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X-ray magnetic circular dichroism (XMCD) is generally not observed for antiferromagnetic (AFM) states because XMCD signals from the antiparallelly coupled spins cancel each other. In this letter, we theoretically show the presence of an…

Strongly Correlated Electrons · Physics 2021-04-21 N. Sasabe , M. Kimata , T. Nakamura

A systematic ab-initio study within the framework of the local-spin-density approximation including spin-orbit coupling and an orbital-polarization term is performed for the spin and orbital moments and for the X-ray magnetic circular…

Materials Science · Physics 2009-11-07 Matej Komelj , Claude Ederer , James W. Davenport , Manfred Faehnle

High-throughput X-ray magnetic circular dichroism (XMCD) spectroscopy was conducted on Fe-Co-Ni compositionally graded films to systematically analyze the variation of magnetic properties as a function of composition. On-the-fly XMCD…

Materials Science · Physics 2025-06-27 Y. Yamasaki , N. Sasabe , Y. Ishii , Y. Sekiguchi , A. Sumiyoshiya , Y. Tanimoto , Y. Kotani , T. Nakamura , H. Nomura

We present numerical simulations of x-ray magnetic circular dichroism (XMCD) at the L$_{2,3}$ edge of Ni in the weakly ferromagnetic altermagnet NiF$_2$. Our results predict a significant XMCD signal for light propagating perpendicular to…

Materials Science · Physics 2025-05-28 A. Hariki , K. Sakurai , T. Okauchi , J. Kuneš

X-ray magnetic circular dichroism (XMCD) and resonant inelastic X-ray scattering with magnetic circular dichroism (RIXS-MCD) provide unparalleled insights into the electronic and magnetic dynamics of complex materials. Yet, their spectra…

Corrections to the atomic orbital sum rule for circular magnetic x-ray dichroism in solids are derived using orthonormal LMTOs as a single-particle basis for electron band states.

Materials Science · Physics 2009-10-31 R. Benoist , P. Carra , O. K. Andersen

X-ray magnetic circular dichroism provides a means to identify ferromagnetic, chiral, and altermagnetic orders via their time-reversal-symmetry ($\mathcal{T}$) breaking. However, differentiating magnetic domains related by crystallographic…

Cluster magnetic multipoles are order parameters that describe the symmetry of spin arrangements in magnetic materials. High-order multipoles are particularly important in non-collinear antiferromagnets, where they determine key physical…

Mesoscale and Nanoscale Physics · Physics 2025-01-14 Myoung-Woo Yoo , Axel Hoffmann

We present numerical simulation of the X-ray magnetic circular dichroism (XMCD) of the $L_{2,3}$ and $M_{2,3}$ edges of Ru in antiferromagnetic RuO$_2$ using a combination of density functional + dynamical mean-field theory and…

Strongly Correlated Electrons · Physics 2024-03-13 A. Hariki , Y. Takahashi , J. Kuneš

The magneto-optical Kerr effect (MOKE) has recently been discovered in antiferromagnetic Kagome lattice Mn3Sn. Since the compound exhibits a coplanar $120^\circ$ antiferromagnetic (AFM) order, the magnetic moments cancel each other, and the…

Strongly Correlated Electrons · Physics 2020-08-26 Yuichi Yamasaki , Hironori Nakao , Taka-hisa Arima

The orbital and spin magnetic moments, and the X-ray-magnetic circular-dichroism (XMCD) spectra at the $M_{4,5}$ edges of the U atoms in a UAs/Co multilayer and in an $\alpha$-U film are calculated within the framework of the…

Strongly Correlated Electrons · Physics 2009-11-10 Matej Komelj , Natasa Stojic

Polarization-dependent photon spectroscopy (dichroism) using signal-enhancing superchiral beams is shown to be sensitive to magnetic properties of the sample, whereas previous investigations explored charge-like electronic properties of…

Materials Science · Physics 2019-03-06 S. W. Lovesey , J. T. Collins , S. P. Collins

The theory of the method of magnetic circular dichroism spectroscopy in reflected light (RMCD) has been developed using a simplified scheme without an analyzer, with the use of an additional mirror in the optical system and with the…

Optics · Physics 2025-12-01 Yuri Markin , Zoja Kun'kova

X-ray free-electron lasers (XFELs) have been widely used for applications such as X-ray crystallography and magnetic spin probes because of their unprecedented performance. Recently, time-resolved X-ray magnetic circular dichroism (XMCD)…

Instrumentation and Detectors · Physics 2018-07-04 Bangjie Deng , Jiawei Yan , Qingmin Zhang , Yaodong Sang , Haixiao Deng

We present a derivation of the orbital and spin sum rules for magnetic circular dichroic spectra measured by electron energy loss spectroscopy in a transmission electron microscope. These sum rules are obtained from the differential cross…

Other Condensed Matter · Physics 2009-11-13 L. Calmels , F. Houdellier , B. Warot-Fonrose , C. Gatel , M. J. Hÿtch , V. Serin , E. Snoeck , P. Schattschneider

A computational expression for the Faraday A term of magnetic circular dichroism (MCD) is derived within coupled cluster response theory and alternative computational expressions for the B term are discussed. Moreover, an approach to…

Computational Physics · Physics 2020-05-14 Rasmus Faber , Simone Ghidinelli , Christof Hättig , Sonia Coriani

Recently, the topic of altermagnetism has attracted tremendous attention and RuO2 have been demonstrated to be one of the most promising altermagnetic candidates. However, disputes still remain on the existence of magnetic order in RuO2.…

The X-ray magnetic circular dichroism (XMCD) has been measured at the Co K edge in Co-hcp and R-Co compounds (R=La, Tb, Dy). The structure of the experimental XMCD spectra in the near-edge region has been observed to be highly sensitive to…

Materials Science · Physics 2009-10-31 J. P. Rueff , R. M. Galera , Ch. Giorgetti , E. Dartyge , Ch. Brouder , M. Alouani

We present an x-ray spectromicroscopic investigation of single-crystalline magnetic FeMn/Co bilayers on Cu(001), using X-ray magnetic circular (XMCD) and linear (XMLD) dichroism at the Co and Fe L3 absorption edges in combination with…

Materials Science · Physics 2007-06-13 W. Kuch , F. Offi , L. I. Chelaru , J. Wang , K. Fukumoto , M. Kotsugi , J. Kirschner , J. Kunes

Ca_1-xSr_xRuO_3, which is ferromagnetic for Sr concentration x > 0.3, has been studied by x-ray magnetic circular dichroism (XMCD) in Ru 3p and O 1s core-level x-ray absorption. XMCD signals appear at x ~ 0.3 and monotonically increases…

Strongly Correlated Electrons · Physics 2008-04-21 J. Okamoto , T. Okane , Y. Saitoh , K. Terai , S. -I. Fujimori , Y. Muramatsu , K. Yoshii , K. Mamiya , T. Koide , A. Fujimori , Z. Fang , Y. Takeda , M. Takano