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Despite the multitude of available methods, the characterisation of ultrafast pulses remains a challenging endeavour, especially at the single-photon level. We introduce a pulse characterisation scheme that maps the magnitude of its…

We propose a novel spectral method for reconstructing quantum wavefunction of an electron pulse, free-electron spectral shearing interferometry (FESSI). We employ a Wien filter to generate two time-delayed replicas of the electron…

Quantum Physics · Physics 2025-08-18 Zhaopin Chen , Bin Zhang , Yiming Pan , Michael Krueger

Accurate and fast characterization of spatiotemporal information of high-intensity, ultrashort pulses is crucial in the field of strong-field laser science and technology. While conventional self-referenced interferometers were widely used…

Optics · Physics 2023-07-19 Yifei Chen , Zhiyuan Huang , Ding Wang , Yu Zhao , Jianhua Fu , Meng Pang , Yuxin Leng , Zhizhan Xu

Attosecond x-ray pulse with known spectro-temporal information is an essential tool for the investigation of ultrafast electron dynamics in quantum systems. Ultrafast free-electron lasers (FELs) have the unique advantage on unprecedented…

Accelerator Physics · Physics 2023-04-17 Yaozong Xiao , Hao Sun , Bo Liu , Zhentang Zhao , Chao Feng

The ability to manipulate and measure the time-frequency structure of quantum light is useful for information processing and metrology. Measuring this structure is also important when developing quantum light sources with high modal purity…

Quantum Physics · Physics 2022-01-12 G. S. Thekkadath , B. A. Bell , R. B. Patel , M. S. Kim , I. A. Walmsley

The ability to characterize the complete quantum state of light is essential for both fundamental and applied science. For single photons the quantum state is provided by the mode that it occupies. The spectral temporal mode structure of…

Single-photon sources are a fundamental resource in quantum optics. The indistinguishability and purity of photons emitted from different sources are crucial (necessary, essential) properties for many quantum applications to ensure…

Quantum Physics · Physics 2020-07-15 Valérian Thiel , Alex O. C. Davis , Ke Sun , Peru D'Ornellas , Xian-Min Jin , Brian J. Smith

We present a technique to completely characterise the spectral-temporal wave function of a broadband photon pair using spectral-shearing interferometry. Our method is fully self-referencing and is generalisable across a wide range of…

Quantum Physics · Physics 2018-09-12 Alex O. C. Davis , Valerian Thiel , Brian J. Smith

A photon is the single excitation of a particular spatiotemporal mode of the electromagnetic field. A precise knowledge of the mode structure is therefore essential for its processing and detection, as well as for applying generic quantum…

We report a new version of spectral phase interferometry for direct electric field reconstruction (SPIDER), which enables consistency checking through the simultaneous acquisition of multiple shears and offers a simple and precise…

Optics · Physics 2019-03-27 Tobias Witting , Dane R. Austin , Ian A. Walmsley

We propose a novel method to reconstruct the spatio-temporal amplitude and phase of the electric field of ultrashort laser pulses using spatially-resolved spectral interferometry. This method is based on a fiber-optic coupler interferometer…

A nonlinear interferometry scheme is described theoretically to induce and resolve electron wave- function beating on time scales shorter than the optical cycle of the time-delayed pump and probe pulses. By employing two moderately intense…

Chemical Physics · Physics 2017-08-23 Christian Ott , Philipp Raith , Thomas Pfeifer

The recent introduction of coherent optical communications has created a compelling need for ultra-fast phase-sensitive measurement techniques operating at milliwatt peak power levels and in time scales ranging from sub-picoseconds to…

We employ two-dimensional (2D) coherent, nonlinear spectroscopy to investigate couplings within individual InAs quantum dots (QD) and QD molecules. Swapping pulse ordering in a two-beam sequence permits to distinguish between rephasing and…

We introduce a self-referenced method for quantum-state tomography of light based on photon-number-resolved double-slit interferometry. Two identical copies of the unknown quantum field illuminate laterally displaced slits, guaranteeing…

Optics · Physics 2025-12-10 Matan Even Tzur

An electrical pulse E(t) is completely defined by its time-dependent amplitude and polarisation direction. For optical pulses the manipulation and characterisation of the light polarisation state is fundamental due to its relevance in…

The generation of ultrafast laser pulses and the reconstruction of their electric fields is essential for many applications in modern optics. Quantum optical fields can also be generated on ultrafast time scales, however, the tools and…

Quantum Physics · Physics 2019-10-02 Jean-Philippe W. MacLean , Sacha Schwarz , Kevin J. Resch

Quantum interferometry methods exploit quantum resources, such as photonic entanglement, to enhance phase estimation beyond classical limits. Nonlinear optics has served as a workhorse for the generation of entangled photon pairs, ensuring…

Quantum Physics · Physics 2025-08-04 Romain Dalidet , Anthony Martin , Grégory Sauder , Laurent Labonté , Sébastien Tanzilli

Fourier transform spectroscopy with classical interferometry corresponds to the measurement of a single-photon intensity spectrum from the viewpoint of the particle nature of light. In contrast, the Fourier transform of two-photon quantum…

Quantum Physics · Physics 2021-11-04 Hiroya Seki , Kensuke Miyajima , Ryosuke Shimizu

We introduce an experimental technique for complete phase-sensitive characterization of arbitrary unitary spectral-temporal transformations of optical modes. Our method recovers the complex spectral transfer function, or Green's function,…

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