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We report on the structural evolution, spin phonon interactions, and magnetoelastic effects in bulk LaFeO3 perovskite across its antiferromagnetic transition. We found that while the lattice constants exhibit slight deviations at the Neel…

GeCu2O4 exhibits a tetragonal spinel structure due to the strong Jahn-Teller distortion associated with Cu2+ ions. We show that its magnetic structure can be described as slabs composed of a pair of layers with orthogonally oriented spin…

Materials Science · Physics 2016-12-14 T. Zou , Y. -Q. Cai , C. R. dela Cruz , V. O. Garlea , S. D. Mahanti , J. -G. Cheng , X. Ke

Spin-nematic and spin-smectic phases have been reported in magnetic materials, which break rotational symmetry while preserving translational symmetry along certain directions. However, until now the analogy to liquid crystals remained…

We present a neutron diffraction study of FeV2O4, which is rare in exhibiting spin and orbital degrees of freedom on both cation sublattices of the spinel structure. Our data confirm the existence of three structural phase transitions…

Strongly Correlated Electrons · Physics 2012-09-03 G. J. MacDougall , V. O. Garlea , A. A. Aczel , H. D. Zhou , S. E. Nagler

We report the discovery of a spin one diamond lattice in NiRh2O4. This spinel undergoes a cubic to tetragonal phase transition at T = 440 K that leaves all nearest neighbor interactions equivalent. In the tetragonal phase, magnetization…

Strongly Correlated Electrons · Physics 2018-03-30 J. R. Chamorro , L. Ge , J. Flynn , M. Subramanian , M. Mourigal , T. M. McQueen

We present neutron diffraction analysis of BaFe$_2$(As$_{1-x}$P$_x$)$_2$ over a wide temperature (10 to 300 K) and compositional ($0.11 \leq x \leq 0.79$) range, including the normal state, the magnetically ordered state, and the…

The unusual magnetic properties of a novel low-dimensional quantum ferrimagnet Cu$_2$Fe$_2$Ge$_4$O$_{13}$ are studied using bulk methods, neutron diffraction and inelastic neutron scattering. It is shown that this material can be described…

Strongly Correlated Electrons · Physics 2009-11-10 T. Masuda , A. Zheludev , B. Grenier , S. Imai , K. Uchinokura , E. Ressouche , S. Park

We present a unique study of the frustrated spinel MgV2O4 which possesses highly coupled spin, lattice and orbital degrees of freedom. Using large single-crystal and powder samples, we find a distortion from spinel at room temperature…

Strongly Correlated Electrons · Physics 2010-10-14 Elisa M. Wheeler , Bella Lake , A. T. M. Nazmul Islam , Manfred Reehuis , Paul Steffens , Tatiana Guidi , Adrian H. Hill

Entangled spin and orbital degrees of freedom provide a multiflavor route to novel magnetic states inaccessible in conventional spin systems. Here, we report the experimental identification of an emergent vortex lattice in the multiflavor…

We discuss the origin of spin correlations observed in neutron scattering experiments on the paramagnetic phase of a number of frustrated spinel compounds, most notably ZnCr2O4. These correlations are striking for two reasons. First, they…

Strongly Correlated Electrons · Physics 2010-06-22 P. H. Conlon , J. T. Chalker

With decreasing temperature Sr$_2$VO$_4$ undergoes two structural phase transitions, tetragonal-to-orthorhombic-to-tetragonal, without long-range magnetic order. Recent experiments suggest, that only at very low temperature Sr$_{2}$VO$_{4}$…

Materials Science · Physics 2017-11-15 Bongjae Kim , Sergii Khmelevskyi , Peter Mohn , Cesare Franchini

Antiferromagnetic Heisenberg model on the triangular lattice is perhaps the best known example of frustrated magnets, but it orders at low temperatures. Recent density matrix renormalization group (DMRG) calculations find that next nearest…

Quantum Gases · Physics 2018-05-08 Ahmet Keles , Erhai Zhao

The classical bilinear-biquadratic nearest-neighbor Heisenberg antiferromagnet on the pyrochlore lattice does not exhibit conventional Neel-type magnetic order at any temperature or magnetic field. Instead spin correlations decay…

Strongly Correlated Electrons · Physics 2010-05-18 Nic Shannon , Karlo Penc , Yukitoshi Motome

Motivated by recent experiments, we present a comprehensive theoretical study of the geometrically frustrated strongly correlated magnetic insulator Mn$_3$O$_4$ spinel oxide based on a microscopic Hamiltonian involving lattice, spin and…

Strongly Correlated Electrons · Physics 2017-08-23 Santanu Pal , Siddhartha Lal

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

Frustration in spin system can give rise to unique ordered states and as a consequence several physical phenomena are expected such as multiferroics, high temperature superconductors and anomalous hall effect. Here we report the "new…

Strongly Correlated Electrons · Physics 2018-08-01 GiBaik Sim , SungBin Lee

We derive a spin-orbital Hamiltonian for a triangular lattice of e_g orbital degenerate (Ni^{3+}) transition metal ions interacting via 90 degree superexchange involving (O^{2-}) anions, taking into account the on-site Coulomb interactions…

Strongly Correlated Electrons · Physics 2009-11-11 Albert J. W. Reitsma , Louis F. Feiner , Andrzej M. Oles'

{\alpha}-CaCr2O4 is a distorted triangular antiferromagnet. The magnetic Cr3+ ions which have spin-3/2 and interact with their nearest neighbors via Heisenberg direct exchange interactions, develop long-range magnetic order below T_N=42.6…

Strongly Correlated Electrons · Physics 2011-11-22 S. Tóth , B. Lake , S. A. J. Kimber , O. Pieper , M. Reehuis , A. T. M. N. Islam , O. Zaharko , C. Ritter , A. H. Hill , H. Ryll , D. N. Argyriou , A. J. Williams

We study double-exchange models with itinerant t2g electrons in spinel and pyrochlore crystals. In both cases the localized spins form a network of corner-sharing tetrahedra. We show that the strong directional dependence of t2g orbitals…

Strongly Correlated Electrons · Physics 2011-10-26 Gia-Wei Chern , Cristian D. Batista

The collective behavior of interacting magnetic moments can be strongly influenced by the topology of the underlying lattice. In geometrically frustrated spin systems, interesting chiral correlations may develop that are related to the spin…

Strongly Correlated Electrons · Physics 2007-05-23 D. Grohol , K. Matan , J. H. Cho , S. -H. Lee , J. W. Lynn , D. G. Nocera , Y. S. Lee