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We explore the impact of optical excitation using two interfering ultrashort optical pulses on ultrafast magnetization dynamics. Our investigation focuses on Pt/Co/Pt multilayers and TbCo alloy samples, employing a dual pump approach. We…

The ultrafast response to an optical pulse excitation of the spin-spin exchange interaction in transition metal anti-ferromagnets is studied within the framework of the time-dependent spin-density functional theory. We propose a formulation…

Mesoscale and Nanoscale Physics · Physics 2017-08-16 Jacopo Simoni , Maria Stamenova , Stefano Sanvito

Optical pump-probe setups are commonly used for excitation and investigation of the spin dynamics in various types of magnetic materials. However, usually the spatially homogeneous excitation is considered. In the present study we describe…

We study ultrafast magnetization quenching of ferromagnetic iron following excitation by an optical vs a terahertz pump pulse. While the optical pump (photon energy of 3.1 eV) induces a strongly nonthermal electron distribution, terahertz…

A time-resolved optical pump-probe technique has been applied for studying the ultrafast dynamics in the magnetic semiconductor EuTe near the absorption band gap. We show that application of external magnetic field up to 6 T results in…

We investigate the impact of non-collinear dual optical excitation on the magnetization precession in a permalloy thin film using two ultrashort laser pulses. By analyzing the magnetization dynamics using time-resolved magneto-optical…

Materials Science · Physics 2024-06-28 Sergii Parchenko , Davide Pecchio , Ritwik Mondal , Peter M. Oppeneer , Andreas Scherz

The dynamics of single laser-driven electrons and many particle systems with spin are investigated on the basis of a classical theory. We demonstrate that the spin forces can alter the electron dynamics in an ultra-relativistic laser field…

Plasma Physics · Physics 2014-06-17 Meng Wen , Heiko Bauke , Christoph H. Keitel

We investigate the spin-resolved electron dynamics in a double quantum dot driven by ultrafast asymmetric electromagnetic pulses. Using a analytical model we show that applying an appropriate pulse sequence allows to control coherently the…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 J. Waetzel , A. S. Moskalenko , J. Berakdar

All-optical re-switching has been investigated in the half-metallic Heusler ferrimagnet Mn2Ru0.9Ga, where Mn atoms occupy two inequivalent sites in the XA-type structure. The effect of a second 200 fs 800 nm pump pulse that follows a first…

Materials Science · Physics 2021-05-05 C. Banerjee , K. Rode , G. Atcheson , S. Lenne , P. Stamenov , J. M. D. Coey , J. Besbas

Since the beginning of femtomagnetism, it has been hotly debated how an ultrafast laser pulse can demagnetize a sample and switch its spins within a few hundred femtoseconds, but no consensus has been reached. In this paper, we propose that…

Materials Science · Physics 2015-06-22 G. P. Zhang , Mingqiang Gu , X. S. Wu

Based on a multi-particle-state stimulated Raman adiabatic passage approach, a comprehensive theoretical study on the ultrafast optical manipulation of electron spins in quantum wells is presented. In addition to corroborating the…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Jinshuang Jin , Xin-Qi Li

Laser radiation incident on a ferromagnetic sample produces excited electrons and currents whose spin polarization must not be aligned with the magnetization -- an effect due to spin-orbit coupling that is ubiquitous in spin- and…

Materials Science · Physics 2023-11-03 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

We explore the possibility of ultrafast, coherent all-optical magnetization switching in antiferromagnets by studying the action of the inverse Faraday effect in CrPt, an easy-plane antiferromagnet. Using a combination of density functional…

Spin angular momentum transfer in magnetic bilayers offers the possibility of ultrafast and low-loss operation for next-generation spintronic devices. We report the field- and temperature- dependent measurements on the magnetization…

Materials Science · Physics 2023-01-03 X. Liu , P. Liu , H. C. Yuan , J. Y. Shi , H. L. Wang , S. H. Nie , F. Jin , Z. Zheng , X. Z. Yu , J. H. Zhao , H. B. Zhao , G. Lüpke

Ultrafast light pulses can modify the electronic properties of quantum materials by perturbing the underlying, intertwined degrees of freedom. In particular, iron-based superconductors exhibit a strong coupling among electronic nematic…

Frontiers of attosecond science are constantly shifting, thus addressing more and more intricate effects with increasing resolution. Ultrashort pulses offer a practical way to prepare complex superpositions of quantum states, follow, and…

Quantum Physics · Physics 2019-05-16 Huihui Wang , Tobias Möhle , Oliver Kühn , Sergey I. Bokarev

Superconducting state dynamics following excitation of a superconductor with a femtosecond optical pulse is studied in terms of a phenomenological Rothwarf and Taylor model. Analytical solutions for various limiting cases are obtained. The…

Superconductivity · Physics 2009-11-11 V. V. Kabanov , J. Demsar , D. Mihailovic

Resonant optical excitation of apical oxygen vibrational modes in the normal state of underdoped YBa2Cu3O6+x induces a transient state with optical properties similar to those of the equilibrium superconducting state. Amongst these, a…

A theoretical calculation is performed for the ultrafast spin dynamics in nickel using an exact diagonalization method. The present theory mainly focuses on a situation where the intrinsic charge and spin dynamics is probed by the nonlinear…

Materials Science · Physics 2009-10-31 G. P. Zhang , W. Hübner

Tunnel-coupled optically active quantum dot molecules (QDMs), have the potential to operate as spin-photon-interfaces with coupled spins that interact with two different photon frequencies at the same time. A prerequisite is to…

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