English

X-ray Magnetic Circular Dichroism in RuO$_2$

Strongly Correlated Electrons 2024-03-13 v2 Materials Science

Abstract

We present numerical simulation of the X-ray magnetic circular dichroism (XMCD) of the L2,3L_{2,3} and M2,3M_{2,3} edges of Ru in antiferromagnetic RuO2_2 using a combination of density functional + dynamical mean-field theory and configuration interaction treatment of Anderson impurity model. We study the dependence of the dichroic spectra on the orientation of the N\'eel vector and discuss it in the context of altermagnetism. Approximate equivalence between the XMCD spectra for geometries with X-rays propagating parallel and perpendicular to the N\'eel vector is found and shown to be exact in absence of valence spin-orbit coupling and core-valence multipolar interaction.

Keywords

Cite

@article{arxiv.2312.02629,
  title  = {X-ray Magnetic Circular Dichroism in RuO$_2$},
  author = {A. Hariki and Y. Takahashi and J. Kuneš},
  journal= {arXiv preprint arXiv:2312.02629},
  year   = {2024}
}

Comments

7 pages, 6 figures