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Chemical manifestations of strong light-matter coupling have been recently subject of intense experimental and theoretical studies. Here we review the present status of this field. Section 1 is an introduction to molecular polaritonics and…

Chemical Physics · Physics 2021-12-15 Tao E. Li , Bingyu Cui , Joseph E. Subotnik , Abraham Nitzan

We investigate the quantum optical properties of a single photon emitter coupled to a finite-size metal nanoparticle using a photon Green function technique that rigorously quantizes the electromagnetic fields. We first obtain pronounced…

Mesoscale and Nanoscale Physics · Physics 2012-02-07 C. Van Vlack , Philip Trøst Kristensen , S. Hughes

Photon-photon scattering in vacuum is extremely weak. However, strong effective interactions between single photons can be realized by employing strong light-matter coupling. These interactions are a fundamental building block for quantum…

Quantum Physics · Physics 2017-07-07 Dibyendu Roy , C. M. Wilson , Ofer Firstenberg

The light emission from a scanning tunneling microscope operated on a Ag(111) surface at 6 K is analyzed from low conductances to values approaching the conductance quantum. Optical spectra recorded at a sample voltages V reveal emission…

Mesoscale and Nanoscale Physics · Physics 2018-09-11 Peter-Jan Peters , Fei Xu , Kristen Kaasbjerg , Gianluca Rastelli , Wolfgang Belzig , Richard Berndt

We investigate a periodic array of aluminum nanoantennas embedded in a light-emitting slab waveguide. By varying the waveguide thickness we demonstrate the transition from weak to strong coupling between localized surface plasmons in the…

The regime of strong light-matter coupling is typically associated with weak excitation. With current realizations of cavity-QED systems, strong coupling may persevere even at elevated excitation levels sufficient to cross the threshold to…

We present a detailed study of the electroluminescence of intersubband devices operating in the light-matter strong coupling regime. The devices have been characterized by performing angle resolved spectroscopy that shows two distinct light…

Mesoscale and Nanoscale Physics · Physics 2012-12-27 Pierre Jouy , Angela Vasanelli , Yanko Todorov , Luca Sapienza , Raffaele Colombelli , Ulf Gennser , Carlo Sirtori

When light and matter are weakly coupled, they can be described as two distinctive systems exchanging quanta of energy. By contrast, for very large coupling strength, the systems hybridize and form compounds that cannot be described in…

Quantum Physics · Physics 2021-05-25 Louis Garbe

We develop a new general formulation to explore light-driven electron transport through a single-molecule device with multiple pathways. Three individual systems are proposed including (i) a two-terminal molecular junction based on…

Mesoscale and Nanoscale Physics · Physics 2014-01-20 Liang-Yan Hsu , Herschel Rabitz

The interaction of a single photon with an individual two-level system is the textbook example of quantum electrodynamics. Achieving strong coupling in this system so far required confinement of the light field inside resonators or…

We study the emission from a molecular photonic cavity formed by two proximal photonic crystal defect cavities containing a small number (<3) of In(Ga)As quantum dots. Under strong excitation we observe photoluminescence from the bonding…

Strong light-matter interactions facilitate not only emerging applications in quantum and non-linear optics but also modifications of materials properties. In particular the latter possibility has spurred the development of advanced…

Mesoscale and Nanoscale Physics · Physics 2021-08-17 Jakub Fojt , Tuomas P. Rossi , Tomasz J. Antosiewicz , Mikael Kuisma , Paul Erhart

Quantum light-matter systems at strong coupling are notoriously challenging to analyze due to the need to include states with many excitations in every coupled mode. We propose a nonperturbative approach to analyze light-matter correlations…

Mesoscale and Nanoscale Physics · Physics 2021-04-15 Yuto Ashida , Atac Imamoglu , Eugene Demler

We report low-temperature transport measurements through a double quantum dot device in a configuration where one of the quantum dots is coupled directly to the source and drain electrodes, and a second (side-coupled) quantum dot interacts…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 D. Y. Baines , T. Meunier , D. Mailly , A. D. Wieck , C. Bäuerle , L. Saminadayar , Pablo S. Cornaglia , Gonzalo Usaj , C. A. Balseiro , D. Feinberg

Semiconductor quantum dot molecules are considered as promising candidates for quantum technological applications due to their wide tunability of optical properties and coverage of different energy scales associated with charge and spin…

Controlling light-matter interactions is emerging as a powerful strategy to enhance the performance of organic light-emitting diodes (OLEDs). By embedding the emissive layer in planar microcavities or other modified optical environments,…

Materials Science · Physics 2026-02-06 Olli Siltanen , Kimmo Luoma , Konstantinos S. Daskalakis

Recent scanning tunnelling microscopy (STM) experiments reported single-molecule fluorescence induced by tunneling currents in the nanoplasmonic cavity formed by the STM tip and the substrate.The electric field of the cavity mode couples…

Mesoscale and Nanoscale Physics · Physics 2019-12-18 Quentin Schaeverbeke , Rémi Avriller , Thomas Frederiksen , Fabio Pistolesi

In many systems consisting of interacting subsystems, the complex interactions between elements can be represented using multilayer networks. However percolation, key to understanding connectivity and robustness, is not trivially…

Disordered Systems and Neural Networks · Physics 2020-11-04 G. J. Baxter , R. A. da Costa , S. N. Dorogovtsev , J. F. F. Mendes

Controlling electrically-stimulated quantum light sources (QLS) is key for developing integrated and low-scale quantum devices. The mechanisms leading to quantum emission are complex, as a large number of electronic states of the system…

Mesoscale and Nanoscale Physics · Physics 2024-02-28 Katharina Kaiser , Anna Rosławska , Michelangelo Romeo , Fabrice Scheurer , Tomáš Neuman , Guillaume Schull

The possibility of strong coupling between a single molecule and surface plasmons is analyzed on the basis of a microscopic classical description. It is predicted that strong single molecule - plasmon coupling can happen for a silver…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Mykhaylo M. Dvoynenko