fields…

Materials Science · Physics 2024-01-17 Yugang Zhang , Zefang Li , Jing Zhang , Long Zhang , Yonghong Li , Shuang Liu , Young Sun , Wenhong Wang , Yisheng Chai

The great success of point defects and dopants in semiconductors for quantum information processing has invigorated a search for molecules with analogous properties. Flexibility and tunability of desired properties in a large chemical space…

Materials Science · Physics 2023-01-11 Karolina Janicka , Aleksander L. Wysocki , Kyungwha Park

Recent radio frequency scanning tunneling spectroscopy (rf-STS) experiments have demonstrated nuclear and electron spin excitations up to $\pm12\hbar$ in a single molecular spin quantum dot (qudot). Despite the profound experimental…

We realize a strongly coupled double quantum dot in a single all-organic molecule by introducing a non-conjugated bridge in between two identical conjugated moieties. Spin-1/2 Kondo and Kondo enhanced low-energy excitations for respectively…

Mesoscale and Nanoscale Physics · Physics 2016-10-18 Max Koole , Jan C. Hummelen , Herre S. J. van der Zant

Although chromium trihalides are widely regarded as a promising class of two-dimensional magnets for next-generation devices, an accurate description of their electronic structure and magnetic interactions has proven challenging to achieve.…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 Ravi Yadav , Lei Xu , Michele Pizzochero , Jeroen van den Brink , Mikhail I. Katsnelson , Oleg V. Yazyev

The chiral $Fe_3O(NC_5H_5)_3(O_2CC_6H_5)_6$ molecular cation, with C$_3$ symmetry, is composed of three six-fold coordinated spin-carrying Fe$^{3+}$ cations that form a perfect equilateral triangle. Experimental reports demonstrating the…

Materials Science · Physics 2019-11-06 Alexander I Johnson , M. Fhokrul Islam , Carlo M. Canali , Mark R Pederson

Quantum spin rings represent fundamental model systems that exhibit distinctive quantum phenomena-such as quantum critical behavior and quasiparticle excitations-arising from their periodic boundary conditions and enhanced quantum…

We report the magnetic excitation spectrum as measured by inelastic neutron scattering for a polycrystalline sample of Sr$_3$CuPtO$_6$. Modeling the data by the 2+4 spinon contributions to the dynamical susceptibility within the chains, and…

The properties of the electronic ground state of the polar and paramagnetic chromium--closed-shell-atom molecules have been investigated. State-of-the-art \textit{ab initio} techniques have been applied to compute the potential energy…

Atomic Physics · Physics 2013-07-31 Michał Tomza

Collective motions in strongly interacting magnets involve many spins and are often described in terms of integer-spin excitations. However, in certain cases, the collective motion can behave as if these integer excitations break apart into…

The study of CoNb$_2$O$_6$ sits at the confluence of simplicity and complexity: on one hand, the model for Ising chains -- the building blocks of CoNb$_2$O$_6$ -- in a transverse field, can be exactly solved and, thus, serves as an…

Strongly Correlated Electrons · Physics 2022-05-31 Y. Xu , L. S. Wang , Y. Y. Huang , J. M. Ni , C. C. Zhao , Y. F. Dai , B. Y. Pan , X. C. Hong , P. Chauhan , S. M. Koohpayeh , N. P. Armitage , S. Y. Li

A broad continuum-like spin excitation (1--10 meV) with a peak structure around 2.4 meV has been observed in the ferroelectric $ab$ spiral spin phase of Gd$_{0.7}$Tb$_{0.3}$MnO$_3$ by using terahertz (THz) time-domain spectroscopy. Based on…

Strongly Correlated Electrons · Physics 2008-11-26 N. Kida , Y. Yamasaki , R. Shimano , T. Arima , Y. Tokura

The magnetic excitations in the paramagnetic-tetragonal phase of underdoped Ba(Fe0.953Co0.047)2As2, as measured by inelastic neutron scattering, can be well described by a phenomenological model with purely diffusive spin dynamics. At low…

Frustrated triangular molecular magnets (MMs) with anti-ferromagnetic ground states (GS) are an important class of magnetic systems with potential applications in quantum information processing. The two-fold degenerate GS of these…

Mesoscale and Nanoscale Physics · Physics 2025-01-20 M. F. Islam , Kushantha P. K. Withanage , C. M. Canali , Mark R. Pederson

High energy resolution spectroscopic studies of quantum magnets have proven to be extremely valuable in directly accessing magnetodynamics quantities, such as energy barriers, magnetic interactions, lifetime of excited states and…

Mesoscale and Nanoscale Physics · Physics 2022-02-17 Sascha Brinker , Felix Küster , Stuart S. P. Parkin , Paolo Sessi , Samir Lounis

High-spin states in the doubly-odd $^{198}$Bi nucleus have been studied by using the $^{185,187}$Re($^{16}$O, xn) reactions at the beam energy of 112.5 MeV. $\gamma-\gamma$ coincidence were measured by using the INGA array with 15 Compton…

The magnetic excitation spectrum and Hamiltonian of the quantum magnet BaCuTe2O6 is studied by inelastic neutron scattering (INS) and density functional theory (DFT). INS on powder and single crystal samples reveals overlapping spinon…

Strongly Correlated Electrons · Physics 2023-05-19 A. Samartzis , S. Chillal , H. O. Jeschke , D. J. Voneshen , Z. Lu , A. T. M. N. Islam , B. Lake

Transition-metal ions with $5d^2$ electronic configuration in a cubic crystal field are prone to have a vanishing dipolar magnetic moment but finite higher-order multipolar moments, and they are expected to exhibit exotic physical…

Strongly Correlated Electrons · Physics 2025-07-16 J. Okamoto , G. Shibata , Yu. S. Posonov , H. Hayashi , K. Yamaura , H. Y. Huang , A. Singh , C. T. Chen , A. Tanaka , S. V. Streltsov , D. J. Huang , A. Fujimori

Recent inelastic neutron diffraction measurements on Cr$_2$(Te, W, Mo)O$_6$ have revealed that these systems consist of bilayers of spin-3/2 Cr$^{3+}$ ions with strong antiferromagnetic inter-bilayer coupling and tuneable intra-bilayer…

Strongly Correlated Electrons · Physics 2019-04-04 Kingshuk Majumdar , Subhendra D. Mahanti

A family of double-quantum excitation schemes is described for the solution nuclear magnetic resonance (NMR) of near-equivalent spin-1/2 pairs. These new methods exploit the spinor behaviour of 2-level systems, whose signature is the change…

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