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Controlling nonequilibrium dynamics in quantum materials requires ultrafast probes with spectral selectivity. We report femtosecond reflectivity measurements on the cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ using…

We report a novel experimental technique to investigate ultrafast dynamics in photoexcited molecules by probing the third-order nonlinear optical susceptibility. A non-colinear 3-pulse scheme is developed to probe the ultrafast dynamics of…

We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick"…

Optics · Physics 2015-06-11 C. Bloomquist , S. Zhdanovich , A. A. Milner , V. Milner

This paper presents a study of electron spin dynamics in bulk GaAs at low temperatures for elevated optical excitation conditions. Our time-resolved Faraday rotation measurements yield sub-nanosecond electron spin dephasing-times over a…

Materials Science · Physics 2015-05-13 M. Krauss , R. Bratschitsch , Z. Chen , S. T. Cundiff , H. C. Schneider

Using matrix product state techniques we study the nonequilibrium dynamical response of the half-filled Hubbard ladder when subject to an optical pump. Optical pumping offers a way of producing and manipulating new strongly correlated…

Strongly Correlated Electrons · Physics 2026-04-14 E. Merhej , J. P. Hague , R. M. Konik , A. J. A. James

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

Coherent light-matter interactions mediated by opto-magnetic phenomena like the inverse Faraday effect (IFE) are expected to provide a non-thermal pathway for ultrafast manipulation of magnetism on timescales as short as the excitation…

The spin transfer torque is a phenomenon in which angular momentum of a spin polarized electrical current entering a ferromagnet is transferred to the magnetization. The effect has opened a new research field of electrically driven…

Materials Science · Physics 2012-05-07 P. Nemec , E. Rozkotova , N. Tesarova , F. Trojanek , E. De Ranieri , K. Olejnik , J. Zemen , V. Novak , M. Cukr , P. Maly , T. Jungwirth

Faraday waves, typically observed in driven fluids, result from the confluence of nonlinearity and parametric amplification. Here we show that optical pulses can generate analogous phenomena that persist much longer than the pump…

Mesoscale and Nanoscale Physics · Physics 2025-11-11 Daniel Kaplan , Pavel A. Volkov , Andrea Cavalleri , Premala Chandra

The present work is dedicated to the theoretical analysis of two-photon excitation of atoms in a discrete energy spectrum by ultrashort electromagnetic pulses of femto- and subfemtosecond ranges of durations. As examples, excitation of…

Atomic Physics · Physics 2016-05-25 Valery Astapenko , Sergey Sakhno

Identifying the microscopic nature of non-equilibrium energy transfer mechanisms among electronic, spin and lattice degrees of freedom is central for understanding ultrafast phenomena such as manipulating magnetism on the femtosecond…

A central prospect of antiferromagnetic spintronics is to exploit magnetic properties that are unavailable with ferromagnets. However, this poses the challenge of accessing such properties for readout and control. To this end, light-induced…

The inverse Faraday effect is an opto-magnetic phenomenon that describes the ability of circularly polarized light to induce magnetism in solids. The capability of light to control magnetic order in solid state materials and devices is of…

Materials Science · Physics 2023-12-20 Víctor H. Ortiz , Shashi B. Mishra , Luat Vuong , Sinisa Coh , Richard B. Wilson

Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…

We present a concept for selective excitation of magnetostatic surface waves with quasi-discrete spectrum using spatially patterned femtosecond laser pulses inducing either ultrafast change of magnetic anisotropy or inverse Faraday effect.…

Rashba-type spin-orbit coupling gives rise to distinctive surface and interface phenomena, such as spin-momentum locking and spin splitting. In nonequilibrium settings, one of the key manifestations is the (Rashba-)Edelstein effect, where…

Materials Science · Physics 2025-10-08 Oliver Busch , Franziska Ziolkowski , Börge Göbel , Ingrid Mertig , Jürgen Henk

The coupling of laser light to matter can exert sub-cycle coherent control over material properties, with optically induced currents and magnetism shown to be controllable on ultrafast femtosecond time scales. Here, by employing laser light…

Optics · Physics 2024-06-19 Q. Z. Li , S. Shallcross , J. K. Dewhurst , S. Sharma , P. Elliott

We investigate the interaction of femtosecond laser pulses with spins including relativistic corrections. The time-ordered magneto-optical signals corresponding to a pump-probe configuration are calculated in the case of one electron…

Strongly Correlated Electrons · Physics 2012-01-04 Hélène Vonesch , Jean-Yves Bigot

Understanding how fast short-range interactions build up long-range order is one of the most intriguing topics in condensed matter physics. FeRh is a test specimen for studying this problem in magnetism, where the microscopic spin-spin…

Designing material properties on demand has important implications to potential future technological applications. While theoretically it is always possible to tune various intrinsic energy scales, there are fundamental limitations to this…

Strongly Correlated Electrons · Physics 2025-02-13 Benedikt Fauseweh , Jian-Xin Zhu