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We study the transport through a molecular junction exhibiting interference effects. We show that these effects can still be observed in the presence of molecular vibrations if Coulomb repulsion is taken into account. In the Kondo regime,…

Strongly Correlated Electrons · Physics 2019-09-04 P. Roura-Bas , F. Güller , L. Tosi , A. A. Aligia

Destructive quantum interference in electron transport through molecules provides an unconventional route for suppressing electric current. In this work we introduce "interference vectors" for each interference and use them to characterize…

Mesoscale and Nanoscale Physics · Physics 2017-07-20 Panu Sam-ang , Matthew G. Reuter

Recent observations of destructive quantum interference in single-molecule junctions confirm the role played by quantum effects in the electronic conductance properties of molecular systems. We show here that the destructive interference…

Mesoscale and Nanoscale Physics · Physics 2017-09-25 Riccardo Frisenda , Vera Jansen , Ferdinand C. Grozema , Herre S. J. van der Zant , Nicolas Renaud

Destructive quantum interference (DQI) in single molecule electronics is a purely quantum mechanical effect and entirely defined by inherent properties of the molecule in the junction such as its structure and symmetry. This definition of…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Xin Zhao , Victor Geskin , Robert Stadler

Quantum interference can profoundly affect charge transport in single molecules, but experiments can usually measure only the conductance at the Fermi energy. Because in general the most pronounced features of the quantum interference are…

Destructive quantum interference in single molecule electronics is an intriguing phe- nomenon; however, distinguishing quantum interference effects from generically low transmission is not trivial. In this paper, we discuss how quantum…

Mesoscale and Nanoscale Physics · Physics 2014-10-01 Jacob Lykkebo , Alessio Gagliardi , Alessandro Pecchia , Gemma C. Solomon

Quantum interference, be it destructive or constructive, has a substantial influence on the magnitude of molecular conductance and consequently there is significant interest in predicting these effects. It is commonly thought that…

Mesoscale and Nanoscale Physics · Physics 2015-10-21 Kim G. L. Pedersen , Anders Borges , Per Hedegård , Gemma C. Solomon , Mikkel Strange

Destructive quantum interference (QI) has been a source of interest as a new paradigm for molecular electronics as the electronic conductance is widely dependent on the occurrence or absence of destructive QI effects. In order to interpret…

Mesoscale and Nanoscale Physics · Physics 2022-09-23 O. Sengul , A. Valli , R. Stadler

We analyze quantum interference and decoherence effects in single-molecule junctions both experimentally and theoretically by means of the mechanically controlled break junction technique and density-functional theory. We consider the case…

Mesoscale and Nanoscale Physics · Physics 2012-09-26 Stefan Ballmann , Rainer Härtle , Pedro B. Coto , Marcel Mayor , Mark Elbing , Martin R. Bryce , Michael Thoss , Heiko B. Weber

Molecular electronics offers unique scientific and technological possibilities, resulting from both the nanometre scale of the devices and their reproducible chemical complexity. Two fundamental yet different effects, with no classical…

Mesoscale and Nanoscale Physics · Physics 2017-05-12 Andrew K. Mitchell , Kim G. L. Pedersen , Per Hedegaard , Jens Paaske

Quantum interference (QI) effects in molecular junctions may be used to obtain large thermoelectric responses. We study the electrical conductance G and the thermoelec- tric response of a series of molecules featuring a quinoid core using…

Mesoscale and Nanoscale Physics · Physics 2015-07-02 M. Strange , J. S. Seldenthuis , C. J. O. Verzijl , J. M. Thijssen , G. C. Solomon

Quantum interference effects and decoherence mechanisms in single-molecule junctions are analyzed employing a nonequilibrium Green's function approach. Electrons tunneling through quasi-degenerate states of a nanoscale molecular junction…

Mesoscale and Nanoscale Physics · Physics 2011-07-25 R. Härtle , M. Butzin , O. Rubio-Pons , M. Thoss

The gravitationally induced entanglement is a type of quantum entanglement that can be generated between two mesoscopic particles using their Newtonian gravitational interaction. It has attracted a great deal of attention as a new platform…

Quantum Physics · Physics 2024-01-10 Aiham M. Rostom

Molecular junctions -- whether actual single molecules in nanowire break junctions or artificial molecules realized in coupled quantum dot devices -- offer unique functionality due to their orbital complexity, strong electron interactions,…

Mesoscale and Nanoscale Physics · Physics 2024-08-15 Sudeshna Sen , Andrew K. Mitchell

The quest for molecular structures exhibiting strong quantum interference effects in the transport setting has long been on the forefront of chemical research. Here, we establish theoretically that the unusual geometry of spiro-conjugated…

Mesoscale and Nanoscale Physics · Physics 2018-04-03 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

As the dimensions of a conductor approach the nano-scale, quantum effects will begin to dominate its behavior. This entails the exciting possibility of controlling the conductance of a device by direct manipulation of the electron wave…

The characterization of quantum correlations is crucial to the development of new quantum technologies and to understand how dramatically quantum theory departs from classical physics. Here we systematically study single- and multiparticle…

Quantum Physics · Physics 2020-06-05 Rejane Alves de Brito , Bertúlio de Lima Bernardo

Quantum theory permits interference between indistinguishable paths but, at the same time, restricts its order. Single-particle interference, for instance, is limited to the second order, that is, to pairs of single-particle paths. To date,…

Quantum Physics · Physics 2021-05-13 Marc-Oliver Pleinert , Alfredo Rueda , Eric Lutz , Joachim von Zanthier

In this work, we explore an unconventional class of problems in the study of (quantum) critical phenomena, termed ''deep boundary criticality''. Traditionally, critical systems are analyzed with two types of perturbations: those uniformly…

Strongly Correlated Electrons · Physics 2025-10-23 Shang Liu

Using exact-diagonalization techniques supplemented by a Dyson equation embedding procedure, the transport properties of multilevel quantum dots are investigated in the Kondo regime. The conductance can be decomposed into the contributions…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 C. A. Büsser , G. B. Martins , K. A. Al-Hassanieh , Adriana Moreo , Elbio Dagotto
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